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The release of dissolved actinium to the ocean: A global comparison of different end-members

The measurement of short-lived ²²³Ra often involves a second measurement for supported activities, which represents ²²⁷Ac in the sample. Here we exploit this fact, presenting a set of 284 values on the oceanic distribution of ²²⁷Ac, which was collected when analyzing water samples for short-lived radium isotopes by the radium delayed coincidence counting system. The present work compiles ²²⁷Ac data from coastal regions all over the northern hemisphere, including values from ground water, from estuaries and lagoons, and from marine end-members. Deep-sea samples from a continental slope off Puerto Rico and from an active vent site near Hawaii complete the overview of ²²⁷Ac near its potential sources.The average ²²⁷Ac activities of nearshore marine end-members range from 0.4 dpm m^− 3 at the Gulf of Mexico to 3.0 dpm m^− 3 in the coastal waters of the Korean Strait. In analogy to ²²⁸Ra, we find the extension of adjacent shelf regions to play a substantial role for ²²⁷Ac activities, although less pronounced than for radium, due to its weaker shelf source. Based on previously published values, we calculate an open ocean ²²⁷Ac inventory of 1.35 * 10¹⁸ dpm ²²⁷Ac_ex in the ocean, which corresponds to 37 moles, or 8.4 kg. This implies a flux of 127 dpm m⁻² y^− 1 from the deep-sea floor. For the shelf regions, we obtain a global inventory of ²²⁷Ac of 4.5 * 10¹⁵ dpm, which cannot be converted directly into a flux value, as the regional loss term of ²²⁷Ac to the open ocean would have to be included.Ac has so far been considered to behave similarly to Ra in the marine environment, with the exception of a strong Ac source in the deep-sea due to ²³¹Pa_ex. Here, we present evidence of geochemical differences between Ac, which is retained in a warm vent system, and Ra, which is readily released [Moore, W.S., Ussler, W. and Paull, C.K., 2008-this issue. Short-lived radium isotopes in the Hawaiian margin: Evidence for large fluid fluxes through the Puna Ridge. Marine Chemistry]. Another potential mechanism of producing deviations in ²²⁷Ac/²²⁸Ra and daughter isotope ratios from the expected production value of lithogenic material is observed at reducing environments, where enrichment in uranium may occur. The presented data here may serve as a reference for including ²²⁷Ac in circulation models, and the overview provides values for some end-members that contribute to the global Ac distribution.     

Submarine groundwater discharge and nutrient addition to the coastal zone and coral reefs of leeward Hawai'i

Multiple tracers of groundwater input (salinity, Si, ²²³Ra, ²²⁴Ra, and ²²⁶Ra) were used together to determine the magnitude, character (meteoric versus seawater), and nutrient contribution associated with submarine groundwater discharge across the leeward shores of the Hawai'ian Islands Maui, Moloka'i, and Hawai'i. Tracer abundances were elevated in the unconfined coastal aquifer and the nearshore zone, decreasing to low levels offshore, indicative of groundwater discharge (near-fresh, brackish, or saline) at all locations. At several sites, we detected evidence of fresh and saline SGD occurring simultaneously. Conservative estimates of SGD fluxes ranged widely, from 0.02–0.65 m³ m^− 2 d^− 1at the various sites. Groundwater nutrient fluxes of 0.04–40 mmol N m^− 2 d^− 1 and 0.01–1.6 mmol P m^− 2 d^− 1 represent a major source of new nutrients to coastal ecosystems along these coasts. Nutrient additions were typically greatest at locations with a substantial meteoric component in groundwater, but the recirculation of seawater through the aquifer may provide a means of transferring terrestrially-derived nutrients to the coastal zone at several sites.     

ESTIMATION OF ERRORS IN ABSORBANCE RATIO MEASUREMENTS

Ratio measurements are commonly used to address a variety of analytical problems in environmental,forensic and pharmaceutical laboratories.In absorbance ratioing techniques,analytical chemists rely onthe spectral features of the analyte(s)of interest.The absorbances at two wavelengths are monitored andthe ratio of these two absorbances is computed.This ratio is then used to confirm the identity of theanalyte(s)of interest,the purity of a product or the overlap of chromatographic peaks.These decisionsoften have far-reaching consequences(e.g.the identification of the source,biogenic or petrogenic,ofhydrocarbons in biological tissues or water).Given the cost and the liabilities associated with suchdecisions,it is unfortunate that these ratios are seldom reported with any statistical confidence.Thepurpose of this study is to delineate the parameters that affect absorbance ratio measurements.Themodels that can be used to estimate the statistical confidence in these measurements are derived andevaluated experimentally.The results show that these models can estimate the relative standard deviationsin absorbance ratios accurately.They can also estimate the effect of signal-to-noise ratio and the choiceof wavelengths on the precision of absorbance ratios.     

韧性剪切构造成岩成矿作用及对金矿化的控制--以内蒙古武川县后石花金矿为例

本文以内蒙古中部后石花金矿为例,简述了"韧性剪切构造成岩成矿作用"的新观点.研究表明,韧性剪切成岩过程包括细粒化作用、热流体作用、酸碱交代作用;韧性剪切带这种深层次断裂构造形成过程中,其推覆演化是逐渐减压过程,降压效应和剪切带本身的膨胀渗透作用,引起了剪切带内部积累的能量梯度(压力、温度、物质),导致弥漫于大面积围岩中和下地壳的液体进入韧性剪切带中."节流阀"作用形成韧性剪切成岩成矿热液系统.韧性剪切构造对金矿的控制核心是成岩成矿为统一的热动力系统,早期以成岩为主,中晚期以蚀变和矿化为主.     

Resistivity Logs of the Chinese Continental Scientific Drilling Main Hole:Implication for the Crustal Electrical Structure of Dabie-Sulu Terrane,Central-Eastern China

To understand the electrical structure of the Sulu(苏鲁) terrane,we analyzed the resis-tivity logs of the Chinese Continental Scientific Drilling main hole(CCSD-MH) and obtained the statis-tical characteristics of the resistivity log of ultrahigh-pressure(UHP) metamorphic rocks.To check the logs' quality,we compared the resistivity log data with the core test data.The two datasets show a good coherence.On the whole,the resistivity of the UHP metamorphic rocks from the CCSD-MH is very high(mostly higher than 1...     

Photometry of four binary subdwarf B stars and the nature of their unseen companion stars

We present light curves of four binary subdwarf B stars (sdB), Ton 245, Feige 11, PG 1432+159 and PG 1017−086. We also present new spectroscopic data for PG 1017−086 from which we derive its orbital period,   P =0.073 d  , and the mass function,   f _m=0.0010±0.0002 M_⊙.  This is the shortest period for an sdB binary measured to date. The values of P and f _m for the other sdB binaries have been published elsewhere. We are able to exclude the possibility that the unseen companion stars to Ton 245, Feige 11 and PG 1432+159 are main-sequence stars or subgiant stars from the absence of a sinusoidal signal, which would be caused by the irradiation of such a companion star, i.e. they show no reflection effect. The unseen companion stars in these binaries are likely to be white dwarf stars. In contrast, the reflection effect in PG 1017−086 is clearly seen. The lack of eclipses in this binary combined with other data suggests that the companion is a low-mass M-dwarf or, perhaps, a brown dwarf.