气压变化引起地表垂直向位移的估计：与汪福田同志商榷

本文利用理想的弹性半空间及Guterberg水平层状地层模型,估算出10hPa气压在半径100km圆心处,引起地表垂直向位移变化,它的量级很小,只有几毫米。     

华北断块区地震幕与气温异常

本文利用1951-1980年期间中国气温资料研究了1966-1976年间华北断块区地震幕活动与1960年2月-1977年1月气温异常之间的关系。主要结论如下:1.华北断块及其邻近地区1960年2月天气异常增温到1977年1月天气异常降温过程与地震幕活动开始和结束的时间相关联;1967年5月、1973年1月、1975年9月和1976年2月的气温异常与该地震幕中1969年7月18日渤海7.4、1975年2月4日海城7.3和1976年7月28日唐山7.8级三次地震密切相关。2.气温异常时问和异常范围之间以及它们与地震能量之间都有较高的可信度,表明气温异常与地震幕之间有成因上的联系。3.从1960年2月气温异常开始到1976年7月28日唐山7.8级地震发生时的16.5年可按0.618~N划分为18个时段,4次7.0级以上地震和5次气温异常发生的时间恰好位于某几个时间段上。     

Atmospheric pollution assessment near potential source of natural aerosols in the South Gobi Desert region,China

ABSTRACT

Rapid economic growth, a high degree of urbanization and the proximity of a large number of desert and semidesert landscapes can have a significant impact on the atmosphere of adjacent territories, leading to high levels of atmospheric pollution. Therefore, identifying possible sources of atmospheric pollution is one of the main tasks. In this study, we carried out an analysis of spatial and temporal characteristics of five main atmospheric pollutants (PM_2.5, PM₁₀, SO₂, NO₂, and CO) near potential source of natural aerosols, affecting seven cities (Wuhai, Alashan, Wuzhong, Zhongwei, Wuwei, Jinchang, Zhangye), located in immediate proximity to the South Gobi deserts. The results, obtained for the period from 1 January 2016 to 31 December 2018, demonstrate total concentrations of PM_2.5 and PM₁₀ are 38.2 ± 19.5 and 101 ± 80.7 μg/m³ exceeding the same established by the Chinese National Ambient Air Quality Standard (CNAAQS), being 35 and 70 μg/m³, respectively. Based on the data from Moderate Resolution Imaging Spectroradiometer (MODIS) for the whole period, Clean Сontinental (71.49%) and Mixed (22.29%) types of aerosols prevail in the region. In the spring and winter seasons maximum concentrations of pollutants and high values of Aerosol Optical Depth (AOD) in the region atmosphere are observed. PM_2.5 and PM₁₀ ratio shows the presence of coarse aerosols in the total content with value 0.43. The highest concentrations of pollutants were in the period of dust storms activity, when PM_2.5 and PM₁₀ content exceeded 200 and 1000 µg/m³, and AOD value exceeded 1. UV Aerosol Index (UVAI), Aerosol Absorbing Optical Depth (AAOD), and Single Scattering Albedo (SSA), obtained from Ozone Monitoring Instrument (OMI), demonstrate the high content of dust aerosols in the period of sandstorms. Analysis of backward trajectories shows that dust air masses moved from North to Northwest China, affecting large deserts such as Taklamakan, Gurbantunggut, Badain Jaran, Tengger, and Ulan Buh deserts.     

Gas and Particulate Products Distribution from the Photooxidation of α-Humulene in the Presence of NOx, Natural Atmospheric Air and Sunlight

The photooxidation of -humulene in the presence of NO_x, natural sunlight, and rural background air was investigated using a combination of gas chromatography-mass spectrometry (GC-MS) and high performance liquid chromatography (HPLC). Identification and quantification of gas and particulate reaction products were reported over the course of the reaction. The daytime photooxidation was carried out in a large outdoor smog chamber (190 m³). A wide range of ring retaining and ring opening products in the gas and particle phase are reported. On average, measured gas and particle phase products accounted for 44% of the reacted -humulene carbon. Measurements show that a number of reaction products with low vapor pressures (e.g. 3-seco--humulone aldehyde, 7-seco--humulone aldehyde, -humulal aldehyde, -humulene 3-oxide or -humulene 7-oxide, -humulaic/alic acid isomers, and 3-seco--14-hydroxyhumulone aldehyde) were found in the early stage of the reaction and may play an important role in the early formation of secondary organic aerosol. A detailed mechanism is proposed to account for most products observed in this investigation.     

甘肃省春季沙尘暴强弱年份大气环流特征对比分析

文中使用NCEP/NCAR1955～2000年全球月平均再分析网格点资料(2.5°×2.5°纬度/经度)和甘肃省区域性沙尘暴过程资料,分别选取了甘肃省5个春季典型沙尘暴年份和5个春季非沙尘暴年份,对其气候平均的大尺度环流场和有关物理量场的动力和热力结构差异进行了对比分析。初步探讨了甘肃省春季沙尘暴发生与全球海温异常的关系。分析结果表明,甘肃省春季沙尘暴年和非沙尘暴年大尺度高低空环流场和有关物理量场差异明显,从而揭示了沙尘暴形成的大尺度环流以及动力和热力因子影响的事实,以期对我国西北地区沙尘暴气候成因有更全面深入的了解,为沙尘暴短期气候预测提供理论依据和强信号。     

The distribution of meteoric <Superscript>36</Superscript>Cl/Cl in the United States: a comparison of models

The natural distribution of ³⁶Cl/Cl in groundwater across the continental United States has recently been reported by Davis et al. (2003). In this paper, the large-scale processes and atmospheric sources of ³⁶Cl and chloride responsible for controlling the observed ³⁶Cl/Cl distribution are discussed.The dominant process that affects ³⁶Cl/Cl in meteoric groundwater at the continental scale is the fallout of stable chloride from the atmosphere, which is mainly derived from oceanic sources. Atmospheric circulation transports marine chloride to the continental interior, where distance from the coast, topography, and wind patterns define the chloride distribution. The only major deviation from this pattern is observed in northern Utah and southern Idaho where it is inferred that a continental source of chloride exists in the Bonneville Salt Flats, Utah.In contrast to previous studies, the atmospheric flux of ³⁶Cl to the land surface was found to be approximately constant over the United States, without a strong correlation between local ³⁶Cl fallout and annual precipitation. However, the correlation between these variables was significantly improved (R ²=0.15 to R ²=0.55) when data from the southeastern USA, which presumably have lower than average atmospheric ³⁶Cl concentrations, were excluded. The total mean flux of ³⁶Cl over the continental United States and total global mean flux of ³⁶Cl are calculated to be 30.5±7.0 and 19.6±4.5 atoms m^–2 s^–1, respectively.The ³⁶Cl/Cl distribution calculated by Bentley et al. (1986) underestimates the magnitude and variability observed for the measured ³⁶Cl/Cl distribution across the continental United States. The model proposed by Hainsworth (1994) provides the best overall fit to the observed ³⁶Cl/Cl distribution in this study. A process-oriented model by Phillips (2000) generally overestimates ³⁶Cl/Cl in most parts of the country and has several significant local departures from the empirical data.

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Resumen Davis et al. (2003) han informado de la distribución natural de la proporción ³⁶Cl/Cl en las aguas subterráneas de la parte continental de los Estados Unidos de América [EUA]. En este artículo, se discute cuáles son los procesos a gran escala y las fuentes atmosféricas del ³⁶Cl y del cloruro que dan lugar a la distribución observada de ³⁶Cl/Cl.El proceso dominante que afecta a la relación ³⁶Cl/Cl en las aguas subterráneas de origen meteórico a escala continental es el aporte de cloruro estable desde la atmósfera, que procede principalmente de los océanos. La circulación atmosférica transporta el cloruro marino hacia el interior, donde la distancia a la costa, topografía y corrientes del viento definen la distribución del cloruro. La única desviación principal de este esquema tiene lugar al norte de Utah y en el sur de Idaho, donde se deduce que existe una fuente continental de cloruro en los Rellanos Salados de Bonneville (Salt Flats).En contraste con estudios previos (Knies et al. 1994; Phillips 2000), se ha descubierto que el flujo atmosférico de ³⁶Cl hacia la superficie terrestre es aproximadamente constante en todos los estados, sin deducirse una correlación fuerte entre el aporte de ³⁶Cl y la precipitación anual. Sin embargo, la correlación entre estas variables se ve mejorada de forma significativa, con coeficientes de regresión comprendidos entre 0,15 y 0,55, cuando se excluyen los datos recogidos en el sudeste de los EUA, que tienen concentraciones de ³⁶Cl atmosférico presuntamente inferiores a la media. El flujo medio total de ³⁶Cl calculado en la zona continental de los Estados Unidos vale 30,5±7,0 átomos por metro cuadrado y segundo, mientras que el flujo total global de ³⁶Cl es de 19,6±4,5 átomos por metro cuadrado y segundo.La distribución de ³⁶Cl/Cl calculada por Bentley et al. (1986) infravalora la magnitud y variabilidad observada en los valores medidos a lo largo de los Estados Unidos. El modelo propuesto por Hainsworth (1994) proporciona el mejor ajuste conjunto a la distribución observada de ³⁶Cl/Cl en este estudio. El modelo orientado a procesos de Phillips (2000) sobreestima por lo general la distribución de ³⁶Cl/Cl en la mayoría del país y difiere significativamente de algunos valores locales empíricos.

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Résumé La distribution naturelle du rapport ³⁶Cl/Cl dans les eaux souterraines des États-Unis a été récemment présentée par Davis et al. (2003). Dans ce travail, les processus à grande échelle et les sources atmosphériques de ³⁶Cl et de chlorure responsables du contrôle de la distribution observée du rapport ³⁶Cl/Cl sont discutés. Le processus dominant qui affecte le rapport ³⁶Cl/Cl dans les eaux souterraines dorigine météorique à léchelle continentale est lapport atmosphérique de chlorure stable, qui provient pour lessentiel de sources océaniques. La circulation atmosphérique transporte des chlorures marins vers lintérieur des continents, où la distribution de chlorure est définie par la distance à la côte, la topographie et les régimes des vents. La seule exception majeure à ce schéma est observée dans le nord de lUtah et le sud de lIdaho où lon suppose quil existe une source continentale de chlorure dans les bas-fonds salés de Bonneville. Au contraire de précédentes études (Knies et al. 1994; Phillips 2000), on trouve que le flux atmosphérique de ³⁶Cl vers le sol est approximativement constant sur lensemble des États-Unis, sans forte corrélation entre la retombée locale de ³⁶Cl et les précipitations annuelles. Cependant, la corrélation entre ces variables devient significative (R ²=0.15 à 0.55) lorsquon supprime les données du sud-est des États-Unis, dont on pense quelles présentent des concentrations en ³⁶Cl atmosphérique inférieures à la moyenne. Le flux total moyen de ³⁶Cl sur les États-Unis continentaux et le flux moyen global de ³⁶Cl sont respectivement évalués à 30.5 ± 7.0 et 19.6 ± 4.5 atomes.m^–2.s^–1. La distribution du rapport ³⁶Cl/Cl calculée par Bentley et al. (1986) sous-estime lordre de grandeur et la variabilité observés pour la distribution mesurée du rapport ³⁶Cl/Cl sur les États-Unis continentaux. Le modèle proposé par Hainsworth (1994) fournit le meilleur ajustement densemble à la distribution du rapport ³⁶Cl/Cl observée dans cette étude. Un modèle orienté vers les processus proposé par Phillips (2000) surestime dans lensemble le rapport ³⁶Cl/Cl dans la plupart des régions du pays et présente plusieurs désaccords locaux avec les données empiriques.

     

Aging of Titan's Aerosols

Titan's haze is composed of aerosols containing long chain polymers of acetylene with some hydrogen cyanide. These polymers have alternating double/single and triple/single bonds, which can open spontaneously or under the action of UV radiation or particle impact. Once opened, they can induce the opening of a double or triple bond in an adjacent chain and link to it. This cross-linking and chain elongation hardens or “ages” the polymer particles, making them less sticky. As observed experimentally and calculated theoretically, newly formed polymer particles grow by collecting other polymer chains and by complete merging into symmetrical spheres. However, when aged, they merely adhere to each other and do not merge. Eventually, when hard enough, they do not even adhere to each other. In this paper we calculate the spontaneous aging process as applied to Titan's atmospheric conditions and find that the surface tension and viscosity of the aerosols below H∼570 km are one order of magnitude harder than when the aerosols formed. Furthermore, UV irradiation and particle impacts reduce both viscosity and surface tension by an additional factor of 10-100. Thus, the aerosol particles expected to be encountered by the descending Huygens probe will, most likely, be quite hard.     

Estimation of Scalar Source/Sink Distributions in Plant Canopies Using Lagrangian Dispersion Analysis: Corrections for Atmospheric Stability and Comparison with a Multilayer Canopy Model

Source/sink distributions of heat, water vapour andCO₂ within a rice canopy were inferred using aninverse Lagrangian dispersion analysis and measuredmean profiles of temperature, specific humidity andCO₂ mixing ratio. Monin–Obukhov similarity theorywas used to account for the effects of atmosphericstability on _w(z), the standard deviation ofvertical velocity and _L(z), the Lagrangian timescale of the turbulence. Classical surface layer scaling was applied in the inertial sublayer (z > z_ruf)using the similarity parameter = (z - d)/L, where z is height above ground, d is the zero plane displacementheight for momentum, L is the Obukhov length,and z_ruf 2.3h_c, where h_c iscanopy height. A single length scale h_c, was usedfor the stability parameter 3 = h_c/L in the height range 0.25 < z/h_c < 2.5. This choice is justified by mixing layer theory, which shows that within the roughness sublayer there is one dominant turbulence length scaledetermined by the degree of inflection in the windprofile at the canopy top. In the absence of theoretical or experimental evidence for guidance,standard Monin–Obukhov similarity functions, with = h_c/L, were used to calculate the stabilitydependence of _w(z) and _L(z) in the roughness sublayer. For z/h_c < 0.25 the turbulence length and time scales are influenced by the presence of the lowersurface, and stability effects are minimal. With theseassumptions there was excellent agreement between eddycovariance flux measurements and deductions from theinverse Lagrangian analysis. Stability correctionswere particularly necessary for night time fluxes whenthe atmosphere was stably stratified.The inverse Lagrangian analysis provides a useful toolfor testing and refining multilayer canopy models usedto predict radiation absorption, energy partitioningand CO₂ exchanges within the canopy and at thesoil surface. Comparison of model predictions withsource strengths deduced from the inverse analysisgave good results. Observed discrepancies may be dueto incorrect specification of the turbulent timescales and vertical velocity fluctuations close to theground. Further investigation of turbulencecharacteristics within plant canopies is required toresolve these issues.     

Response of Atmospheric Low-frequency Wave to Oceanic Forcing in the Tropics

1. IntroductionInvestigations about atmospheric LFW have been a focus of research since Madden andJulian/s outstanding analysis works (1971, 1972). Many dynamical and thermal mechanisms(Chao et al., 1996; Fu et al., 1998; Hendon et al., 1998; Krishnamurti et al., 1988; Lau andChan, 1988) have been advised to explain LFW. Among them are oceanic effects, such as SSTeffect, thermal forcing and others. Usually atmosphere and ocean are taken as a coupled system, which is used to explain ENS…