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81.
When reference frames and diffusing components are properly selected, the flux equations for diffusion of the major components in natural garnets may often be approximated by: J DC. In such cases it is shown that, for reasonable diffusion coefficients and boundary conditions, observed zoning profiles in natural garnets may be explained with pure diffusion models. These models allow for original inhomogeneities in the host rock and may be used to explain why single hand specimens may show such a variety of zoning profiles within a single mineral species. 相似文献
82.
The sorption of silver by poorly crystallized manganese oxides was studied using synthesized samples of three members of the manganous manganite (birnessite) group, of different chemical composition and crystallinity, and a poorly organized γ-MnO2. All four oxides sorbed significant quantities of silver. The manganous manganites showed the greatest sorption (up to 0.5 moles silver/mole MnOx at pH 7) while the γ-MnO2 showed the least (0.3 moles silver/ mole MnOx at pH 7). Sorption of silver was adequately described by the Langmuir equation over a considerable concentration range. The relationship failed at low pH values and high equilibrium silver concentrations. The sorption capacity showed a direct relationship with pH. However, the rate of increase of sorption capacity decreased at the higher pH values.Silver sorption maxima. were not directly related to surface area but appeared to vary with the amount of occluded sodium and potassium present in the manganese oxide. The important processes involved in the uptake of silver by the four poorly crystallized manganese oxides ara considered to be surface exchange for manganese, potassium and sodium as well as exchange for structural manganese, potassium and sodium. 相似文献
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Europa's surface is chemically altered by radiolysis from energetic charged particle bombardment. It has been suggested that hydrated sulfuric acid (H2SO4·nH2O) is a major surface species and is part of a radiolytic sulfur cycle, where a dynamic equilibrium exists between continuous production and destruction of sulfur polymers Sx, sulfur dioxide SO2, hydrogen sulfide H2S, and H2SO4·nH2O. We measured the rate of sulfate anion production for cyclo-octal sulfur grains in frozen water at temperatures, energies, and dose rates appropriate for Europa using energetic electrons. The measured rate is GMixture(SO42−)=fSulfur (r0/r)βG1 molecules (100 eV)−1, where fSulfur is the sulfur weight fraction, r is the grain radius, r0=50 μm, β≈1.9, and G1=0.4±0.1. Equilibrium column densities N are derived for Europa's surface and follow the ordering N(H2SO4) » N(S)>N(SO2)>N(H2S). The lifetime of a sulfur atom on Europa's surface for radiolysis to H2SO4 is τ(−S)=120(r/r0)β years. Rapid radiolytic processing hides the identity of the original source of the sulfurous material, but Iogenic plasma ion implantation and an acidic or salty ocean are candidate sources. Sulfate salts, if present, would be decomposed in <3800 years and be rapidly assimilated into the sulfur cycle. 相似文献
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Leon Bagas David L. Huston James Anderson Terrence P. Mernagh 《Mineralium Deposita》2007,42(1-2):127-144
Significant gold deposits in the western Tanami region of Western Australia include deposits in the Bald Hill and Coyote areas. The ca. 1,864 Ma Bald Hill sequence of turbiditic and mafic volcanic rocks hosts the Kookaburra and Sandpiper deposits and a number of smaller prospects. The ca. 1,835 Ma turbiditic Killi Killi Formation hosts the Coyote deposit and several nearby prospects. The Kookaburra deposit forms as a saddle reef within a syncline, and the Sandpiper deposit is localized within graphitic metasedimentary rocks along a limb of an anticline. Gold in these deposits is hosted by anastomosing quartz–(–pyrite–arsenopyrite) veins within quartz–sericite schist with disseminated arsenopyrite, pyrite, and marcasite (after pyrrhotite). Based on relative timing relationships with structural elements, the auriferous veins are interpreted to have been emplaced before or during the ca. 1,835–1,825 Ma Tanami Orogeny (regional D1). Gold deposition is thought to have been caused by pressure drops associated with saddle reef formation (Kookaburra) and chemical reactions with graphitic rocks (Sandpiper). The Coyote deposit, the largest in the western Tanami region, consists of a number of ore lenses localized along the limbs of the Coyote Anticline, which formed during the Tanami Orogeny. The largest lenses are associated with the Gonzalez Fault, which is located along the steeply dipping southern limb of this fold. Gold was introduced at ca. 1,790 Ma into dilatant zones that formed in local perturbations along this fault during later reactivation (regional D5) towards the end of a period of granite emplacement. Gold is associated with quartz–chlorite–pyrite–(arsenopyrite–galena–sphalerite) veins with narrow (<?5 mm) chloritic selvages. A quartz–muscovite–biotite–K–feldspar–(tourmaline–actinolite–arsenopyrite) assemblage, which is interpreted to relate to granite emplacement, overprints the regional greenschist facies metamorphic assemblage. The mineralogical similarity between this overprinting assemblage and the vein assemblage suggests that the auriferous veins at the Coyote deposit are associated with the granite-related metamorphic–metasomatic assemblage. Gold deposition is thought to have been caused by pressure drops within dilatant zones. 相似文献
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John B. Anderson Richard Wheeler Charles P. Dunning Sue Shepley Marion Fowke 《Environmental Geology》1978,2(2):67-78
A historical record of the effects of human development upon Lake Macatawa is established using geologic criteria. Significant
cultural events are recognized using the pollen record, particularly ambrosia/vesiculate pollen ratios, and occurrences of
detrital and chemical contaminants within the more recent sedimentary column. Detrital contaminants include such things as
cinder and ash from coal burning power plants and animal hair from early tanning operations. Trace metal contaminants, frequently
associated with specific industrial events, are particularly useful in establishing a modern sedimentary chronology.
The impact of human activity upon Lake Macatawa is measured using fossil diatoms. The advantage of this method of environmental
impact assessment is that it provides a historical perspective in which changes within an environment are related to its natural
conditions. 相似文献
90.
Self-diffusion of oxygen in a natural phlogopite mica (annite 4%) has been measured under hydrothermal conditions at 2000 bars pressure and from 500 to 800°C using water enriched in18O. Diffusional transport is dominantly parallel to the c crystallographic axis. A linear Arrhenius plot was obtained with a pre-exponential term = (1.03 ± 0.38) × 10?9cm2sec?1 a and an activation energy of 29 ± 2kcal/g-atom O. The difference in transport rate between oxygens in the OH groups and those in tetrahedral sites is small to non-existent unless the OH oxygens diffuse much more slowly than the other oxygens, which we consider unlikely. A typical phlogopite crystal, 0.2 mm thick by 1 mm across will lose radiogenic argon faster than it will exchange oxygen at temperatures above 435°C, but the reverse holds at lower temperatures if the diffusion mechanism can be extrapolated to temperatures below 500°C. Such a crystal will lose only 5% of its argon if held at 380°C for 1 m.y., but could exchange 27% of its oxygen in that time. The rate at which phlogopite will undergo deformation by diffusional creep does not appear to be controlled by oxygen diffusion. 相似文献