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61.
G. Diego Gatta Nicola Rotiroti Martin Fisch Milen Kadiyski Thomas Armbruster 《Physics and Chemistry of Minerals》2008,35(9):521-533
The elastic and structural behaviour of the synthetic zeolite CsAlSi5O12 (a = 16.753(4), b = 13.797(3) and c = 5.0235(17) Å, space group Ama2, Z = 2) were investigated up to 8.5 GPa by in situ single-crystal X-ray diffraction with a diamond anvil cell under hydrostatic conditions. No phase-transition occurs within the P-range investigated. Fitting the volume data with a third-order Birch–Murnaghan equation-of-state gives: V 0 = 1,155(4) Å3, K T0 = 20(1) GPa and K′ = 6.5(7). The “axial moduli” were calculated with a third-order “linearized” BM-EoS, substituting the cube of the individual lattice parameter (a 3, b 3, c 3) for the volume. The refined axial-EoS parameters are: a 0 = 16.701(44) Å, K T0a = 14(2) GPa (βa = 0.024(3) GPa?1), K′ a = 6.2(8) for the a-axis; b 0 = 13.778(20) Å, K T0b = 21(3) GPa (βb = 0.016(2) GPa?1), K′ b = 10(2) for the b-axis; c 0 = 5.018(7) Å, K T0c = 33(3) GPa (βc = 0.010(1) GPa?1), K′ c = 3.2(8) for the c-axis (K T0a:K T0b:K T0c = 1:1.50:2.36). The HP-crystal structure evolution was studied on the basis of several structural refinements at different pressures: 0.0001 GPa (with crystal in DAC without any pressure medium), 1.58(3), 1.75(4), 1.94(6), 3.25(4), 4.69(5), 7.36(6), 8.45(5) and 0.0001 GPa (after decompression). The main deformation mechanisms at high-pressure are basically driven by tetrahedral tilting, the tetrahedra behaving as rigid-units. A change in the compressional mechanisms was observed at P ≤ 2 GPa. The P-induced structural rearrangement up to 8.5 GPa is completely reversible. The high thermo-elastic stability of CsAlSi5O12, the immobility of Cs at HT/HP-conditions, the preservation of crystallinity at least up to 8.5 GPa and 1,000°C in elastic regime and the extremely low leaching rate of Cs from CsAlSi5O12 allow to consider this open-framework silicate as functional material potentially usable for fixation and deposition of Cs radioisotopes. 相似文献
62.
In situ strength measurements on natural upper-mantle minerals 总被引:1,自引:0,他引:1
Junji Yamamoto Jun-ichi Ando Hiroyuki Kagi Toru Inoue Akihiro Yamada Daisuke Yamazaki Tetsuo Irifune 《Physics and Chemistry of Minerals》2008,35(5):249-257
Using in situ strength measurements at pressures up to 10 GPa and at room temperature, 400, 600, and 700°C, we examined rheological
properties of olivine, orthopyroxene, and chromian-spinel contained in a mantle-derived xenolith. Mineral strengths were estimated
using widths of X-ray diffraction peaks as a function of pressure, temperature, and time. Differential stresses of all minerals
increase with increasing pressure, but they decrease with increasing temperature because of elastic strain on compression
and stress relaxation during heating. During compression at room temperature, all minerals deform plastically at differential
stress of 4–6 GPa. During subsequent heating, thermally induced yielding is observed in olivine at 600°C. Neither orthopyroxene
nor spinel shows complete stress relaxation, but both retain some stress even at 700°C. The strength of the minerals decreases
in the order of chromian-spinel ≈ orthopyroxene > olivine for these conditions. This order of strength is consistent with
the residual pressure of fluid inclusions in mantle xenoliths. 相似文献
63.
Emilia Palonen 《GeoJournal》2008,73(3):219-230
As in most parts of Central and Eastern Europe, there is a tradition in Hungary of changing street names and memorials in
the wake of major political transitions. This article focuses on the change of street names and memorials, i.e. the city-text,
in Hungary’s political capital, Budapest, between 1985 and 2001. The city-text in Budapest became a locus of dispute between
different political authorities, including the nation state, the metropolitan municipality, and the district, each bearing
different political ideals during and after the fall of communism. Discursive changes in the post-communist city-text emerged
expressing specific conceptions of national sovereignty, but the direction of the changes were debated. Different levels of
administration in Budapest and Hungary had divergent visions of what the new discourse on national sovereignty should be.
The changes, therefore, did not express a simple transition to an agreed-upon post-communist value system, but were the result
of a symbolic struggle between different levels of administration over what should be commemorated in the city-text. 相似文献
64.
Lars Olov Andersson 《Physics and Chemistry of Minerals》2008,35(9):505-520
The EPR spectra of Maxixe-type beryl contain a large number of overlapping signals. The angular dependence of the 1:3:3:1
signal typical for the CH3 radical shows that this radical is located at the center of the channel cavity with its symmetry axis parallel to the crystal
c-axis and is rotating around this axis. Its EPR spectrum is axially symmetric with g
// = 2.00263, g
⊥ = 2.00249 and A// = 2.288 mT, A⊥ = 2.256 mT. These anisotropies have the opposite signs of those found for surface-adsorbed methyl radicals. Hydrogen atoms
are located at position 2a at the center of the beryl cavity and the EPR parameters of the narrow doublet signal are A
0 = 1,407 MHz and g = 2.00230. Another doublet signal, which is broader and has axial symmetry with g
// = 2.00265, g
⊥ = 2.00625 and A// = 0.895 mT, A⊥ = 0.885 mT, could come from a HCO3 radical. One narrow and easily saturated signal with g
// = 2.00227 and g
⊥ = 2.00386 is interpreted to arise from a carbon monoxide radical in the beryl channel, oriented with its axis parallel to
the crystal c-axis. Additional weak doublet lines, which have similar g values as the carbon monoxide radical, are created by nearby hydrogens. A powder spectrum with g
// = 2.0017 and g
⊥ = 2.0004 appears upon UV irradiation of the single crystal and is easily saturated. This spectrum is interpreted to arise
from a carbon dioxide radical, which rotates around its symmetry axis. 相似文献
65.
Ramesh Sivanpillai X. Ben Wu R. Srinivasan Charles T. Smith Michael G. Messina 《GeoJournal》2008,71(4):211-220
Comparing satellite data derived map products are affected by differences in data characteristics, image acquisition dates,
processing techniques, and classification schemes used for assigning pixels to a thematic class. By comparing two forest maps
generated from Landsat Enhanced Thematic Mapper Plus (ETM+) and Advanced Very High Resolution Radiometer (AVHRR) images acquired
on the same day, and processed using identical classification scheme and methods these differences were minimized. The ETM+
derived map had higher classification accuracy values and more precise area estimates than the AVHRR derived map. In the ETM+
derived map, 87 of the 599 verification data were misclassified, whereas in the AVHRR derived map, 155 of the 469 verification
data were misclassified. Detailed error analyses by land cover class revealed that a land use based definition of forest accounted
for 74% (64 out of 87) and 57% (89 out of 155) of the classification errors in ETM+ and AVHRR derived maps, respectively. 相似文献
66.
This paper explores the links between a strategic policy, urban consolidation, and house prices by examining the changes in
the mix of housing and in house price for the period 1991–2004. We contend that urban consolidation could be seen as a source
of additional supply, (which might be expected to be felt in lower prices and so contribute to a local policy objective) but
also as a stimulus to demand (by developers who could bid up the price of lots where it was understood more housing could
be built). Analyses were carried out at the metropolitan and sub-regional scales using correlation tests. The research finds
very weak statistical connections, and concludes that this policy has not been associated with price changes. 相似文献
67.
68.
Concern for natural hazard-triggered technological disasters (Natech disasters) in densely populated and industrialized areas
is growing. Residents living in urban areas subject to high natural hazard risk are often unaware of the potential for secondary
disasters such as hazardous materials releases from neighboring industrial facilities, chemical storage warehouses or other
establishments housing hazardous materials. Lessons from previous disasters, such as the Natech disaster during the Kocaeli
earthquake in Turkey in 1999 call for the need to manage low frequency/high consequence events, particularly in today’s densely
populated areas. However, there is little guidance available on how local governments and communities can assess Natech risk.
To add to the problem, local governments often do not have the human or economic resources or expertise to carry out detailed
risk assessments. In this article, we propose a methodology for preliminary assessment of Natech risk in urban areas. The
proposed methodology is intended for use by local government officials in consultation with the public. The methodology considers
possible interactions between the various systems in the urban environment: the physical infrastructure (e.g., industrial
plants, lifeline systems, critical facilities), the community (e.g., population exposed), the natural environment (e.g., delicate
ecosystems, river basins), and the risk and emergency management systems (e.g., structural and nonstructural measures). Factors
related to vulnerability and hazard are analyzed and qualitative measures are recommended. Data from hazardous materials releases
during the Kocaeli, Turkey earthquake of August 17, 1999 are used as a case study to demonstrate the applicability of the
methodology. Limitations of the proposed methodology are discussed as well as future research needs.
相似文献
Norio OkadaEmail: |
69.
The Cambrian-Vendian groundwater body plays an important role in drinking water supply of capital Tallinn and other settlements
in northern Estonia. Water quality in this deep-seated confined groundwater body is influenced by the intrusion of present-day
seawater and pumping-induced upward migration of deeper saline groundwater. The aim of this study is to evaluate the threshold
values applying the methodology worked out within the EU 6th FP project “Background criteria for the identification of groundwater
thresholds (BRIDGE)” and to compare the results with the values proposed by local authorities. A database containing 250 monitoring
points was completed and used for the calculation of natural background levels (as the 90 and 97.7 percentile) in groundwater.
The calculation of threshold values is based on natural background levels and reference values. In case of Cambrian-Vendian
groundwater body the receptor is drinking water, thus limit values set by Estonian drinking water standard were used as reference
values. The threshold values proposed by local authorities are more or less the same as calculated by BRIDGE methodology.
Exceptionally different values are derived in case of chloride and ammonium. 相似文献
70.
The Samborombon Bay wetland is located on the west margin of the Rio de la Plata estuary, in the Province of Buenos Aires,
Argentina. This paper analyses the geological, geomorphologic, soil and vegetation characteristics of the southernmost sector
of this wetland and their influence on surface water and groundwater. The study area presents three hydrologic units: coastal
dunes, sand sheets and coastal plain. Coastal dunes and sand sheets are recharge zones of high permeability with well-drained,
non-saline soils, and a few surface water flows. Changes in the water table are related to rainfall. Groundwater in coastal
dunes is Ca–Mg–HCO3 to Na–HCO3, and of low salinity (590 mg/l). Groundwater in sand sheets is mainly Na–HCO3 with a salinity of about 1,020 mg/l. The coastal plain exhibits medium to low permeability sediments, with submerged saline
soils poorly drained. Groundwater is Na–Cl with a mean salinity of 16,502 mg/l. A surface hydrological network develops in
the coastal plain. Surface water levels near the shoreline are affected by tidal fluctuations; far from the shoreline water
accumulates because of poor drainage. Both sectors have Na–Cl water, but the former is more saline. Human intervention and
sea level rise may affect the wetland severely. 相似文献