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31.
Background
Induced precipitation of phosphate minerals to scavenge trace elements from groundwater is a potential remediation approach for contaminated aquifers. The success of engineered precipitation schemes depends on the particular phases generated, their rates of formation, and their long term stability. The purpose of this study was to examine the precipitation of calcium phosphate minerals under conditions representative of a natural groundwater. Because microorganisms are present in groundwater, and because some proposed schemes for phosphate mineral precipitation rely on stimulation of native microbial populations, we also tested the effect of bacterial cells (initial densities of 105 and 107 mL-1) added to the precipitation medium. In addition, we tested the effect of a trace mixture of propionic, isovaleric, formic and butyric acids (total concentration 0.035 mM).Results
The general progression of mineral precipitation was similar under all of the study conditions, with initial formation of amorphous calcium phosphate, and transformation to poorly crystalline hydroxylapatite (HAP) within one week. The presence of the bacterial cells appeared to delay precipitation, although by the end of the experiments the overall extent of precipitation was similar for all treatments. The stoichiometry of the final precipitates as well as Rietveld structure refinement using x-ray diffraction data indicated that the presence of organic acids and bacterial cells resulted in an increasing a and decreasing c lattice parameter, with the higher concentration of cells resulting in the greatest distortion. Uptake of Sr into the solids was decreased in the treatments with cells and organic acids, compared to the control.Conclusions
Our results suggest that the minerals formed initially during an engineered precipitation application for trace element sequestration may not be the ones that control long-term immobilization of the contaminants. In addition, the presence of bacterial cells appears to be associated with delayed HAP precipitation, changes in the lattice parameters, and reduced incorporation of trace elements as compared to cell-free systems. Schemes to remediate groundwater contaminated with trace metals that are based on enhanced phosphate mineral precipitation may need to account for these phenomena, particularly if the remediation approach relies on enhancement of in situ microbial populations. 相似文献32.
Koji Sugie Kenshi Kuma Satoshi Fujita Satomi Ushizaka Koji Suzuki Tsutomu Ikeda 《Journal of Oceanography》2011,67(2):183-196
We report on the ability for luxury Fe uptake and the potential for growth utilizing intracellular Fe pools for 4 coastal
centric diatom isolates and in situ phytoplankton assemblages, mainly composed of diatoms. Iron uptake of the diatom isolates
and natural phytoplankton assemblages in the Oyashio region during spring blooms were prevented by adding hydroxamate siderophore
desferrioxamine B (DFB). After the addition of DFB, intracellular Fe in the diatom isolates supported 2.4–4.2 cell divisions
with 1.2–2.6 Chl a doublings. The intracellular Fe was primarily used for cell generation rather than Chl a production, leading to a reduction in the Chl a cell quota in the Fe-starved cells with time. The metabolic properties of the Fe-starved cells with their cell morphologies
were different among species or genera. An on-deck incubation experiment also exhibited 1.9 cell divisions and 0.81 Chl a doublings of phytoplankton after the addition of DFB, also indicating the preference of cell generation over Chl a production. A decrease in the level of cellular Chl a, a main light-harvesting pigment in Fe-starved diatoms, may become a superior survival strategy to protect the cells from
high irradiance that can cause photo-oxidative damages through photosynthesis. Such relatively low-Fe with high-light conditions
could often occur in surface waters of the Oyashio region from spring to summer. 相似文献
33.
Tetsuichi Fujiki Kazuhiko Matsumoto Shuichi Watanabe Takuji Hosaka Toshiro Saino 《Journal of Oceanography》2011,67(3):295-303
We deployed a profiling buoy system incorporating a fast repetition rate fluorometer in the western subarctic Pacific and
carried out time-series observations of phytoplankton productivity from 9 June to 15 July 2006. The chlorophyll a (Chl a) biomass integrated over the euphotic layer was as high as 45–50 mg Chl a m−2 in the middle of June and remained in the 30–40 mg Chl a m−2 range during the rest of observation period; day-to-day variation in Chl a biomass was relatively small. The daily net primary productivity integrated over the euphotic layer ranged from 144 to 919 mg C m−2 day−1 and varied greatly, depending more on insolation rather than Chl a biomass. In addition, we found that part of primary production was exported to a 150-m depth within 2 days, indicating that
the variations in primary productivity quickly influenced the organic carbon flux from the upper ocean. Our results suggest
that the short-term variability in primary productivity is one of the key factors controlling the carbon cycle in the surface
ocean in the western subarctic Pacific. 相似文献
34.
Transport of oceanic nitrate from the continental shelf to the coastal basin in relation to the path of the Kuroshio 总被引:1,自引:0,他引:1
Ryo Sugimoto Akihide Kasai Toshihiro Miyajima Kouichi Fujita 《Continental Shelf Research》2009,29(14):1678-1688
Hydrographic and biogeochemical observations were conducted along the longitudinal section from Ise Bay to the continental margin (southern coast of Japan) to investigate changes according to the Kuroshio path variations during the summer. The strength of the uplift of the cold deep water was influenced by the surface intrusion of the Kuroshio water to the shelf region. When the intrusion of the Kuroshio surface water to the shelf region was weak in 2006, the cold and NO3−-rich shelf water intruded into the bottom layer in the bay from the shelf. This bottom intrusion was intensified by the large river discharge. The nitrogen isotope ratio (δ15N) of NO3− (4–5‰) in the bottom bay water was same as that in the deeper NO3− over the shelf, indicating the supply of new nitrogen to the bay. The warm and NO3−-poor shelf water intruded into the middle layer via the mixing region at the bay mouth when the Kuroshio water distributed in the coastal areas off Ise Bay in 2005. The regenerated NO3− with isotopically light nitrogen (δ15N=−1‰) was supplied from the shelf to the bay. This NO3− is regenerated by the nitrification in the upper layer over the shelf. The contribution rate of regenerated NO3− over the shelf to the total NO3− in the subsurface chlorophyll maximum layer in the bay was estimated at 56% by a two-source mixing model coupled with the Rayleigh equation. 相似文献
35.
The general-relativistic equations of hydrodynamics for a nonideal fluid are derived in the modified Lagrangian form. Together with the zeroth and first moment equations of radiative transfer derived by Morita and Kaneko (1986), the equations provide a complete set of the modified Lagrangian equations of radiation hydrodynamics. The equations of hydrodynamics are specialized for a thermally conducting, Newtonian viscous fluid in the modified Lagrangian form, which are the generalization of the specialrelativistic equations of hydrodynamics derived by Greenberg (1975). 相似文献
36.
In low-lying areas of urban and suburban regions in Asia, the use of landfill has allowed urban land use to encroach onto watery landforms, such as back marshes, which were formerly used as rice fields. To improve understanding of the associations between land-use patterns and landfill development, we carried out a case study in the urban fringe of Metro Manila in the Philippines. We examined landfill volume derived from land-use change using GIS, and field surveyed qualitative aspects of the landfill used. We calculated the rate of application of landfill in low-lying housing development areas to be 5.0 × 103 m3 km?2 year?1, most of which consisted of offsite disposal of construction waste or crushed rock produced by urban development and renewal on the adjoining uplands. The flow of fill material from offsite sources to onsite landfill development areas was on the basis of individual agreements between suppliers and developers. 相似文献
37.
38.
Minoru Kitamura Toru Kobari Makio C. Honda Kazuhiko Matsumoto Kosei Sasaoka Rie Nakamura Kazuyuki Tanabe 《Journal of Oceanography》2016,72(3):387-402
Seasonal changes in mesozooplankton biomass and their community structures were observed at time-series stations K2 (subarctic) and S1 (subtropical) in the western North Pacific Ocean. At K2, the maximum biomass was observed during the spring when primary productivity was still low. The annual mean biomasses in the euphotic and 200- to 1000-m layers were 1.39 (day) and 2.49 (night) g C m?2 and 4.00 (day) and 3.63 (night) g C m?2, respectively. Mesozooplankton vertical distribution was bimodal and mesopelagic peak was observed in a 200- to 300-m layer; it mainly comprised dormant copepods. Copepods predominated in most sampling layers, but euphausiids were dominant at the surface during the night. At S1, the maximum biomass was observed during the spring and the peak timing of biomass followed those of chlorophyll a and primary productivity. The annual mean biomasses in the euphotic and 200- to 1000-m layers were 0.10 (day) and 0.21 (night) g C m?2 and 0.47 (day) and 0.26 (night) g C m?2, respectively. Copepods were dominant in most sampling layers, but their mean proportion was lower than that in K2. Mesozooplankton community characteristics at both sites were compared with those at other time-series stations in the North Pacific and with each other. The annual mean primary productivities and sinking POC fluxes were equivalent at both sites; however, mesozooplankton biomasses were higher at K2 than at S1. The difference of biomasses was probably caused by differences of individual carbon losses, population turnover rates, and trophic structures of communities between the two sites. 相似文献
39.
40.