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Direct measurements of calcite faces were performed using in situ atomic force microscopy (AFM) to reveal the dissolution processes as a function of solution saturation state and temperature. Time-sequential AFM images demonstrated that step velocities at constant temperature increased with increasing undersaturation. The anisotropy of obtuse and acute step velocities appeared to become more significant as solutions approached equilibrium and temperature increased. At saturation state Ω > 0.02, a curvilinear boundary was formed at the intersection of two acute steps and the initially rhombohedral etch pit exhibited a nearly triangular shape. This suggests that the and steps may not belong to the calcite-aqueous solution equilibrium system. Further increase in the saturation state (Ω ? 0.3) led to a lack of etch pit formation and dissolution primarily occurred at existing steps, in accordance with Teng (2004). Analysis of step kinetics at different temperatures yielded activation energies of 25 ± 6 kJ/mol and 14 ± 13 kJ/mol for obtuse and acute steps, respectively. The inconsistencies in etch pit morphology, step anisotropy, and step activation energies from the present study with those of studies far-from-equilibrium can be explained by increased influence of the backward reaction, or growth, near-equilibrium. We propose that the backward reaction occurs preferentially at the acute-acute kink sites. The kinetics and effective activation energies of near-equilibrium calcite dissolution presented in this work provide accurate experimental data under likely CO2 sequestration conditions, and thus are crucial to the development of robust geochemical models that predict the long-term performance of mineral-trapped CO2. 相似文献
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通过对近期黄河下游山东河段来水来沙特点的分析,指出了自1986~1996年以来的枯水少沙系列,使下游河道的水沙条件发生了根本变化,年水量大幅度减少,年径流量减少了一半,水量年内分配发生变化,河道淤积持续发展,对下游的防洪保安构成了新的威胁。 相似文献
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Riparian plants can adapt their water uptake strategies based on climatic and hydrological conditions within a river basin. The response of cold-alpine riparian trees to changes in water availability is poorly understood. The Lhasa River is a representative cold-alpine river in South Tibet and an under-studied environment. Therefore, a 96 km section of the lower Lhasa River was selected for a study on the water-use patterns of riparian plants. Plant water, soil water, groundwater and river water were measured at three sites for δ18O and δ2H values during the warm-wet and cold-dry periods in 2018. Soil profiles differed in isotope values between seasons and with the distance along the river. During the cold-dry period, the upper parts of the soil profiles were significantly affected by evaporation. During the warm-wet period, the soil profile was influenced by precipitation infiltration in the upper reaches of the study area and by various water sources in the lower reaches. Calculations using the IsoSource model indicated that the mature salix and birch trees (Salix cheilophila Schneid. and Betula platyphylla Suk.) accessed water from multiple sources during the cold-dry period, whereas they sourced more than 70% of their requirement from the upper 60–80 cm of the soil profile during the warm-wet period. The model indicated that the immature rose willow tree (Tamarix ramosissima Ledeb) accessed 66% of its water from the surface soil during the cold-dry period, but used the deeper layers during the warm-wet period. The plant type was not the dominant factor driving water uptake patterns in mature plants. Our findings can contribute to strategies for the sustainable development of cold-alpine riparian ecosystems. It is recommended that reducing plantation density and collocating plants with different rooting depths would be conducive to optimal plant growth in this environment. 相似文献
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Marine waters from six sites around Hong Kong with varying levels of sewage pollution were examined for noroviruses (NoVs) by PCR cloning and sequencing of a highly-variable N-terminal region of the VP1 capsid gene, at the ORF1-ORF2 junction of NoV. Phylogenetic analysis of genogroups GI- and GII-specific PCR clones obtained from different marine sites indicated that human NoV GI.1 and GII.4 strains are the most prevalent genotypes circulating in Hong Kong waters. GI- and GII-specific TaqMan-based real-time PCR assays targeting the ORF1-ORF2 junction of NoVs were used to quantify NoV particles in marine water samples in parallel with total Escherichia coli counts which were enumerated on TBX medium. No correlation of any significance between NoV and E. coli counts was observed which highlighted the inadequacy in using E. coli as a fecal indicator to predict the level of NoVs in marine waters to protect public health. 相似文献
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Green and Vernon (1974) have experimentally determined a divariant field of cordierite-orthoamphibole-kyanite-quartz with a slope of 12±4 bars per °C occurring between 8.0 and 10.4 kbar at 750° C and between 9.5 and 11.3 kbar at 850° C. However, the writers' thermodynamic calculation of the divariant band indicates a more limited range of 0.65 and 0.7 kbar at 750° C and 850° C respectively, with an estimated error of ±0.2 kbar. 相似文献
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野外实践教学在地学人才培养中具有重要作用,稳定的实习基地是开展实践教学的前提和基础。克拉玛依所处的准噶尔盆地西北缘地区位于哈萨克斯坦、塔里木与西伯利亚三大板块的交汇处,自晚古生代以来经历了多期次、多阶段长期而复杂的地质演化,褶皱构造、大型纵向走滑断裂构造发育,广泛发育晚古生代花岗岩侵入体和蛇绿混杂岩带,沉积地层连续、完整,沉积构造典型、特征显著,古生物化石丰富,白杨河深切峡谷、河流阶地地貌以及乌尔禾魔鬼城雅丹风蚀地貌各具特色,西北缘油砂矿、紫砂矿、金丝玉等矿藏储量丰富。区域内的地层、古生物、构造、地貌、矿产资源等为克拉玛依工程教育基地各院校的地学类相关专业的野外实践教学提供了丰富的教学资源,是一个理想的野外地质实习基地。 相似文献
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