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71.
Carbon isotopic fractionation in lipids from methanotrophic bacteria: relevance for interpretation of the geochemical record of biomarkers 总被引:11,自引:0,他引:11
Experiments with cultured aerobic methane oxidising bacteria confirm that their biomarker lipids will be significantly depleted in 13C compared to the substrate. The methanotrophic bacteria Methylococcus capsulatus and Methylomonas methanica, grown on methane and using the RuMP cycle for carbon assimilation, show maximum 13C fractionation of approximately 30% in the resultant biomass. In M. capsulatus, the maximum fractionation is observed in the earliest part of the exponential growth stage and decreases to approximately 16% as cells approach stationary phase. This change may be associated with a shift from the particulate form to the soluble form of the methane monooxygenase enzyme. Less than maximum fractionation is observed when cells are grown with reduced methane availability. Biomass of M. capsulatus grown on methanol was depleted by 9% compared to the substrate. Additional strong 13C fractionation takes place during polyisoprenoid biosynthesis in methanotrophs. The delta 13C values of individual hopanoid and steroid biomarkers produced by these organisms were as much as l0% more negative than total biomass. In individual cultures, squalene was 13C-enriched by as much as 14% compared to the triterpane skeleton of bacteriohopaneaminopentol. Much of the isotopic dispersion in lipid metabolites could be attributed to shifts in their relative abundances, combined with an overall reduction in fractionation during the growth cycle. In cells grown on methanol, where there was no apparent effect of growth stage on overall fractionation there were still significant isotopic differences between closely related lipids including a 5.3% difference between the hopane and 3 beta-methylhopane skeletons. Hopane and sterane polyisoprenoids were also 13C-depleted compared to fatty acids. These observations have significant implications for the interpretation of specific compound isotopic signatures now being measured for hydrocarbons and other lipids present in sediments and petroleum. In particular, biomarker lipids produced by a single organism do not necessarily have the same carbon isotopic composition. 相似文献
72.
On the basis of issues raised by observations of BL Lac objects and the qualitative jet model proposed by Bakeret al. in 1988, we have been led to consider the quantitative role of coherent, stimulated emission in jets and construct a new jet model of blazars in which a relativistic electron beam with an axial symmetric, power-law distribution is injected from the central engine into the jet plasma. We study quantitatively the synchrotron emission of the relativistic electron beams. Using the weak turbulent theory of plasma, we discuss the interaction between relativistic electron beams and jet plasma, and the roles of stimulated emission. The main results are:
- The synchrotron emission increases sensitively with the increase of the angle between the direction of the beam and the magnetic field. When the direction of the beam is vertical to the magnetic field, the synchrotron emission reaches its maximum, i.e. the emitted waves are beamed in the direction of the jet axis. We suggest that radio selected BL Lac objects belong to this extreme classification.
- The synchrotron emission of the relativistic beam increases rapidly with the increase of the Lorentz factor of the relativistic electron,γ, whenγ ≤ 22.5, then decreases rapidly with increase ofγ.
- The stimulated emission also increases with increasing Lorentz factorγ of the relativistic electrons whenγ ≤ 35 and then decreases with the increasingγ. The maximum stimulated emission and the maximum synchrotron emission occur at different frequencies. Stimulated emission is probably very important and reasonable flare mechanism in blazars.
- The rapid polarization position angle (PA) swings may arise from the interaction between the relativistic electron beam and the turbulent plasma.
73.
Z. Borovec 《GeoJournal》1993,29(4):359-364
Sequential extraction of the fine fraction (63 µm) of the bottom sediments of the Labe river in Central Bohemia indicates that the readily reducible sediment fraction is a major reservoir of silver for release into the aqueous phase. Molybdenum is preferentially mobilized by ion-exchange, while beryllium is accumulated in all the chemical fractions of the sediments, especially in the moderately reducible and the organic/sulphidic phases.Contamination of the aquatic system from anthropogenic sources is characterized by the formation of relatively unstable chemical forms and only a small portion of these elements remain in the stable residual fraction. 相似文献
74.
Dr. J. Ulrych Dr. E. Pivec Dr. K. Zák Dr. J. Bendl Dr. P. Bosák 《Mineralogy and Petrology》1993,48(1):65-81
Summary Dykes of alkaline and ultramafic carbonate lamprophyres (monchiquite-ouachitite and aillikite) intrude the Carboniferous sediments of Central Bohemia. Their characteristic feature is the presence of substantial amounts of a sodalite group mineral (presumably haüyne), carbonate and barite. Isotopic compositions of
13C (–3.4 to –6.2) and
18O ( + 13.5 to + 15.9) indicate that the carbonate is of primary magmatic origin and that fluids were formed at temperatures of 500 to 350°C. High contents of CO2 (3.6 to 17.6 wt.%) and incompatible elements, high LREE/HREE ratios (30.0 to 57.7), and low Rb/Sr (0.025 to 0.078) and87Sr/86Sr (0.7038 to 0.7042) ratios suggest the ultramafic lamprophyres are related to deep-seated carbonated magmas of mantle origin. Low degree of partial melting ( < 1%) of the mantle peridotite is envisaged, with additional transport of fluids rich in incompatible elements into the crustal chamber. Alkaline lamprophyres are fractionated derivatives which originated from the same source. Magma intrusion from different levels of a magma chamber into fracture zones under horizontal tension without a central intrusion could result in variability in lamprophyre composition (cumulates or evolved derivatives).
With 8 Figures 相似文献
Alkalische und ultramafische Karbonat-Lamprophyre der zentralen böhmischen Karbonbecken, Tschische Republik
Zusammenfassung Alkalische und ultramafische Karbonat-Lamprophyrgänge (Monchiquit-Ouachitit und Aillikit) intrudieren in karbonische Sedimente Zentralböhmens. Sie sind charakterisiert durch das Auftreten von beträchtlichen Mengen an Mineralen der Sodalith-Gruppe (v.a. Haüyn), Karbonaten und Baryt. Ihre Isotopenzusammensetzung von 13C (–3.4 bis –6.2) und 18O (13.5 bis 15.9) zeigt, daß die Karbonate primär magmatischen Ursprungs sind und daß assoziierte Fluide in einem Temperaturbereich von 350 bis 500°C gebildet wurden. Hohe Gehalte an CO2 (3.6 bis 17.6 Gew. %), inkompatiblen Elementen, hohe LREE/HREE-Verhältnisse (30.0 bis 57.7), sowie niedrige Rb/Sr—(0.025 bis 0.078) und87Sr/86Sr-(0.7038 bis 0.7042) Verhältnisse lassen vermuten, daß die ultramafischen Lamprophyre mit karbonatischen Magmen des Mantels in Beziehung stehen. Eine niedrige Aufschmelzungsrate ( < 1%) von Mantelperidotit mit zusätzlichem Transport von, an inkompatiblen Elementen angereicherten Fluiden, in die krustale Magmenkammer wird diskutiert. Alkalische Lamprophyre sind als stärker fraktionierte Magmen, die derselben Quelle entstammen, zu verstehen. Die Intrusion der aus verschiedenen Bereichen der Magmenkammer stammenden Magmen in durch horizontale Dehnung verursachte Störungszonen könnte das Fehlen eines zentralen Intrusionskörpers und die unterschiedliche Zusammensetzung der Lamprophyre (Kumulate oder entwickelte Derivate) erklären.
With 8 Figures 相似文献
75.
It has been argued that the loss-cone-driven electron cyclotron maser instability can account for the properties of millisecond microwave spike bursts observed during some solar flares. However, as it propagates outward from the corona, maser radiation undergoes gyroresonance absorption when its frequency is a harmonic of the local electron-cyclotron frequency. Existing analytical models using slab geometries predict that this absorption should be sufficiently strong to prevent the radiation from being seen at the observed levels, except under highly restrictive conditions or for unrealistic plasma parameters. A more comprehensive analysis is presented here to determine if and when maser radiation can escape to produce microwave spike bursts. This analysis employs numerical raytracing and incorporates propagation and absorption of fundamental maser emission in a realistic model of a coronal flux loop. It is found that ranges of physical conditions do exist under which maser radiation can escape to an observer and that these conditions are much more limiting for fundamental emission in the extraordinary ()-mode than in the ordinary (o)-mode. Detailed investigation implies that escaping radiation in the -mode is highly directional and chiefly observable toward the center of the solar disk, while escapingo-mode radiation is found to emerge from the corona over a much wider range of directions, with some cases corresponding to radiation observable near the solar limb. 相似文献
76.
We analyse conditions of the innermost portion of an accretion disk and establish a set of equations for this region. A stable innermost region may exist, which can probably explain the observed UV and X-ray spectra, avoiding the unstable emission. We then discuss the detailed radial structure of a disk around a black hole for typical AGN parameters and obtain different kinds of- relationships for different regions of a disk. On the basis of this, we discuss the stability. A new type of cycle is present, which we call a double S shaped cycle. In this cycle, the extent of accretion rate variability is much larger than that in dwarf nova cycles. This probably solves the problem of violent variability of AGN. In the meantime, the very high accretion rate at the hottest state in limit cycles in the unstable region may provide continuous injection of matter to the jet and power the relativistic motion of the jet. 相似文献
77.
First, a sequence of four-zone models for the interior of Venus is constructed under the assumption of hydrostatic equilibrium. While the equation of state for each zone is taken to be the Bullen's relation with its coefficients consistent with the PREM Earth model (Dziewonski and Anderson, 1981), the position of core-mantle boundary is determined by matching solutions of the Emden's equation in different regions. The results of hydrostatic models indicate the presence of a reasonably large molten iron core in Venus, broadly similar to the Earth. It is also found that the position of the core-mantle interface is nearly model-independent. Second, we focus on the question why Venus does not possess a significant global magnetic field and on what we can learn from this fact. Solutions of magnetohydrodynamic equations appropriate for the molten core of Venus are discussed. It is argued that, because the Elsasser number measuring the relative importance of Coriolis and Lorentz forces satisfies 1, equations for the problem of thermal convection in the Venusian fluid core must be nearly uncoupled with the dynamo equation. The existence of a global magnetic field, though small, then suggests that the size of the magnetic Reynolds numberR
m
must beR
m
=O(10), sustaining a dynamo action near its marginal state but not an active dynamo in the Venusian molten core. On the basis of asymptotic relations for finite amplitude convection, a useful constraint on important physical parameters for the liquid core of Venus is derived and discussed. 相似文献
78.
Abstrakt The Kle search programme for minor planets using 0,63m Maksutov camera of Kle Observatory was begun in 1977 as a long-term project continuing up to the present day. The discovery frequency according to seasons in the year shows multiple differences between particular months.The comparison with the number of observing nights and obtained search plates; weather conditions and other influences will be discussed. The Kle minor planet discovery frequency also will be compared with the data base of all numbered minor planets. 相似文献
79.
In this note we derive an exact solution of transfer equation in a plane-parallel semiinfinite atmosphere with albedo >1, by the method of Laplace transform and Wiener-Hopf technique. The emergent intensityI(0, ) is obtained in terms of theH
0-functionH
0() (Das Gupta, 1978) for which some good approximations are given. Intensity at any depth is also obtained.I(0, )/I(0, 0) is plotted in graphs against [0,1], and shows a maximum which drops and shifts towards the origin as increases. 相似文献
80.
D. M. Z. Jassur 《Astrophysics and Space Science》1980,67(1):19-30
Photometric observations of the short-period (RS CVn-type) eclipsing binary system CG Cyg have been presented. Two sets of results, obtained from an analysis of theB, V andR light curves, represent ‘occultation’ and ‘transit’ solutions. The occultation solution is preferred as it gives a better fit to the colour curve. This hypothesis may also offer a more promising explanation of the observed peculiarities such as period changes and the light variation outside eclipses. 相似文献