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1.
S. Oreshin L. Vinnik L. Makeyeva G. Kosarev R. Kind F. Wentzel 《Geophysical Journal International》2002,151(2):393-402
2.
The rate of the reversible homogeneous disproportionation of polysulfides was studied by following the optical absorbance of polysulfide solutions in a continuous plug flow reactor equipped with an on-line photometric detector. In order to avoid heterogeneous slow reactions involving sulfur colloids or precipitate, the reaction was initiated by an abrupt pH change from an undersaturated solution containing predominantly tetrasulfide species to a pH where pentasulfide is the dominant species. The disproportionation was found to follow first order reversible reaction dynamics. At environmentally relevant conditions the characteristic time of the disproportionation reaction is of the order of 10 s. This characteristic time implies that necessary conditions for speciation of the different polysulfide species by chromatography or another separation and subsequent quantification scheme should be of the order of 1 s. 相似文献
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4.
Bo Barker Jørgensen Michael E. Böttcher Lev N. Neretin 《Geochimica et cosmochimica acta》2004,68(9):2095-2118
The main terminal processes of organic matter mineralization in anoxic Black Sea sediments underlying the sulfidic water column are sulfate reduction in the upper 2-4 m and methanogenesis below the sulfate zone. The modern marine deposits comprise a ca. 1-m-deep layer of coccolith ooze and underlying sapropel, below which sea water ions penetrate deep down into the limnic Pleistocene deposits from >9000 years BP. Sulfate reduction rates have a subsurface maximum at the SO42−-CH4 transition where H2S reaches maximum concentration. Because of an excess of reactive iron in the deep limnic deposits, most of the methane-derived H2S is drawn downward to a sulfidization front where it reacts with Fe(III) and with Fe2+ diffusing up from below. The H2S-Fe2+ transition is marked by a black band of amorphous iron sulfide above which distinct horizons of greigite and pyrite formation occur. The pore water gradients respond dynamically to environmental changes in the Black Sea with relatively short time constants of ca. 500 yr for SO42− and 10 yr for H2S, whereas the FeS in the black band has taken ca. 3000 yr to accumulate. The dual diffusion interfaces of SO42−-CH4 and H2S-Fe2+ cause the trapping of isotopically heavy iron sulfide with δ34S = +15 to +33‰ at the sulfidization front. A diffusion model for sulfur isotopes shows that the SO42− diffusing downward into the SO42−-CH4 transition has an isotopic composition of +19‰, close to the +23‰ of H2S diffusing upward. These isotopic compositions are, however, very different from the porewater SO42− (+43‰) and H2S (−15‰) at the same depth. The model explains how methane-driven sulfate reduction combined with a deep H2S sink leads to isotopically heavy pyrite in a sediment open to diffusion. These results have general implications for the marine sulfur cycle and for the interpretation of sulfur isotopic data in modern sediments and in sedimentary rocks throughout earth’s history. 相似文献
5.
The paper describes a stationary model of the boundary layer of a large-scale vortex. The model takes into account two types of nonlinearities: (1) advection of the momentum and centrifugal accelerations, that is related to large values of the Rossby number; (2) a nonlinear turbulent friction on the lower boundary (generally speaking, not only quadratic, but also more complicated). Nevertheless, the model may be studied analytically. This approach allows discovery and analysis of several universal regularities, which are not revealed by numerical modeling. The model provides the actual values for the speed of the surface wind and the angle of cross-isobar surface flow in the tropical cyclones. 相似文献
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In a recent paper, Gurrola, Minster & Owens (1994; hereafter referred to as GMO) introduced a technique for the analysis of seismic data and applied it to the records of station OBN in Russia. GMO claimed that this was a new technique in earthquake seismology, and that their results for OBN provided a new insight into the deep structure of the Russian platform. We have some comments on their techniques and results. 相似文献
8.
The Earth's crust faults and lineaments group in clusters with predominant N-S and E-W (System I) and NW-SE and NE-SW (System II) directions. The earthquake epicenters of the Benioff seismofocal zones follow the same regularities. In other words, seismofocal zones (epicenters of earthquakes) constitute a part of the regular network of the Earth's crust and lithosphere faults and lineaments. Mathematical modeling of stress distribution in the lithosphere due to a change of the Earth's ellipsoid compression showed that the principal stresses σ1 and σ2 are oriented in N-S and E-W directions, while corresponding shear stresses τ are oriented in NE-SW and NW-SE directions. It is shown that the secular deceleration of the Earth's rotation can be a reasonable mechanism for the change of Earth's ellipsoid compression and, consequently, for the origin of the regular system of faults and lineaments described above. 相似文献
9.
Pascal Chardonnet Valery Chechetkin Lev Titarchuk 《Astrophysics and Space Science》2010,325(2):153-161
We present a model of a gamma-ray burst (GRB) related to “very massive” stars. In the framework of our model, the GRB phenomenon
is a result of helium burning in degenerate conditions in a massive star (≳130 M
⊙), in which the thermal nuclear burning occurs in the deflagration regime and has a pulsating temporal pattern. The shock
runs away from the burning (reaction) zone, which leads to the development of a coronal outflow (jet-like) structure. In our
scenario the GRB observable prompt fast rise and decay part can be a result of photon propagation through the hot corona (Comptonization
photosphere) of the star. On the other hand, the GRB afterglow is a cooling phase of the expanding and outflowing envelope.
Presumably, the X-ray part of the GRB emergent spectrum is formed due to upscattering of soft photons of outer layers of the
star off hot coronal electrons, and thus it should have a specific shape of the Comptonization spectrum. 相似文献
10.