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41.
To investigate the solubility and the sites of incorporation of hydrogen in olivine as a function of point defect concentration, two-stage high-temperature annealing experiments have been carried out. The first annealing stage (the dry preannealing stage) was conducted at a total pressure of 0.1 MPa, a temperature of 1300° C and various oxygen fugacities in the range 10?11–10?4 MPa for times > 12 h. In these heat treatments, the samples were buffered against either orthopyroxene or magnesiowustite, or they remained unbuffered. The second annealing stage (the hydrothermal annealing stage) was performed at 300 MPa and 900–1050 ° C under a hydrogen fugacity of ~ 158 MPa for 1–5 h. Infrared spectra from the annealed samples revealed two distinct groups of bands. Group I bands occurred at wavenumbers in the range 3450–3650 cm?1, while Group II bands occurred in the range 3200–3450 cm?1. The hydrogen solubility associated with Group I bands is proportional to f O 2 to the 1/6 power for samples preannealed in contact with orthopyroxene, to the 1/3 power for samples preannealed in contact with magnesiowustite, and to the 1/13 power for samples preannealed in the absence of a solid-state buffer. The hydrogen concentration for Group II bands varies with f o 2 to the 1/3 power for opxbuffered samples, to the 1/2 power for mw-buffered samples, and to the 1/3 power for unbuffered samples. The dependence of hydrogen solubility on oxygen fugacity and orthopyroxene activity suggests that hydrogen is incorporated into the olivine structure via association with point defects. The presence of two distinct groups of absorption bands indicates that hydrogen is associated with two distinct lattice defects. The following point defect model for the mechanism of incorporation of hydrogen in olivine is consistent with these results: Hydrogen ions responsible for the Group I bands are associated with doubly charged oxygen interstitials, while hydrogen ions responsible for the Group II bands are associated with singly charged oxygen interstitials. Furthermore, the infrared bands observed in naturally derived olivines are present in spectra from our hydrothermally annealed crystals. Thus, the mechanisms of incorporation of hydrogen in olivine under geological conditions are the same as those operative under laboratory conditions. The maximum solubility reached in these experiments was ~ 360H/106Si, which corresponds to ~ 0.002 wt% of H2O. This value is a lower bound for the solubility of hydrogen in olivine under upper mantle conditions. 相似文献
42.
R.G. Smith E.J. Brooker D.J. Douglas E.S.K. Quan G. Rosenblatt 《Journal of Geochemical Exploration》1984,21(1-3)
This paper discusses the application of the newly developed ELAN 250 I.C.P./mass spectrometer to exploration geochemistry. This instrument combines an inductively coupled plasma with a quadrupole mass spectrometer. The combination of these two existing technologies makes it possible for the first time to perform stable-isotope and elemental analysis rapidly and concurrently.Particular attention is paid to the use of lead isotopes to type Au and base-metal occurrences. Data are presented on galena samples obtained from the Geological Survey of Canada and the Royal Ontario Museum. Consideration is also given to the potential usefulness of Pb isotopes and trace-element data to type mineral occurrences and to identify new ones. 相似文献
43.
通过对以《有泰拉萨天气日志》为主的历史文献资料的深入挖掘 ,作者分析了 1 90 4年 2月 9日~ 1 90 7年 4月 1 7日拉萨的气候特征 :气候温暖 ,暖冬现象显著 ,而且 1 90 5年气温高于 1 90 4年 ;干旱气候占主导地位 ,间有多雨期 ;天气多变 ,多风 ,有雾 ;水灾、雪灾、干旱等自然灾害严重。拉萨与全球同时段的气候变化大体一致。 相似文献
44.
麦兹火山-沉积盆地内铅锌矿呈似层状、透镜状,矿石构造以条纹条带状、块状、斑杂状为主,矿物成分相对简单,矿体直接容矿围岩为火山-沉积岩.矿床δ34S值为-20.6‰~-10‰;矿床石英流体包裹体水的δD值为-89.1‰~-49.48‰,δ18OSMOW值为4.7‰~1.2‰.矿化层中方解石的δ13C值介于-6.7‰~-14.3‰之间,δ18O值在10.3‰~12.9‰之间.矿床属火山-沉积岩容矿的块状硫化物矿床,介于典型的火山岩容矿的块状硫化物型矿床(VHMS)和典型沉积岩容矿的硫化物矿床(SEDEX型)之间的过渡类型(一种新类型块状硫化物矿床). 相似文献
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吉林省是我国非金属矿产资源较丰富的大省之一,矿泉水资源也质优量大,且具有竞争优势,开发利用率极为可观。本文从非金属的深细加工、尾矿利用,矿业结构调整以及矿泉水的开发规模等方面探讨了利用我省的资源发展地方经济的后发优势等问题。 相似文献
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