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41.
The current study focuses on understanding key factors controlling geochemical export in eight diverse coastal watersheds at seasonal and annual time scales. Geochemical, atmospheric and hydrologic data across a range of hydro‐climatic regimes and varying land uses were investigated and relationships analysed. A hyperbolic dilution model was fitted for each watershed system to evaluate discharge–concentration relationships. Nitrate concentration effects were observed in watersheds exposed to high atmospheric deposition rates as well as agricultural watersheds, whereas urban watersheds showed nitrate dilution effects. Dilution patterns were observed for calcium, magnesium and sulfate for almost all watersheds. Seasonal loads for almost all constituents were noted to be mainly driven by hydrologic seasonality, but are also dependent on inputs (atmospheric deposition and land use sources). Understanding the primary controls on hydro‐chemical interactions is critical for developing and refining predictive water quality models, especially in coastal watersheds where sensitive downstream ecosystems act as receiving waters for upstream pollutant loads. Copyright © 2012 John Wiley & Sons, Ltd. 相似文献
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Thomas H. BURBINE Timothy J. McCOY Larry R. NITTLER Gretchen K. BENEDIX Edward A. CLOUTIS Tamara L. Dickinson 《Meteoritics & planetary science》2002,37(9):1233-1244
Abstract— We investigate the possibility that Mercury's crust is very reduced with FeO concentrations of less than ?0.1 wt%. We believe that such a surface could have a composition of enstatite, plagioclase, diopside, and sulfide, similar to the mineral assemblages found in aubritic meteorites. To test this hypothesis, we investigated the spectra of aubrites and their constituent minerals as analogs for the surface of Mercury. We found that some sulfides have distinctive absorption features in their spectra shortwards of ?0.6 μm that may be apparent in the spectrum of such an object. Determination of the surface composition of Mercury using orbital x‐ray spectroscopy should easily distinguish between a lunar highlands and enstatite basalt composition since these materials have significant differences in concentrations of Al, Mg, S, and Fe. The strongest argument against Mercury having an enstatite basalt composition is its extreme spectral redness. Significant reddening of the surface of an object (such as Mercury) is believed to require reduction of FeO to nanophase iron, thus requiring a few percent FeO in the material prior to alteration. 相似文献
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Ricardo Génova-Santos José Alberto Rubiño-Martín Rafael Rebolo † Kieran Cleary ‡ Rod D. Davies Richard J. Davis Clive Dickinson § Nelson Falcón ‡‡ Keith Grainge Carlos M. Gutiérrez Michael P. Hobson Michael E. Jones ¶ Rüdiger Kneissl Katy Lancaster Carmen P. Padilla-Torres Richard D. E. Saunders Paul F. Scott Angela C. Taylor ¶ Robert A. Watson †† 《Monthly notices of the Royal Astronomical Society》2005,363(1):79-92
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Robert A. Watson Pedro Carreira Kieran Cleary Rod D. Davies Richard J. Davis Clive Dickinson Keith Grainge † Carlos M. Gutiérrez Michael P. Hobson Michael E. Jones Rüdiger Kneissl Anthony Lasenby Klaus Maisinger Guy G. Pooley Rafael Rebolo José Alberto Rubiño-Martin ‡ Ben Rusholme § Richard D. E. Saunders Richard Savage Paul F. Scott Ane Slosar Pedro J. Sosa Molina Angela C. Taylor David Titterington Elizabeth Waldram Althea Wilkinson 《Monthly notices of the Royal Astronomical Society》2003,341(4):1057-1065
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Paul Duuring Stephen M. Rowins Bradley S. M. McKinley Jenni M. Dickinson Larry J. Diakow Young-Seog Kim Robert A. Creaser 《Mineralium Deposita》2009,44(4):463-496
The Toodoggone district comprises Upper Triassic to Lower Jurassic Hazelton Group Toodoggone Formation volcanic and sedimentary
rocks, which unconformably overlie submarine island-arc volcanic and sedimentary rocks of the Lower Permian Asitka Group and
Middle Triassic Takla Group, some of which are intruded by Upper Triassic to Lower Jurassic plutons and dikes of the Black
Lake suite. Although plutonism occurred episodically from ca. 218 to 191 Ma, the largest porphyry Cu–Au ± Mo systems formed
from ca. 202 to 197 Ma, with minor mineralization occurring from ca. 197 to 194 Ma. Porphyry-style mineralization is hosted
by small-volume (<1 km3), single-phase, porphyritic igneous stocks or dikes that have high-K calc-alkaline compositions and are comparable with volcanic-arc
granites. The Fin porphyry Cu–Au–Mo deposit is anomalous in that it is 16 m.y. older than any other porphyry Cu–Au ± Mo occurrence
in the district and has lower REEs. All porphyry systems are spatially restricted to exposed Asitka and Takla Group basement
rocks, and rarely, the lowest member of the Hazelton Group (i.e., the ca. 201 Ma Duncan Member). The basement rocks to intrusions
are best exposed in the southern half of the district, where high rates of erosion and uplift have resulted in their preferential
exposure. In contrast, low- and high-sulfidation epithermal systems are more numerous in the northern half of the district,
where the overlying Hazelton Group rocks dominate exposures. Cogenetic porphyry systems might also exist in the northern areas;
however, if they are present, they are likely to be buried deeply beneath Hazelton Group rocks. High-sulfidation epithermal
systems formed at ca. 201 to 182 Ma, whereas low-sulfidation systems were active at ca. 192 to 162 Ma. Amongst the studied
epithermal systems, the Baker low-sulfidation epithermal deposit displays the strongest demonstrable genetic link with magmatic
fluids; fluid inclusion studies demonstrate that its ore fluids were hot (>468°C), saline, and deposited metals at deep crustal
depths (>2 km). Sulfur, C, O, and Pb isotope data confirm the involvement of a magmatic fluid, but also suggest that the ore
fluid interacted with Asitka and Takla Group country rocks prior to metal deposition. In contrast, in the Shasta, Lawyers,
and Griz-Sickle low-sulfidation epithermal systems, there is no clear association with magmatic fluids. Instead, their fluid
inclusion data indicate the involvement of low-temperature (175 to 335°C), low-salinity (1 to 11 equiv. wt.% NaCl) fluids
that deposited metals at shallow depths (<850 m). Their isotope (i.e., O, H, Pb) data suggest interaction between meteoric
and/or metamorphic ore fluids with basement country rocks. 相似文献
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