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631.
Paul R. J. Saey Clemens Schlosser Pascal Achim Matthias Auer Anders Axelsson Andreas Becker Xavier Blanchard Guy Brachet Luis Cella Lars-Erik De Geer Martin B. Kalinowski Gilbert Le Petit Jenny Peterson Vladimir Popov Yury Popov Anders Ringbom Hartmut Sartorius Thomas Taffary Matthias Zähringer 《Pure and Applied Geophysics》2010,167(4-5):499-515
Activity concentration data from ambient radioxenon measurements in ground level air, which were carried out in Europe in the framework of the International Noble Gas Experiment (INGE) in support of the development and build-up of a radioxenon monitoring network for the Comprehensive Nuclear-Test-Ban Treaty verification regime are presented and discussed. Six measurement stations provided data from 5 years of measurements performed between 2003 and 2008: Longyearbyen (Spitsbergen, Norway), Stockholm (Sweden), Dubna (Russian Federation), Schauinsland Mountain (Germany), Bruyères-le-Châtel and Marseille (both France). The noble gas systems used within the INGE are designed to continuously measure low concentrations of the four radioxenon isotopes which are most relevant for detection of nuclear explosions: 131mXe, 133mXe, 133Xe and 135Xe with a time resolution less than or equal to 24 h and a minimum detectable concentration of 133Xe less than 1 mBq/m3. This European cluster of six stations is particularly interesting because it is highly influenced by a high density of nuclear power reactors and some radiopharmaceutical production facilities. The activity concentrations at the European INGE stations are studied to characterise the influence of civilian releases, to be able to distinguish them from possible nuclear explosions. It was found that the mean activity concentration of the most frequently detected isotope, 133Xe, was 5–20 mBq/m3 within Central Europe where most nuclear installations are situated (Bruyères-le-Châtel and Schauinsland), 1.4–2.4 mBq/m3 just outside that region (Stockholm, Dubna and Marseille) and 0.2 mBq/m3 in the remote polar station of Spitsbergen. No seasonal trends could be observed from the data. Two interesting events have been examined and their source regions have been identified using atmospheric backtracking methods that deploy Lagrangian particle dispersion modelling and inversion techniques. The results are consistent with known releases of a radiopharmaceutical facility. 相似文献
632.
Peter Herzsprung Martin Schultze Bertram Boehrer Anja Duffek Andrea Van der Veen Kurt Friese 《Limnologica》2010,40(2):182-190
Between 1999 and 2002, a former open-cast mine was filled with river water forming the recent Lake Goitsche. During filling initially acid water was neutralised. Phosphorus (P) imported from Mulde River was nearly completely removed from the water column by co-precipitation with iron (Fe) and aluminium (Al) and deposited in the sediment.During extremely high waters of the Mulde River in 2002, a dike breach facilitated a second high import of P into Lake Goitsche with suspended and dissolved matter. The analysis of total phosphorus (TP), however, showed that P again had been eliminated from the water body a few months after the flood event. Sediment investigations before filling with river water, during filling, and after the flood event were used to analyse the process of P immobilisation in a lake with acid mine drainage history.The ratios of Fe to soluble reactive P (SRP) of sediment pore water were up to three orders of magnitudes higher than in natural lakes and can serve as an indicator for potential internal P loading from sediments. The SRP concentrations at the oxic/anoxic boundary were near or below the limit of quantification (< 0.2 μmol/L). Fe and manganese (Mn) redox cycling were responsible for hindering P dissolution from sediment to lake water.Finally it can be stated, that the risk of eutrophication for such a lake seems to be low. 相似文献
633.
Natacha Pasche Georges Alunga Keely Mills Fabrice Muvundja David B. Ryves Michael Schurter Bernhard Wehrli Martin Schmid 《Journal of Paleolimnology》2010,44(4):931-946
This study interprets the recent history of Lake Kivu, a tropical lake in the East African Rift Valley. The current gross
sedimentation was characterized from a moored sediment trap array deployed over 2 years. The past net sedimentation was investigated
with three short cores from two different basins. Diatom assemblages from cores were interpreted as reflecting changes in
mixing depth, surface salinity and nutrient availability. The contemporary sediment trap data indicate seasonal variability,
governed by diatom blooms during the annual mixing in the dry season, similar to Lakes Malawi and Tanganyika. The ratio of
settling fluxes to net sediment accumulation rates implies mineralization rates of 80–90% at the sediment-water interface.
The sediment cores revealed an abrupt change ~40 years ago, when carbonate precipitation started. Since the 1960s, deep-water
methane concentrations, nutrient fluxes and soil mineral inputs have increased considerably and diatom assemblages have altered.
These modifications probably resulted from a combination of three factors, commonly altering lake systems: the introduction
of a non-native fish species, eutrophication, and hydrological changes inducing greater upwelling. Both the fish introduction
and increased rainfall occurred at the time when the onset of carbonate precipitation was observed, whereas catchment population
growth accompanied by intensified land use increased the flux of soil minerals already since the early twentieth century due
to more intense erosion. 相似文献
634.
On characterizing the temporal dominance patterns of model parameters and processes 总被引:1,自引:0,他引:1
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Björn Guse Matthias Pfannerstill Michael Strauch Dominik E. Reusser Stefan Lüdtke Martin Volk Hoshin Gupta Nicola Fohrer 《水文研究》2016,30(13):2255-2270
Diagnostic analyses of hydrological models intend to improve the understanding of how processes and their dynamics are represented in models. Temporal patterns of parameter dominance could be precisely characterized with a temporally resolved parameter sensitivity analysis. In this way, the discharge conditions are characterized, that lead to a parameter dominance in the model. To achieve this, the analysis of temporal dynamics in parameter sensitivity is enhanced by including additional information in a three‐tiered framework on different aggregation levels. Firstly, temporal dynamics of parameter sensitivity provide daily time series of their sensitivities to detect variations in the dominance of model parameters. Secondly, the daily sensitivities are related to the flow duration curve (FDC) to emphasize high sensitivities of model parameters in relation to specific discharge magnitudes. Thirdly, parameter sensitivities are monthly averaged separately for five segments of the FDC to detect typical patterns of parameter dominances for different discharge magnitudes. The three methodical steps are applied on two contrasting catchments (upland and lowland catchment) to demonstrate how the temporal patterns of parameter dynamics represent different hydrological regimes. The discharge dynamic in the lowland catchment is controlled by groundwater parameters for all discharge magnitudes. In contrast, different processes are relevant in the upland catchment, because the dominances of parameters from fast and slow runoff components in the upland catchment are changing over the year for the different discharge magnitudes. The joined interpretation of these three diagnostic steps provides deeper insights of how model parameters represent hydrological dynamics in models for different discharge magnitudes. Thus, this diagnostic framework leads to a better characterization of model parameters and their temporal dynamics and helps to understand the process behaviour in hydrological models. Copyright © 2015 John Wiley & Sons, Ltd. 相似文献
635.
636.
637.
Fluvial seed dispersal considers both the transport and deposition of seeds where channel geomorphic structures, hydrology and seed dispersal traits contribute to transport times and depositional locations. This study examines the influence of stream flow patterns on fluvial seed dispersal of buoyant white alder (Alnus rhombifolia) seeds by applying a one‐dimensional transport model. Conceptually, the model separates the stream into two components: (i) the main channel where the seeds are transported downstream; and (ii) the transient storage zone where seeds are temporarily detained or deposited on the river bank. Transport processes are characterized by an advection–dispersion equation which is coupled to a transient storage model using an exponential decay term. The model parameters: longitudinal dispersion (DL), exchange coefficient (α), main channel area (A) and storage zone (As) are estimated based on field experiments conducted in a confined, bedrock‐gravel bed river with pool‐riffle morphology located in coastal northern California. The riparian zone is inhabited by Alnus rhombifolia that disperse buoyant seeds in mid‐spring coinciding with the end of the wet, Mediterranean season. Artificial seeds, with similar traits of buoyancy and density to alder seeds, were used to quantify transport times and depositional locations. Preferential deposition resulted in stream reaches with larger As, high As/A ratios, and faster exchange coefficients corresponding to divergent stream flow (back‐eddies, re‐circulating flow, flow expansions) caused by geomorphic structures such as the ends of bar/riffle features and bends in the stream. The results demonstrate the importance of transient storage for seed transport and depositional processes. Morphological features that increase a channel's complexity create complex flow structures that detain seeds and provide a greater opportunity for deposition to occur. The model provides a simplification of river hydraulics to represent dispersal dynamics and lends itself to further understanding of hydrochory processes and associated population structure. Copyright © 2015 John Wiley & Sons, Ltd. 相似文献
638.
Organic carbon inputs,common ions and degassing: rethinking mixing dissolution in coastal eogenetic carbonate aquifers
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Caves deliver freshwater from coastal carbonate landscapes to estuaries but how these caves form and grow remains poorly understood. Models suggest fresh and salt water mixing drives dissolution in eogenetic limestone, but have rarely been validated through sampling of mixing waters. Here we assess controls on carbonate mineral saturation states using new and legacy geochemical data that were collected in vertical profiles through three cenotes and one borehole in the Yucatan Peninsula. Results suggest saturation states are primarily controlled by carbon fluxes rather than mixing. Undersaturation predicted by mixing models that rely on idealized end members is diminished or eliminated when end members are collected from above and below actual mixing zones. Undersaturation due to mixing is limited by CO2 degassing from fresh water in karst windows, which results in calcite supersaturation. With respect to saline groundwater, controls on capacity for mixing dissolution were more varied. Oxidation of organic carbon increased pCO2 of saline groundwater in caves (pCO2 = 10–2.06 to 10–0.96 atm) relative to matrix porosity (10–2.39 atm) and local seawater (10–3.12 atm). The impact of increased pCO2 on saturation state, however, depended on the geochemical composition of the saline water and the magnitude of organic carbon oxidation. Carbonate undersaturation due to mixing was limited where gypsum dissolution (Cenote Angelita) or sulfate reduction (Cenote Calica) increased concentrations of common ions (Ca2+ or HCO3?, respectively). Maximum undersaturation was found to occur in mixtures including saline water that had ion concentrations and ratios similar to seawater, but with moderately elevated pCO2 (Cenote Eden). Undersaturation, however, was dominated by the initial undersaturation of the saline end member, mixing was irrelevant. Our results add to a growing body of literature that suggests oxidation of organic carbon, and not mixing dissolution, is the dominant control on cave formation and enlargement in coastal eogenetic karst aquifers. Copyright © 2016 John Wiley & Sons, Ltd. 相似文献
639.
Hartmut H. Hellmer Monika Rhein Günther Heinemann Janna Abalichin Wafa Abouchami Oliver Baars Ulrich Cubasch Klaus Dethloff Lars Ebner Eberhard Fahrbach Martin Frank Gereon Gollan Richard J. Greatbatch Jens Grieger Vladimir M. Gryanik Micha Gryschka Judith Hauck Mario Hoppema Oliver Huhn Torsten Kanzow Boris P. Koch Gert König-Langlo Ulrike Langematz Gregor C. Leckebusch Christof Lüpkes Stephan Paul Annette Rinke Bjoern Rost Michiel Rutgers van der Loeff Michael Schröder Gunther Seckmeyer Torben Stichel Volker Strass Ralph Timmermann Scarlett Trimborn Uwe Ulbrich Celia Venchiarutti Ulrike Wacker Sascha Willmes Dieter Wolf-Gladrow 《Ocean Dynamics》2016,66(11):1379-1413
640.
Corey A Cohn Christopher E Pedigo Shavonne N Hylton Sanford R Simon Martin AA Schoonen 《Geochemical transactions》2009,10(1):8-9