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191.
Daniel D. Riemer Eric C. Apel John J. Orlando Geoffrey S. Tyndall William H. Brune Eric J. Williams William A. Lonneman James D. Neece 《Journal of Atmospheric Chemistry》2008,61(3):227-242
As part of the 2000 Texas Air Quality Study (TexAQS), we studied the isoprene oxidation process under ambient conditions to
discern the presence of chlorine atom (Cl) chemistry in the Houston, Texas urban area. By measuring chloromethylbutenone (CMBO)
and an isomer of chloromethylbutenal (CMBA), we clearly observed sixteen episodes of active Cl chemistry during the 24-day
experiment. Estimated median Cl concentration during each of these episodes was between the detection limit of ~102 atoms cm−3 and 50 - 30 + 70 ×104 50_{ - 30}^{ + 70} \times {10^4} atoms cm−3. Cl concentration during all the episodes averaged 7.6 - 2.0 + 4.7 ×104 7.6_{ - 2.0}^{ + 4.7} \times {10^4} atoms cm−3 and thus amounted to less than 3% of the OH concentration during the same periods. During the episodes, the fraction of oxidation
chemistry initiated by Cl ranged from 3–43% and was strongly dependent on the quantity and type of hydrocarbons present in
the atmosphere. Because of its intermittent presence and low concentration, Cl is not a broadly influential oxidant in the
Houston, Texas urban area. 相似文献
192.
193.
V. Belokurov N. W. Evans P. C. Hewett A. Moiseev R. G. McMahon S. F. Sanchez L. J. King 《Monthly notices of the Royal Astronomical Society》2009,392(1):104-112
We present discovery images, together with follow-up imaging and spectroscopy, of two large-separation gravitational lenses found by our survey for wide arcs [the CAmbridge Sloan Survey Of Wide ARcs in the skY (CASSOWARY)]. The survey exploits the multicolour photometry of the Sloan Digital Sky Survey to find multiple blue components around red galaxies. CASSOWARY 2 (or 'the Cheshire Cat') is composed of two massive early-type galaxies at z = 0.426 and 0.432, respectively, lensing two background sources, the first a star-forming galaxy at z = 0.97 and the second a high -redshift galaxy ( z > 1.4) . There are at least three images of the former source and probably four or more of the latter, arranged in two giant arcs. The mass enclosed within the larger arc of radius ∼11 arcsec is ∼33 × 1012 M⊙ . CASSOWARY 3 comprises an arc of three bright images of a z = 0.725 source, lensed by a foreground elliptical at z = 0.274 . The radius of the arc is ∼4 arcsec and the enclosed mass is ∼2.5 × 1012 M⊙ . Together with earlier discoveries like the Cosmic Horseshoe and the 8 o'clock Arc, these new systems, with separations intermediate between the arcsecond-separation lenses of typical strong galaxy lensing and arcminute-separation cluster lenses, probe the very high end of the galaxy mass function. 相似文献
194.
195.
G. Lodato S. Nayakshin A. R. King J. E. Pringle 《Monthly notices of the Royal Astronomical Society》2009,398(3):1392-1402
We compute the effect of an orbiting gas disc in promoting the coalescence of a central supermassive black hole binary. Unlike earlier studies, we consider a finite mass of gas with explicit time dependence: we do not assume that the gas necessarily adopts a steady state or a spatially constant accretion rate, i.e. that the merging black hole was somehow inserted into a pre-existing accretion disc. We consider the tidal torque of the binary on the disc, and the binary's gravitational radiation. We study the effects of star formation in the gas disc in a simple energy feedback framework.
The disc spectrum differs in detail from that found before. In particular, tidal torques from the secondary black hole heat the edges of the gap, creating bright rims around the secondary. These rims do not in practice have uniform brightness either in azimuth or time, but can on average account for as much as 50 per cent of the integrated light from the disc. This may lead to detectable high-photon-energy variability on the relatively long orbital time-scale of the secondary black hole, and thus offer a prospective signature of a coalescing black hole binary.
We also find that the disc can drive the binary to merger on a reasonable time-scale only if its mass is at least comparable with that of the secondary black hole, and if the initial binary separation is relatively small, i.e. a0 ≲ 0.05 pc. Star formation complicates the merger further by removing mass from the disc. In the feedback model we consider, this sets an effective limit to the disc mass. As a result, binary merging is unlikely unless the black hole mass ratio is ≲0.001. Gas discs thus appear not to be an effective solution to the 'last parsec' problem for a significant class of mergers. 相似文献
The disc spectrum differs in detail from that found before. In particular, tidal torques from the secondary black hole heat the edges of the gap, creating bright rims around the secondary. These rims do not in practice have uniform brightness either in azimuth or time, but can on average account for as much as 50 per cent of the integrated light from the disc. This may lead to detectable high-photon-energy variability on the relatively long orbital time-scale of the secondary black hole, and thus offer a prospective signature of a coalescing black hole binary.
We also find that the disc can drive the binary to merger on a reasonable time-scale only if its mass is at least comparable with that of the secondary black hole, and if the initial binary separation is relatively small, i.e. a
196.
Osvaldo M. Rabbia Laura B. Hernández David H. French Robert W. King John C. Ayers 《Mineralium Deposita》2009,44(8):849-866
Mineralogical, textural, and chemical analyses (EPMA and PIXE) of hydrothermal rutile in the El Teniente porphyry Cu–Mo deposit
help to better constrain ore formation processes. Rutile formed from igneous Ti-rich phases (sphene, biotite, Ti-magnetite,
and ilmenite) by re-equilibration and/or breakdown under hydrothermal conditions at temperatures ranging between 400°C and
700°C. Most rutile nucleate and grow at the original textural position of its Ti-rich igneous parent mineral phase. The distribution
of Mo content in rutile indicates that low-temperature (∼400–550°C), Mo-poor rutile (5.4 ± 1.1 ppm) is dominantly in the Mo-rich
mafic wallrocks (high-grade ore), while high-temperature (∼550-700°C), Mo-rich rutile (186 ± 20 ppm) is found in the Mo-poor
felsic porphyries (low-grade ore). Rutile from late dacite ring dikes is a notable exception to this distribution pattern.
The Sb content in rutile from the high-temperature potassic core of the deposit to its low-temperature propylitic fringe remains
relatively constant (35 ± 3 ppm). Temperature and Mo content of the hydrothermal fluids in addition to Mo/Ti ratio, modal
abundance and stability of Ti-rich parental phases are key factors constraining Mo content and provenance in high-temperature
(≥550°C) rutile. The initial Mo content of parent mineral phases is controlled by melt composition and oxygen fugacity as
well as timing and efficiency of fluid–melt separation. Enhanced reduction of SO2-rich fluids and sulfide deposition in the Fe-rich mafic wallrocks influences the low-temperature (≤550°C) rutile chemistry.
The data are consistent with a model of fluid circulation of hot (>550°C), oxidized (ƒO2 ≥ NNO + 1.3), SO2-rich and Mo-bearing fluids, likely exsolved from deeper crystallizing parts of the porphyry system and fluxed through the
upper dacite porphyries and related structures, with metal deposition dominantly in the Fe-rich mafic wallrocks. 相似文献
197.
Maarten Wynants Aloyce Patrick Linus Munishi Kelvin Mtei Samuel Bodé Alex Taylor Geoffrey Millward Neil Roberts David Gilvear Patrick Ndakidemi Pascal Boeckx William H. Blake 《地球表面变化过程与地形》2021,46(15):3112-3126
Soil resources in parts of Tanzania are rapidly being depleted by increased rates of soil erosion and downstream sediment transport, threatening ecosystem health, water and livelihood security in the region. However, incomplete understanding to what effect the dynamics of soil erosion and sediment transport are responding to land-use changes and climatic variability are hindering the actions needed to future-proof Tanzanian land-use practices. Complementary environmental diagnostic tools were applied to reconstruct the rates and sources of sedimentation over time in three Tanzanian river systems that have experienced changing land use and climatic conditions. Detailed historical analysis of sediment deposits revealed drastic changes in sediment yield and source contributions. Quantitative sedimentation reconstruction using radionuclide dating showed a 20-fold increase in sediment yield over the past 120 years. The observed dramatic increase in sediment yield is most likely driven by increasing land-use pressures. Deforestation, cropland expansion and increasing grazing pressures resulted into accelerating rates of sheet erosion. A regime shift after years of progressive soil degradation and convergence of surface flows resulted into a highly incised landscape, where high amounts of eroded soil from throughout the catchment are rapidly transported downstream by strongly connected ephemeral drainage networks. By integrating complementary spatial and temporal evidence bases, this study demonstrated links between land-use change, increased soil erosion and downstream sedimentation. Such evidence can guide stakeholders and policy makers in the design of targeted management interventions to safeguard future soil health and water quality. 相似文献
198.
Kenneth D. Adams Ted Goebel Kelly Graf Geoffrey M. Smith Anna J. Camp Richard W. Briggs David Rhode 《Geoarchaeology》2008,23(5):608-643
The Great Basin of the western U.S. contains a rich record of Late Pleistocene and Holocene lake‐level fluctuations as well as an extensive record of human occupation during the same time frame. We compare spatial‐temporal relationships between these records in the Lahontan basin to consider whether lake‐level fluctuations across the Pleistocene‐Holocene transition controlled distribution of archaeological sites. We use the reasonably well‐dated archaeological record from caves and rockshelters as well as results from new pedestrian surveys to investigate this problem. Although lake levels probably reached maximum elevations of about 1230–1235 m in the different subbasins of Lahontan during the Younger Dryas (YD) period, the duration that the lakes occupied the highest levels was brief. Paleoindian and Early Archaic archaeological sites are concentrated on somewhat lower and slightly younger shorelines (_1220–1225 m) that also date from the Younger Dryas period. This study suggests that Paleoindians often concentrated their activities adjacent to large lakes and wetland resources soon after they first entered the Great Basin. © 2008 Wiley Periodicals, Inc. 相似文献
199.
Systematic variations in atmospheric heat exchange, surface residence time, and groundwater influx across montane stream networks commonly produce an increasing stream temperature trend with decreasing elevation. However, complex stream temperature profiles that differ from this common longitudinal trend also exist, suggesting that stream temperatures may be influenced by complex interactions among hydrologic and atmospheric processes. Lakes within stream networks form one potential source of temperature profile complexity due to the spatially variable contribution of lake-sourced water to stream flow. We investigated temperature profile complexity in a multi-season stream temperature dataset collected across a montane stream network containing many alpine lakes. This investigation was performed by making comparisons between multiple statistical models that used different combinations of stream and lake characteristics to represent specific hypotheses for the controls on stream temperature. The compared models included a set of models which used a topographically derived estimate of the hydrologic influence of lakes to separate and quantify the effects of stream elevation and lake source-water contributions to longitudinal stream temperature patterns. This source-water mixing model provided a parsimonious explanation for complex stream-network temperature patterns in the summer and autumn, and this approach may be further applicable to other systems where stream temperatures are influenced by multiple water sources. Simpler models that discounted lake effects were more optimal during the winter and spring, suggesting that complex patterns in stream temperature profiles may emerge and subside temporally, across seasons, in response to diversity of water temperatures from different sources. 相似文献
200.