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241.
Quantification of river water infiltration in shallow aquifers using acesulfame and anthropogenic gadolinium 下载免费PDF全文
This study has investigated the use of the artificial sweetener acesulfame and the magnetic resonance imaging contrast agent gadolinium as quantitative tracers for river water infiltration into shallow groundwater. The influence of a river on alluvial groundwater in a subalpine catchment in western Europe has been assessed using the ‘classical’ hydrochemical tracer chloride and the trace contaminants acesulfame and anthropogenic gadolinium. Mixing ratios for riverine bank filtrate with ambient groundwater and the uncertainties associated with the temporal and spatial tracer variability were calculated using acesulfame and gadolinium and compared with those obtained using chloride. The temporal variability of tracer concentrations in river water of gadolinium (standard deviation SD: 63%) and acesulfame (SD: 71%) both exceeded that of chloride (SD: 27%), and this was identified as the main source of uncertainty in the mixing analysis. Similar spatial distributions were detected in the groundwater for chloride and gadolinium, but not for acesulfame. Mixing analyses using acesulfame resulted in calculated mixing ratios that differed from those obtained using gadolinium and chloride by up to 83% and 92%, respectively. At the investigated site, which had oxic conditions and moderate temperatures, acesulfame was found to be a less reliable tracer than either gadolinium or chloride, probably because of natural attenuation and input from other sources. There was no statistically significant difference between the mixing ratios obtained using chloride or gadolinium, the mixing ratios obtained using gadolinium were 40–50% lower than those obtained using chloride. This is mainly due to a bias of the mean gadolinium concentration in river water towards higher values. In view of the uncertainties of the two tracers, neither could be preferred over the other for the quantification of bank filtrate in groundwater. At this specific site gadolinium was able to reliably identify river water infiltration and was a more precise tracer than chloride at low mixing ratios (<20%), because of the exclusive occurrence of gadolinium in river water and its high dynamic range. Copyright © 2015 John Wiley & Sons, Ltd. 相似文献
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To explore planetary evolution, we provide conductive cooling profiles that account for planet size, phonon diffusivity and various internal heating scenarios. Our new analytical solution for simple cooling of spheres reveals that heat is removed from only Earth's outermost ~1000 km over geological time. Numerical models with decaying heat production show that any upward concentration of radionuclides causes high temperatures at shallow depths, forcing interior temperatures to increase with time while producing a thermal gradient that forbids lower mantle convection. Hence, differentiation drives upper mantle magmatism and tectonics, leaving a quiescent but hot deep interior, while slowly melting the core. 相似文献
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Alice Schaffhauser Serge Payette Michelle Garneau Élisabeth C. Robert 《Boreas: An International Journal of Quaternary Research》2017,46(3):428-441
The initiation and growth of boreal peatlands developed on well‐drained, sandy landforms are closely associated with podzolic soil paludification processes. The origin of Sphagnum bogs extending on large deltaic plains was examined to test the hypothesis of the dual impact of indurated (ortstein) podzols and fire on forest soil paludification and concurrent peatland initiation and expansion. Mineral soil, basal organic matter and peat monoliths were sampled for soil and macrofossil analyses along an 800‐m toposequence starting from a mixed‐wood boreal forest to a Sphagnum bog (Lebel bog, eastern Quebec, Canada), and ending at a peat dome in the thickest section of the peatland. Mineral soils along the toposequence are ortstein humo‐ferric podzols distributed in the forest environment and beneath Sphagnum peat in the bog, except at the peat dome. Initial peatland growth occurred c. 6000 cal. a BP. Soil paludification coincided with the cessation of fire occurrence as recorded in the organic and mineral layers preceding Sphagnum expansion. Unlike most temperate and boreal raised bogs, the Sphagnum bog developed directly from a forest environment without passing through a transitional fen stage. Conifer forests regenerated successively after several fires between 4200 and 1600 cal. a BP before bog expansion. Pre‐bog forests were composed of fire‐prone black spruce (Picea mariana) and jack pine (Pinus banksiana) trees, and ericaceous species. Given the distribution and thickness of ortstein horizons progressively decreasing and disappearing towards the peatland dome, growth and expansion of the Sphagnum bog was not caused by soil induration processes, which could have potentially impeded vertical and horizontal drainage. The development of indurated podzols outside and several hundred metres inside the peatland preceded the initiation and expansion of the Sphagnum bog. Cessation of fire activity appears to be a key factor facilitating the lateral expansion of the Sphagnum bog under wet soil conditions. 相似文献
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Robert S. Sommer Norbert Benecke Lembi Lõugas Oliver Nelle Ulrich Schmölcke 《第四纪科学杂志》2011,26(8):805-812
The wild horse Equus ferus was one of the most frequent species of the Late Pleistocene large ungulate fauna in Eurasia and played an important role in the subsistence of human groups, especially at the end the Late Glacial. It is frequently assumed that E. ferus became extinct in Europe at the beginning of the Holocene because of the development of woodlands and loss of open habitats. Because of its preference for open habitats and in spite of its adaptability, the appearance or disappearance of the wild horse could therefore be a suitable palaeoecological indicator for the opening of the Holocene primeval woodlands. We revised the dating and reliability of the subfossil record and dated several bones by atomic mass spectrometry 14C dating. From the beginning of the Holocene (9600 cal a BC) to the end of the Atlantic Period (3750 cal a BC) there are 207 archaeological sites with wild horse records available in Europe. E. ferus survived the Pleistocene Holocene transition in Europe, but the spatiotemporal dynamics of populations fluctuated remarkably in the early and middle Holocene. Small and sparse populations increasingly became extinct during the early Holocene, until between 7100 and 5500 cal a BC the wild horse was almost absent in central parts of the European Lowlands. Particular conditions in natural open patches in the canopy forests, chalklands and floodplains may have maintained the local survival of the horse in some regions of the Lowlands, however. In the Late Atlantic, between 5500 and 3750 cal a BC the range of the wild horse was again extended. It re‐immigrated into central and western Europe, probably as a consequence of increasing landscape opening by Neolithic peoples. The data presented here may be a valuable part of the debate on the degree of openness of the early and middle Holocene landscape. Copyright © 2011 John Wiley & Sons, Ltd. 相似文献
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Jeffrey Robert Thompson 《Geological Journal》2015,50(4):550-551
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Growth mechanisms and geochemistry of carbonate concretions from the Cambrian Wheeler Formation (Utah,USA) 下载免费PDF全文
Carbonate concretions provide unique records of ancient biogeochemical processes in marine sediments. Typically, they form in organic‐rich mudstones, where a significant fraction of the bicarbonate required for carbonate precipitation is supplied from the decomposition of organic matter in the sediments. As a result, carbonates that comprise concretions are usually characterized by broad ranges in δ13C and include values that are significantly depleted relative to seawater. This article reports results from a physical, petrographic and geochemical analysis of 238 concretions from the Wheeler Formation (Cambrian Series 3), Utah, USA, which are unusual in several respects. Most prominently, they formed in organic‐poor mudstones (total organic carbon = 0·1 to 0·5%) and are characterized by a narrow range of δ13C that onlaps the range of contemporaneous seawater values. Subtle centre to edge trends in δ13C demonstrate that concretion precipitation was initiated by local chemical gradients set up by microbial activity in the sediments, but was sustained during growth by a large pool of inorganic bicarbonate probably derived from alkaline bottom waters. The large inorganic pool appears to have been important in facilitating rapid precipitation of the concretion matrix, which occurred via both displacive and replacive carbonate precipitation during early diagenesis. Stable isotope data from cogenetic pyrite (δ34S) and silica (δ18O) phases provide insight into the evolution of biogeochemical processes during concretion growth, and suggest that concretions were formed almost entirely during sulphate reduction, with only minor modification thereafter. Concretions of the Wheeler Formation appear to represent an end‐member system of concretion formation in which rapid growth was promoted by ions supplied from sea‐water. As such, they offer insight into the spectrum of processes that may influence the growth of carbonate concretions in marine sediments. 相似文献
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