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171.
K. Mannschreck K. Bächmann K. H. Becker Th. Heil R. Kurtenbach M. Memmesheimer V. Mohnen A. Obermeier D. Poppe R. Steinbrecher Th. Schmitz A. Volz-Thomas F. Zabel 《Journal of Atmospheric Chemistry》2002,42(1):281-286
The database for volatile organic compounds (VOC data base) was created with the aim of providing an overview of tropospheric hydrocarbon measurements. The data base contains 202 substances, for which atmospheric and useful kinetic data such as rate coefficients, photolysis frequencies, mixing ratios, emission data and ozone formation potentials are compiled from available literature. The database file can be downloaded without charge from http://www.physchem.uni-wuppertal.de/voc-database. Registered users will be informed about the appearance of updates. 相似文献
172.
R. Kurtenbach R. Ackermann K. H. Becker A. Geyer J. A. G. Gomes J. C. Lörzer U. Platt P. Wiesen 《Journal of Atmospheric Chemistry》2002,42(1):395-411
In 1997 and 1998 several field campaigns for monitoring non-methane volatile organic compounds (NMVOCs) and nitrogen oxides (NOx) were carried out in a road traffic tunnel and in the city center of Wuppertal, Germany. C2–C10 aliphatic and aromatic hydrocarbons were monitored using a compact GC instrument. DOAS White and long path systems were used to measure aromatic hydrocarbons and oxygenated aromatic compounds. A formaldehyde monitor was used to measure formaldehyde. Chemiluminescence NO analysers with NO2 converter were used for measuring NO and NO2. The high mixing ratios of the NMVOCs observed in the road traffic tunnel, especially 2.9 ppbv phenol, 1.5ppbv para-cresol and 4.4 ppbv benzaldehyde, in comparison with themeasured background concentration clearly indicate that these compounds were directly emitted from road traffic. Para-Cresol was for the first timeselectively detected as primary pollutant from traffic. From the measured data a NMVOC profile of the tunnel air and the city air, normalised to benzene (ppbC/ppbC), was derived. For most compounds the observed city air NMVOC profile is almost identical with that obtained in the traffic tunnel. Since benzene originates mainly from road traffic emission, the comparison of the normalised emission ratios indicate that the road traffic emissions in Wuppertal have still the largest impact on the city air composition, which is in contrast to the German emission inventory. In both NMVOC profiles, aromatic compounds have remarkably large contributions of more than 40 ppbC%. In addtion, total NMVOC/NOx ratios from 0.6 up to 3.0ppbC/ppb in the traffic tunnel air and 3.4± 0.5 in the city air of Wuppertal were obtained. From the observed para-cresol/toluene and ortho-cresol/toluene ratios in the city air, evidence was found thatalso during daytime NO3 radical reactions play an important role in urban air. 相似文献
173.
Andrew Swales R. Bruce Williamson Laurence F. Van Dam Morag J. Stroud Matt S. McGlone 《Estuaries and Coasts》2002,25(1):43-56
Cores were collected from the length of Pakuranga estuary, a small urban estuary in Auckland, New Zealand, to determine sedimentation
and contaminant history, and in particular the impact of urbanization. Catchment sediment loads for the most recent history
(1953–1995), including urbanization since 1960, were reconstructed using the landcover history and soil erosion modeling.
Pollen and14C dating and pre-urban landcover history were used to reconstruct early estuary sedimentation (i.e., post-3000 yr BP to 1960).
Heavy metal concentrations, particle size,137Cs, pollen, and catchment sediment loads were all needed to disentangle the complex estuarine response to urbanization.137Cs profiles did not reflect the historical fallout pattern, but deposition of137Cs-labelled eroded catchment soil, coinciding with peaks in urban construction. Temporal variations in stormwater137Cs concentrations are likely due to varying contributions from137Cs-rich topsoil and137Cs-poor subsoils. A similar pattern was observed in heavy-metal concentrations and attributed to street runoff rather than
topsoil being diluted by metal-poor subsoils. Dating of the sediment profiles showed that during urbanization sedimentation
rates in the tidal creek and estuary were higher than sedimentation rates associated with past agricultural landuse and the
original forest landcover. Urbanization has brought about substantial environmental changes in the upper estuary through continued
infilling of shallow, intertidal areas, contamination by heavy metals to levels of ecological concern, sediment textural changes,
and rapid mangrove colonization of formerly bare intertidal sediments. 相似文献
174.
175.
Ejecta at North Ray crater (Apollo 16) sampled a unique section of the lunar highlands not accessible at most other landing sites and provide important constraints on the composition of late accreted materials. New data on multiple aliquots of four fragmental matrix breccias and a fragment‐laden melt breccia from this site display a variety of highly siderophile element patterns which may represent the signatures of volatile element‐depleted carbonaceous chondrite‐like material, primitive achondrite, differentiated metal, and an impactor component that cannot be related to known meteoritic material. The latter component is prevalent in these rocks besides characterized by depletions in Re and Os compared to Ir, Ru and Pt, chondritic Re/Os, and a gradual depletion of Pd and Au. The observed characteristics are more consistent with fractionations by nebular processes, like incomplete condensation or evaporation, than with lunar crustal processes, like partial melting or volatilization. The impactor signature preserved in these breccias may stem from primitive meteorites with a refractory element composition moderately different from known chondrites. The presence of distinct impactor components within the North Ray crater breccias together with observed correlations of characteristic element ratios (e.g., Re/Os, Ru/Pt, Pd/Ir) in different impact lithologies of four Apollo landing sites constrains physical mixing processes ranging from the scale of gram‐sized samples to the area covered by the Apollo missions. 相似文献
176.
Application of geochemical and stable isotopic tracers to investigate groundwater salinity in the Ochi-Narkwa Basin,Ghana 总被引:1,自引:1,他引:0
Samuel Y. Ganyaglo Shiloh Osae Tetteh Akiti Thomas Armah Laurence Gourcy Tomas Vitvar 《水文科学杂志》2017,62(8):1301-1316
Rainwater, groundwater and soil-water samples were analysed to assess groundwater geochemistry and the origin of salinity in the Ochi-Narkwa basin of the Central Region of Ghana. The samples were measured for major ions and stable isotopes (δ18O, δ2H and δ13C). The Cl? content in rainwater decreased with distance from the coast. The major hydrochemical facies were Na-Cl for the shallow groundwaters and Ca-Mg-HCO3, Na-Cl and Ca-Mg-Cl-SO4 for the deep groundwaters. Groundwater salinization is caused largely by halite dissolution and to a minor extent by silicate weathering and seawater intrusion. Stable isotope composition of the groundwaters followed a slope of 3.44, suggesting a mixing line. Chloride profiles in the soil zone revealed the existence of salt crusts, which support halite dissolution in the study area. A conceptual flow model developed to explain the mechanism of salinization showed principal groundwater flow in the NW–SE direction.
EDITOR D. KoutsoyiannisASSOCIATE EDITOR K. Heal 相似文献
177.
The importance of characterizing the ecohydrological interactions in natural, damaged/drained, and restored bogs is underscored by the importance of peatlands to global climate change and the growing need for peatland restoration. An understudied aspect of peatland ecohydrology is how shallow lateral flow impacts local hydrological conditions and water balance, which are critical for peatland restoration success. A novel method is presented using microcosms installed in the field to understand the dynamics of shallow lateral flow. Analysis of the difference in water table fluctuation inside and outside the microcosm experimental areas allowed the water balance to be constrained and the calculation of lateral flow and evapotranspiration. As an initial demonstration of this method, a series of four microcosm experiments were set up in locations with differing ecological quality and land management histories, on a raised bog complex in the midlands of Ireland. The timing and magnitude of the lateral flow differed considerably between locations with differing ecological conditions, indicating that shallow lateral flow is an important determining factor in the ecohydrological trajectory of a recovering bog system. For locations where Sphagnum spp. moss layer was present, a slow continuous net lateral input of water from the upstream catchment area supported the water table during drought periods, which was not observed in locations lacking Sphagnum. Consistent with other studies, evapotranspiration was greater in locations with a Spaghnum moss layer than in locations with a surface of peat soil. 相似文献
178.
Abigail McQuatters-Gollop Alison J. Gilbert Laurence D. Mee Jan E. Vermaat Yuri Artioli Christoph Humborg Fred Wulff 《Estuarine, Coastal and Shelf Science》2009,82(4):583-596
Anthropogenic eutrophication affects the Mediterranean, Black, North and Baltic Seas to various extents. Responses to nutrient loading and methods of monitoring relevant indicators vary regionally, hindering interpretation of ecosystem state changes and preventing a straightforward pan-European assessment of eutrophication symptoms. Here we summarize responses to nutrient enrichment in Europe's seas, comparing existing time-series of selected pelagic (phytoplankton biomass and community composition, turbidity, N:P ratio) and benthic (macro flora and faunal communities, bottom oxygen condition) indicators based on their effectiveness in assessing eutrophication effects. Our results suggest that the Black Sea and Northern Adriatic appear to be recovering from eutrophication due to economic reorganization in the Black Sea catchment and nutrient abatement measures in the case of the Northern Adriatic. The Baltic is most strongly impacted by eutrophication due to its limited exchange and the prevalence of nutrient recycling. Eutrophication in the North Sea is primarily a coastal problem, but may be exacerbated by climatic changes. Indicator interpretation is strongly dependent on sea-specific knowledge of ecosystem characteristics, and no single indicator can be employed to adequately compare eutrophication state between European seas. Communicating eutrophication-related information to policy-makers could be facilitated through the use of consistent indicator selection and monitoring methodologies across European seas. This work is discussed in the context of the European Commission's recently published Marine Strategy Directive. 相似文献
179.
180.
Two-dimensional continuous wavelet transform of simulated spatial images of waves on a slowly varying topography 总被引:1,自引:0,他引:1
Laurence Zsu-Hsin Chuang Li-Chung Wu Dong-Jiing Doong Chia Chuen Kao 《Ocean Engineering》2008,35(10):1039-1051
The wavelet transform (WT) is now recognized as a useful, flexible, and efficient technique to analyze intermittent, non-stationary and inhomogeneous signals as well as images which are obtained from experimental or in situ measurements. In this study, the two-dimensional continuous wavelet transform (2-D CWT) was introduced to analyze the spatial image of waves. The numerical algorithm of 2-D CWT was developed and testified in simulated wave field of regular and random waves. Some more simulated wave fields of various wave conditions and sea bed slopes were then assumed to verify the analytical accuracy of this new technique. The comparisons of estimations to theoretical values for several wave parameters show that the 2-D CWT is capable of identifying the directional spectra and wave properties in shallow water. 相似文献