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791.
H. E. Scheel H. Areskoug H. Geiss B. Gomiscek K. Granby L. Haszpra L. Klasinc D. Kley T. Laurila A. Lindskog M. Roemer R. Schmitt P. Simmonds S. Solberg G. Toupance 《Journal of Atmospheric Chemistry》1997,28(1-3):11-28
Surface ozone data from 25 Europeanlow-altitude sites and mountain sites located between79°N and 28°N were studied. The analysiscovered the time period March 1989–February 1993.Average summer and winter O3 concentrations inthe boundary layer over the continent gave rise togradients that were strongest in the north-west tosouth-east direction and west-east direction, respectively. WintertimeO3 ranged from 19 to 27 ppbover the continent, compared to about 32 ppb at thewestern border, while for summer the continentalO3 values ranged between 39 and 56 ppb and theoceanic mixing ratios were around 37 ppb. In the lowerfree troposphere average wintertime O3 mixingratios were around 38 ppb, with only an 8 ppbdifference between 28°N and 79°N. For summerthe average O3 levels decreased from about 55 ppbover Central Europe to 32 ppb at 79°N. Inaddition, O3 and Ox(= O3 + NO2)in polluted and clean air were compared. Theamplitudes of the seasonal ozone variations increasedin the north-west to south-east direction, while thetime of the annual maximum was shifted from spring (atthe northerly sites) to late summer (at sites inAustria and Hungary), which reflected the contributionof photochemical ozone production in the lower partsof the troposphere. 相似文献
792.
S. Solberg T. Krognes F. Stordal OØ Hov H. J. Beine D. A. Jaffe K. C. Clemitshaw S. A. Penkett 《Journal of Atmospheric Chemistry》1997,28(1-3):209-225
Simultaneousindependent measurements of NOy and NOx(NOx= NO + NO2) by high-sensitivitychemiluminescence systems and of PAN (peroxyacetylnitrate) and PPN (peroxypropionyl nitrate) by GC-ECDwere made at Spitsbergen in the Norwegian Arcticduring the first half year of 1994. The average mixingratio of the sum of PAN and PPN (denoted PANs)increased from around 150 pptv in early winter to amaximum of around 500 pptv in late March, whereasepisodic peak values reached 800 pptv. This occurredsimultaneously with a maximum in ozone which increasedto 45–50 ppbv in March–April. The average NOxmixing ratio was 27 pptv and did not show any cyclethrough the period. The NOy mixing ratio showeda maximum in late March, while the difference betweenNOy and PAN decreased during spring. This is anindication of the dominance of PAN in the NOybudget in the Arctic, but possible changes in theefficiency of the NOy converter could alsocontribute to this. Although most PAN in theArctic is believed to be due to long range transport,the observations indicate local loss and formationrates of up to 1–2 pptv h-1 in April–May.Measurements of carbonyl compounds suggest thatacetaldehyde was the dominant, local precursor ofPAN.Now at 1. 相似文献
793.
X. Lee H.H. Neumann G. Hartog R.E. Mickle J.D. Fuentes T.A. Black P.C. Yang P.D. Blanken 《Boundary-Layer Meteorology》1997,84(3):383-398
In this paper we report the results of the analysis of two 60-min wave events that occurred in a boreal aspen forest during the 1994 BOREAS (Boreal Ecosystems-Atmosphere Study) field experiment. High frequency wind and temperature data were provided by three 3-D sonic anemometer/thermometers and fourteen fine-wire thermocouples positioned within and above the forest. Wave phase speeds, estimated from information revealed by spectral analysis and linear plane wave equations, are 2.2 and 1.3 m s-1 for the two events. The wavelengths are 130 m and 65 m respectively and are much larger than the vertical wave displacements. There is strong evidence from the present analysis and from the literature supporting our postulate that these waves are generated by shear instability. We propose that wind shear near the top of the stand is often large enough to reduce the gradient Richardson number below the critical value of 0.25 and thus is able to trigger the instability. When external conditions are favorable, the instability will grow into waves. 相似文献
794.
Mechanical aspects of sedimentary basin formation: development of integrated models for lithospheric and surface processes 总被引:1,自引:0,他引:1
S. Cloetingh R. T. Van Balen M. Ter Voorde B. P. Zoetemeijer T. Den Bezemer 《International Journal of Earth Sciences》1997,86(2):226-240
Different assumptions for the thermo-mechanical properties of the lithosphere strongly affect predictions inferred from quantitative sedimentary basin modeling. Examples from various basins, selected as natural laboratories, illustrate the importance of incorporating a finite strength of the extending lithosphere in forward stratigraphic modeling of large-scale basin stratigraphy. Current models can effectively couple erosion at uplifted rift shoulders of extensional basins with the basin fill architecture of the subsiding basin compartments. Modeling of the synrift strata integrates spatial scales characteristic for subbasins, such as the Oseberg field in the North Sea, with large-scale lithospheric properties characterizing the bulk strength of extending lithosphere. Modeling of compressional basins in foreland fold-and-thrust-belt settings can effectively link lithospheric flexure with surface processes. Scales pertinent to short-term spatial and temporal variations in basin fill and basin deformation can now be addressed, allowing the quantitative investigation of consequences of different modes of thrusting for basin fill geometry and facies characteristics. 相似文献
795.
A key ingredient in simulation of flow in porous media is accurate determination of the velocities that drive the flow. Large‐scale irregularities of the geology (faults, fractures, and layers) suggest the use of irregular grids in simulation. This paper presents a control‐volume mixed finite element method that provides a simple, systematic, easily implemented procedure for obtaining accurate velocity approximations on irregular (i.e., distorted logically rectangular) block‐centered quadrilateral grids. The control‐volume formulation of Darcy’s law can be viewed as a discretization into element‐sized “tanks” with imposed pressures at the ends, giving a local discrete Darcy law analogous to the block‐by‐block conservation in the usual mixed discretization of the mass‐conservation equation. Numerical results in two dimensions show second‐order convergence in the velocity, even with discontinuous anisotropic permeability on an irregular grid. The method extends readily to three dimensions. 相似文献
796.
William T. Perkins Nicholas J.G. Pearce John A. Westgate 《Geostandards and Geoanalytical Research》1997,21(2):175-190
This contribution presents a review of the recent developments in laser ablation inductively coupled plasma-mass spectrometry. We describe the important developments which have occurred in the laser systems used, leading to a spatial resolution of around 20 (im, and give an overview of the major instrument developments which have affected the geological applications of laser ablation ICP-MS. We describe the calibration of laser ablation for the analysis of trace elements in two different matrices: volcanic glass shards and sulfide minerals. We show how single glass shards can be analysed using the National Institute of Standards and Technology (NIST) glass certified reference materials for calibration and demonstrate the effect of using single spot analyses compared to rastering of the calibration sample. We show the importance of inter-shard variation and demonstrate that averaged single shard analyses produce data which compare well with bulk analyses. The calibration of the laser system for sulfide mineral analysis is discussed and two different strategies are proposed, one using spiked pressed powder pellets of sulfides and the other metal reference materials. We present conclusions and recommendations for the calibration of laser ablation ICP-MS instruments. 相似文献
797.
Si K- and L-edge ELNES spectroscopy and multiple-scattering (MS) calculations are used to examine mixed Si coordination compounds
varying in SiVI:SiIV ratio. As in previous studies, the edges are influenced mainly by silicon coordination (tetrahedral vs. octahedral), as supported
by the MS calculations. We demonstrate two methods semi-quantitatively to extract the value of SiVI/(SiVI+SiIV): (1) A linear relationship between the L2,3-L1 splitting and SiVI/(SiVI+SiIV) is observed, (2) a fitting method based on the coaddition of reference tetrahedral and octahedral Si spectra is applied
to both Si K- and L-edge ELNES spectra.
Received: February 10, 1997 / Revised, accepted: May 23, 1997 相似文献
798.
799.
S. A. Spaulding D. M. McKnight E. F. Stoermer P. T. Doran 《Journal of Paleolimnology》1997,17(4):403-420
Diatom assemblages in surficial sediments, sediment cores, sediment traps, and inflowing streams of perennially ice-covered Lake Hoare, South Victorialand, Antarctica were examined to determine the distribution of diatom taxa, and to ascertain if diatom species composition has changed over time. Lake Hoare is a closed-basin lake with an area of 1.8 km2, maximum depth of 34 m, and mean depth of 14 m, although lake level has been rising at a rate of 0.09 m yr-1 in recent decades. The lake has an unusual regime of sediment deposition: coarse grained sediments accumulate on the ice surface and are deposited episodically on the lake bottom. Benthic microbial mats are covered in situ by the coarse episodic deposits, and the new surfaces are recolonized. Ice cover prevents wind-induced mixing, creating the unique depositional environment in which sediment cores record the history of a particular site, rather than a lake-wide integration. Shallow-water (<1 m) diatom assemblages (Stauroneis anceps, Navicula molesta, Diadesmis contenta var. parallela, Navicula peraustralis) were distinct from mid-depth (4–16 m) assemblages (Diadesmis contenta, Luticola muticopsis fo. reducta, Stauroneis anceps, Diadesmis contenta var. parallela, Luticola murrayi) and deep-water (26–31 m) assemblages (Luticola murrayi, Luticola muticopsis fo. reducta, Navicula molesta). Analysis of a sediment core (30 cm long, from 11 m water depth) from Lake Hoare revealed two abrupt changes in diatom assemblages. The upper section of the sediment core contained the greatest biomass of benthic microbial mat, as well as the greatest total abundance and diversity of diatoms. Relative abundances of diatoms in this section are similar to the surficial samples from mid-depths. An intermediate zone contained less organic material and lower densities of diatoms. The bottom section of core contained the least amount of microbial mat and organic material, and the lowest density of diatoms. The dominant process influencing species composition and abundance of diatom assemblages in the benthic microbial mats is episodic deposition of coarse sediment from the ice surface. 相似文献
800.
Guillemots Uria spp. account for ca. 70% of the total harvest of prey taken by seabirds breeding in the Barents Sea region. This paper presents guillemot chick diet data collected recently at four localities (Finnmark, Murman, Bjørnøya and Spitsbergen) and collates all the data found by the authors in the literature and in the archives of Tromsø Museum, the Norwegian Polar Institute and Kandalaksha State Nature Reserve. Guillemots consume a wide variety of prey and, in comparison to the harvest by predatory fish and marine mammals, their impact on the Barents Sea ecosystem is considered to be minimal. We point out the need for more systematic collection of data from different regions and at different times of the year before a final impact assessment can be made. 相似文献