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111.
The first analysis of sterols in Antarctic marine sediment cores (Bransfield Strait and McMurdo Sound) is reported here. The isolated sterols in the sediments from Bransfield Strait are comprised mainly of dinosterol (4,23,24-trimethyl-5cholest-22-en-3β-ol), coprostanol (5β-cholestan-3β-ol) and epicoprostanol (5β-cholestan-3-ol) and trace amounts of cholesterol (cholest-5-en-3β-ol). The sediment cores of McMurdo Sound also contain small quantities of coprostanols in addition to large amounts of marine sterols. Dinosterol is a known dinoflagellate chemical marker, whereas coprostanols are currently being used as tracers for sewage contamination. However, sterol composition in Antarctic sediments is expected to be atypical of sewage input and probably different from those of temperate and tropical zones. The coprostanols must therefore arise from the feces of marine mammals, most probably whales which use the region for feeding and spawning. Based on the results of this study, caution should be exercised in the use of coprostanol to estimate the amount of sewage-derived organic matter transported away from impacted coastal areas. 相似文献
112.
C. J. N. Wilson B. F. Houghton B. J. Pillans S. D. Weaver 《Journal of Volcanology and Geothermal Research》1995,69(3-4)
Mayor Island is a peralkaline rhyolitic caldera volcano characterised by numerous, sector-confined pyroclastic deposits, together with lavas forming at least five composite shields. Correlation of sequences between sectors is difficult because of the scarcity of island-wide marker beds. However, eight distal calc-alkaline fall tephras (ca. 7.3 14C ka to 64 ka) from Okataina and Taupo volcanic centres in the nearby Taupo Volcanic Zone (TVZ) have been identified on the island. These “foreign” TVZ tephras provide marker planes to correlate activity in different sectors of Mayor Island volcano, and refine an eruptive chronology. At least seventeen pyroclastic eruptions and fourteen lava-producing events (including multiple, shield-forming events) have occurred in the past ca. 64 ka. Age controls provided by the calc-alkaline tephras confirm the extremely local dispersal characteristics of many of the Mayor Island eruptives and show that K/Ar ages as young as 25–33 ka on obsidians with 4.2–4.4% K2O are reliable. 相似文献
113.
Peter Baccini Erwin Grieder Ruth Stierli Sabine Goldberg 《Aquatic Sciences - Research Across Boundaries》1982,44(1):99-116
The adsorption characteristics of sediment particles from a prealpine Swiss lake were compared with those of γ-aluminum oxide.
Under lake water conditions, i.e. with particle concentration of 2–16 mg/1 and DOC concentrations of 1–4 mg/1 at pH=8, the
adsorption of copper, zinc and orthophosphate is reduced significantly by the presence of natural organic matter (NOM). It
is postulated that the binding sites of the natural mineral surfaces are occupied almost completely by NOM under natural conditions.
A simple ligand exchange model can explain the observed phenomena. 相似文献
114.
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116.
The ratios of some New Zealand peat, lignite and coal samples were measured and compared with those of various coal precursors (cellulose, lignin and plant resins). The results showed that the major source of oxygen in all cases (except that of high rank coal) was from cellulose with the contribution from lignin and plant resins being insignificant. 相似文献
117.
The judicious choice of dipolar dephasing times or carbon magnetization holding times has been shown to improve resolution in solid state nuclear magnetic resonance (NMR) spectra of complex materials. Signals from protonated and alkylated aromatic carbons are reduced to enhance resolution of aromatic oxygenated groups. Rapidly rotating methyl groups can be resolved from other aliphatic carbon types. These techniques were used to investigate the structure of a brown coal, xylite fractions of a brown coal, a bituminous coal, an oil shale and a solvent-refined coal. The results allow estimates of the fraction of aromatic carbon that is protonated in coal to be made, and demonstrate that methyl groups in coal rotate rapidly at room temperature. 相似文献
118.
A. H. Wilson 《Geotechnical and Geological Engineering》1983,1(2):91-187
Summary The characteristics of soft rocks typical of the British Coal Measures are defined and a series of working hypotheses are developed to provide improved design methods for underground roadway and face supports and pillars in coal mines. Proposed design equations are tested against case history data. 相似文献
119.
Luigi Beccaluva Gianluca Bianchini Massimo Coltorti William Perkins Franca Siena Carmela Vaccaro Marjorie Wilson 《Contributions to Mineralogy and Petrology》2001,142(3):284-297
Peridotite xenoliths entrained in Plio-Pleistocene alkali basalts from Sardinia represent fragments of the uppermost lithospheric mantle, and are characterised by an anhydrous four-phase mineral assemblage. They range in bulk rock composition from fertile spinel-lherzolites to residual spinel-harzburgites. The Sr-Nd isotope and trace element composition of clinopyroxene mineral separates varies between LREE-depleted samples with 87Sr/86Sr as low as 0.70262 and 143Nd/144Nd up to 0.51323 and LREE-enriched samples with 87Sr/86Sr up to 0.70461 and 143Nd/144Nd down to 0.51252. The available data suggest that all the studied peridotite samples suffered variable degrees of partial melting during Pre-Mesozoic times (based on Nd model ages relative to CHUR and DMM). The overprinted enrichment is related to a subsequent metasomatism, induced by fluids rising through the lithosphere that preferentially percolated the originally most depleted domains. Despite the occurrence of orogenic volcanism in the area, preferential enrichment in elements typically associated with slab derived fluids/melts (K, Rb, Sr, Th) relative to LREE has not been detected, and metasomatism seems to be more likely related to the infiltration of highly alkaline basic melts characterised by an EM-like Sr-Nd isotopic composition. Similar 87Sr/86Sr-143Nd/144Nd compositions, characterised by an EM signature, are observed in anorogenic mafic lavas and peridotite xenoliths from widespread localities within the "European" plate, whereas they have not previously been recorded in peridotite xenoliths and associated alkaline mafic lavas from the stable "African" lithospheric domain. 相似文献
120.
Summer temperatures in the Canadian Rockies during the last millennium: a revised record 总被引:4,自引:0,他引:4
We present a significant update to a millennial summer temperature reconstruction (1073–1983) that was originally published in 1997. Utilising new tree-ring data (predominantly Picea engelmannii), the reconstruction is not only better replicated, but has been extended (950–1994) and is now more regionally representative. Calibration and verification statistics were improved, with the new model explaining 53% of May–August maximum temperature variation compared to the original (39% of April–August mean temperatures). The maximum latewood density data, which are weighted more strongly in the regression model than ringwidth, were processed using regional curve standardisation to capture potential centennial to millennial scale variability. The reconstruction shows warm intervals, comparable to twentieth century values, for the first half of the eleventh century, the late 1300s and early 1400s. The bulk of the record, however, is below the 1901–1980 normals, with prolonged cool periods from 1200 to 1350 and from 1450 to the late 19th century. The most extreme cool period is observed to be in the 1690s. These reconstructed cool periods compare well with known regional records of glacier advances between 1150 and the 1300s, possibly in the early 1500s, early 1700s and 1800s. Evidence is also presented of the influence of solar activity and volcanic events on summer temperature in the Canadian Rockies over the last 1,000 years. Although this reconstruction is regional in scope, it compares well at multi-decadal to centennial scales with Northern Hemisphere temperature proxies and at millennial scales with reconstructions that were also processed to capture longer timescale variability. This coherence suggests that this series is globally important for the assessment of natural temperature variability over the last 1,000 years.Authors are listed alphabetically 相似文献