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71.
Norbert Hertkorn Ronald Benner Philippe Schmitt-Kopplin Karl Kaiser John I. Hedges 《Geochimica et cosmochimica acta》2006,70(12):2990-3010
Refractory carboxyl-rich alicyclic molecules (CRAM) are characterized in marine dissolved organic matter (DOM) using nuclear magnetic resonance spectroscopy and ultrahigh resolution mass spectrometry. CRAM are distributed throughout the water column and are the most abundant components of deep ocean DOM ever characterized. CRAM are comprised of a complex mixture of carboxylated and fused alicyclic structures with a carboxyl-C:aliphatic-C ratio of 1:2 to 1:7. CRAM are expected to constitute a strong ligand for metal binding, and multiple coordination across cations could promote aggregation and marine gel formation thereby affecting CRAM reactivity and the bioavailability of nutrients and trace metals. It appears CRAM are ultimately derived from biomolecules with structural similarities to sterols and hopanoids. The occurrence of CRAM in freshwater and terrestrial environments seems likely, considering the global distribution of biomolecules and the similarities of biogeochemical processes among environments. 相似文献
72.
73.
Robert M. Moore Stephen Punshon Claire Mahaffey David Karl 《Deep Sea Research Part I: Oceanographic Research Papers》2009,56(9):1449-1458
Fixed nitrogen is a key nutrient involved in regulating global marine productivity and hence the global oceanic carbon cycle. Oceanic nitrogen (N2) fixation is estimated to supply 8×1012 moles N y?1 to the ocean, approximately equal to current riverine and the atmospheric inputs of fixed N, and between 50 and 100% of current estimates of oceanic denitrification. However, the spatial and temporal variability of N2 fixation remains uncertain, mostly because of the normal low resolution sampling for diazotroph distribution and fixation rates. It is well established that N2 fixation, mediated by the enzyme nitrogenase, is a source of hydrogen (H2), but the extent to which it leads to supersaturation of H2 in oceanic waters is unresolved. Here, we present simultaneous measurements of upper ocean dissolved H2 concentration (nmol L?1), and rates of N2 fixation (μmol N m?3 d?1), determined using 15N2 tracer techniques (at 7 or 15 m), on a transect from Fiji to Hawaii. We find a significant correlation (r=0.98) between dissolved H2 and rates of N2 fixation, with the greatest supersaturation of H2 and highest rates of N2 fixation being observed in the subtropical gyres at the southern (~18°S) and northern (18°N) reaches of the transect. The lowest H2 saturation and N2 fixation were observed in the equatorial region between 8°S and 14°N. We propose that an empirical relationship between H2 supersaturations and N2 fixation measurements could be used to guide sampling for 15N fixation measurements or to aid the spatial interpolation of such measurements. 相似文献
74.
Based on GIS and statistical methods, with the help of searching historical literatures and calculating the landscape indices, the land use changes of Qian'an County in both spatial and temporal aspects from 1945 to 1996 has been analyzed in this paper. And the driving forces of land use changes and their ecological effects are discussed too. The main findings of this study are as follows: (1) Land use changed greatly in Qian'an during 1945-1996, characterized by a decrease in grassland, wetland and water bodies, and an increase in cultivated land, saline-alkali land, and the land for housing and other construction purposes. Grassland decreased by 175,828.66 ha, and cultivated land increased by 102,137.23 ha over the half century. Accordingly, the main landscape type changed from a steppe landscape to a managed agricultural ecosystem. (2) Results of correlation analysis show that the land use change in the study area was mainly driven by the socioeconomic factors. (3) The ecological effects of land use change in the area are characterized by serious salinization, degression of soil fertility and the weakening of landscape suitability. 相似文献
75.
Hubert Engelbrecht Karl B. Föllmi Ursula Baumer Johann Koller 《Swiss Journal of Geoscience》2010,103(1):3-13
A resin nodule was found in glauconite-rich detrital sediments of the Cretaceous Garschella Formation (Aptian to Albian) outcropping at Langer Köchel (Bavaria, S Germany). Gas chromatographic and mass spectrometric analyses of the fossil resin revealed dealkylation and the total defunctionalisation of its polycyclic constituents. Besides many unspecific components a specific one, agathalene, has survived. Agathalene also presents a strongly degraded product, but may have been derived from its natural precursor agathic acid, which is a very specific constituent (biomarker) of recent and fossil kauri resin. Although agathalene is a far less specific secondary biomarker, it indicates the botanic origin of the fossil resin nodule. Besides other potential producers of agathic acid, precursors of the present-day conifer species Agathis dammara and A. australis were distributed in a wider palaeophytogeographic range than today and might have been the botanical source of kauri resin. In view of the east–west directed Early Cretaceous surface current system of the Tethys ocean, the palaeogeographic provenance of the Werdenfels resin nodule probably was a mainland positioned further to the east or southeast of the Helvetic shelf, to where it was transported probably by driftwood of the resin-producing Agathis sp. 相似文献
76.
Over the last years, geospatial web platforms, social media, and volunteered geographic information (VGI) have opened a window of opportunity for traditional Public Participatory GIS (PPGIS) to usher in a new era. Taking advantage of these technological achievements, this paper presents a new approach for a citizen-orientated framework of spatial planning that aims at integrating participatory community work into existing decision-making structures. One major cornerstone of the presented approach is the application of a social geoweb platform (the GeoCitizen platform) that combines geo-web technologies and social media in one single tool allowing citizens to collaboratively report observations, discuss ideas, solve, and monitor problems in their living environment at a local level. This paper gives an account of an ongoing participatory land-zoning process in the Capital District of Quito, Ecuador, where the GeoCitizen platform is applied in a long-term study. 相似文献
77.
Abstract In this study, the development of a moderate coastal storm with intense precipitation that occurred during 12–14 February 1993 is examined using a high‐resolution version of the Canadian Regional Finite‐element (RFE) model with more realistic physical representations. It is shown that the improved RFE model predicts well the coastal cyclogenesis events and also the distribution and intensity of heavy mixed precipitation (rain and snow) associated with the storm. It is found that the cyclogenesis takes place in response to the low‐level inshore advection of high‐θe air from the maritime boundary layer, and the approach of a mid‐level shortwave trough with a warm pool above that is previously associated with a decaying cyclone upstream. More rapid deepening of the cyclone ensues as intense precipitation falls along the warm and cold fronts near the cyclone centre. Diagnosis of the control and sensitivity simulations reveals that the low‐level inshore warm advection and the propagation of the stratospheric warm pool contribute more significantly to the surface pressure falls during the incipient stage, whereas the mid‐level shortwave trough plays an important role in the cyclogenesis at later stages. Overall, latent heat release accounts for about 50% of the cyclone's total deepening, in agreement with the presence of a moderate baroclinic environment and the generation of intense precipitation. The diabatic and kinematic structures near the rain‐snow boundary are examined to gain insight into the influence of melting snow on the cyclogenesis. It is shown that the improved RFE model reproduces well the rain‐snow boundary structures as previously observed. Moreover, a thermally indirect circulation (perturbation) can be seen in the vicinity of the rain‐snow boundary. It is found, however, that melting of snow tends to produce a weak negative or negligible impact on the cyclogenesis, as opposed to previous hypotheses. 相似文献
78.
79.
The 2dF Galaxy Redshift Survey: the bJ -band galaxy luminosity function and survey selection function
Peder Norberg Shaun Cole Carlton M. Baugh Carlos S. Frenk Ivan Baldry Joss Bland-Hawthorn Terry Bridges Russell Cannon Matthew Colless Chris Collins Warrick Couch Nicholas J. G. Cross Gavin Dalton Roberto De Propris Simon P. Driver George Efstathiou Richard S. Ellis Karl Glazebrook Carole Jackson Ofer Lahav Ian Lewis Stuart Lumsden Steve Maddox Darren Madgwick John A. Peacock Bruce A. Peterson Will Sutherland Keith Taylor 《Monthly notices of the Royal Astronomical Society》2002,336(3):907-931
80.
Peder Norberg Carlton M. Baugh Ed Hawkins Steve Maddox John A. Peacock Shaun Cole Carlos S. Frenk Joss Bland-Hawthorn Terry Bridges Russell Cannon Matthew Colless Chris Collins Warrick Couch Gavin Dalton Roberto De Propris Simon P. Driver George Efstathiou Richard S. Ellis Karl Glazebrook Carole Jackson Ofer Lahav Ian Lewis Stuart Lumsden Darren Madgwick Bruce A. Peterson Will Sutherland Keith Taylor 《Monthly notices of the Royal Astronomical Society》2001,328(1):64-70
We investigate the dependence of the strength of galaxy clustering on intrinsic luminosity using the Anglo-Australian two degree field galaxy redshift survey (2dFGRS). The 2dFGRS is over an order of magnitude larger than previous redshift surveys used to address this issue. We measure the projected two-point correlation function of galaxies in a series of volume-limited samples. The projected correlation function is free from any distortion of the clustering pattern induced by peculiar motions and is well described by a power law in pair separation over the range . The clustering of galaxies in real space is well-fitted by a correlation length and power-law slope . The clustering amplitude increases slowly with absolute magnitude for galaxies fainter than M *, but rises more strongly at higher luminosities. At low luminosities, our results agree with measurements from the Southern Sky Redshift Survey 2 by Benoist et al. However, we find a weaker dependence of clustering strength on luminosity at the highest luminosities. The correlation function amplitude increases by a factor of 4.0 between and −22.5, and the most luminous galaxies are 3.0 times more strongly clustered than L * galaxies. The power-law slope of the correlation function shows remarkably little variation for samples spanning a factor of 20 in luminosity. Our measurements are in very good agreement with the predictions of the hierarchical galaxy formation models of Benson et al. 相似文献