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91.
The natural human female hormones oestrone and 17β-oestradiol have been implicated in the disruption of endocrine systems in some wildlife adjacent to sewage effluents. The sorption behaviour of these two compounds under estuarine conditions was studied by spiking either 2.55 μg of oestrone or 2.65 μg of 17β-oestradiol in kinetic experiments. In equilibrium experiments, 3 ng of oestrone or 3.2 ng of 17β-oestradiol was added in each of the centrifuge tubes. Sorption onto sediment particles was relatively slow, with sorption equilibrium being reached in about 70 and 170 h for oestrone and 17β-oestradiol, respectively. The effects of a variety of environmental parameters on sorption were studied including salinity, sediment concentration (SC), the presence of a third phase, particle size and, also, surfactant concentrations. Results show that although salinity did not induce any statistically significant effect on the sorption of 17β-oestradiol, it did statistically enhance the sorption of oestrone, and a salting constant of 0.3 l mol−1 was derived. The partition coefficient for both compounds decreased with increasing sediment concentration, a phenomenon that has been widely reported and attributed to the presence of colloids (which could enhance dissolved concentrations). In this paper, the true partition coefficients for sediment particles (Kptrue) and colloidal particles (Kctrue) have been calculated, and a Kptrue value of 141 and 102 ml g−1 was obtained for oestrone and 17β-oestradiol, respectively. In addition, Kctrue values for oestrone (222×102 ml g−1) and 17β-oestradiol (135×102 ml g−1) were two orders of magnitude higher than their respective Kptrue values, suggesting that the colloidal particles are significantly stronger sorbents for natural oestrogens than sediment particles. Particles of different sizes were found to have different partition coefficients due to the strong relationships between partition coefficients for the two compounds and particulate organic carbon (POC) contents and specific surface areas (SSAs). The presence of a surfactant was shown to reduce the partition coefficients for the two compounds, although its concentrations being used were higher than those normally found in the natural environment. 相似文献
92.
93.
Abstract. The emergence of the Isthmus of Panama subdivided the amphi-American biota. In the present study, Pacific and Atlantic populations of four cognate pairs of crabs were used to discern whether exposure to different thermal regimes in habitats, in the putative absence of gene flow, has resulted in physiological divergence. Populations that potentially form a common genetic pool were also used; these were populations of the Atlantic Panama cognate that occur in Belize and Florida. Decreases in water temperature occur periodically in Pacific Panama and Florida, but not in Atlantic Panama or Belize. In this study, physiological divergence in oxygen uptake was assessed in response to repeated exposure to either control and decreased temperature or control and increased temperature. Results indicate that, in only some of the genera tested, exposure to decreases in habitat temperature has resulted in divergence. Partial support is found for the corollary that adaptation to an environment with periods of decreased temperature results in reduced compensation during exposure to elevated temperature. 相似文献
94.
A repeat hydrographic section has been maintained over two decades along the 180° meridian across the subarctic-subtropical
transition region. The section is naturally divided into at least three distinct zones. In the Subarctic Zone north of 46°N,
the permanent halocline dominates the density stratification, supporting a subsurface temperature minimum (STM). The Subarctic
Frontal Zone (SFZ) between 42°–46°N is the region where the subarctic halocline outcrops. To the south is the Subtropical
Zone, where the permanent thermocline dominates the density stratification, containing a pycnostad of North Pacific Central
Mode Water (CMW). The STM water colder than 4°C in the Subarctic Zone is originated in the winter mixed layer of the Bering
Sea. The temporal variation of its core temperature lags 12–16 months behind the variations of both the winter sea surface
temperature (SST) and the summer STM temperature in the Bering Sea, suggesting that the thermal anomalies imposed on the STM
water by wintertime air-sea interaction in the Bering Sea spread over the western subarctic gyre, reaching the 180° meridian
within a year or so. The CMW in this section originates in the winter mixed layer near the northern edge of the Subtropical
Zone between 160°E and 180°. The CMW properties changed abruptly from 1988 to 1989; its temperature and salinity increased
and its potential density decreased. It is argued that these changes were caused by the climate regime shift in 1988/1989
characterized by weakening of the Aleutian Low and the westerlies and increase in the SST in the subarctic-subtropical transition
region.
This revised version was published online in August 2006 with corrections to the Cover Date. 相似文献
95.
96.
Eurgain H. John Sonia D. Batten Roger P. Harris Graeme C. Hays 《Journal of Sea Research》2001,46(3-4)
Zooplankton sampling has been carried out by the Continuous Plankton Recorder (CPR) survey since the 1930s enabling the study of long-term changes in plankton populations, the elucidation of seasonal patterns of abundance, and more recently providing zooplankton biomass estimates for ecosystem models. Data for zooplankton abundance collected by CPR tows in the Western English Channel (between 1988 and 1998) were compared to vertically integrated samples collected from station L4 off Plymouth, UK. Comparisons were made for locally abundant copepods (including Acartia, Calanus, Para/Pseudocalanus, Centropages, Oithona and Temora) collected by CPR and WP-2 nets. All dominant species recorded at L4 were also common to the CPR data. However, the position of the taxa in the two datasets was not equivalent. Seasonal cycles revealed by CPR data were significantly similar to those recorded throughout the water column at L4 for most taxa. However, absolute levels of abundance differed for the two datasets: abundances were underestimated by CPR samples when compared to those of vertically integrated samples by a factor of between 2 and 35, with the exception of Centropages. The differing mesh sizes (200 and 270 μm) of the WP-2 net and CPR mesh could only partially explain these differences in abundance, implying that the behaviour of individual taxa and their depth in the water column also influenced the abundance recorded. 相似文献
97.
崂山花岗岩地区含锶、偏硅酸矿泉水的形成机理 总被引:1,自引:0,他引:1
报道了崂山花岗岩地区矿泉水的特征。指出其矿泉类型为含锶、偏硅酸型,并讨论了其形成机理。 相似文献
98.
使用切向流超滤系统得到粒度较均匀的Fe(OH)3胶体,进而对Fe(OH)3胶体粒子与Cu2 的作用进行了研究,并将实验结果与南沙群岛海区表层水中铜与胶体物质结合状况的调查数据进行了比较分析,得到如下结果:(1)在海水介质中,铜在Fe(OH)3胶体上结合的百分率(pH>5)随pH的升高而下降,随着Fe(OH)3胶体浓度的减小而下降?(2)在天然海水介质中,使铜在Fe(OH)3胶体上结合的百分率在50%-70%的有机物浓度为1.0mg·L-1,有机物浓度的增大使铜与无机胶体结合的百分率有下降的趋势? 相似文献
99.
100.