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151.
152.
Sources and distribution of terrigenous organic matter delivered by the Atchafalaya River to sediments in the northern Gulf of Mexico 总被引:6,自引:0,他引:6
Elizabeth S. Gordon 《Geochimica et cosmochimica acta》2003,67(13):2359-2375
Suspended sediments (SS) from the Atchafalaya River (AR) and the Mississippi River and surficial sediment samples from seven shallow cross-shelf transects west of the AR in the northern Gulf of Mexico were examined using elemental (%OC, C/N), isotopic (δ13C, Δ14C), and terrigenous biomarker analyses. The organic matter (OM) delivered by the AR is isotopically enriched (∼−24.5‰) and relatively degraded, suggesting that soil-derived OM with a C4 signature is the predominant OM source for these SS. The shelf sediments display OC values that generally decrease seaward within each transect and westward, parallel to the coastline. A strong terrigenous C/N (29) signal is observed in sediments deposited close to the mouth of the river, but values along the remainder of the shelf fall within a narrow range (8-13), with no apparent offshore trends. Depleted stable carbon isotope (δ13C) values typical of C3 plant debris (−27‰) are found near the river mouth and become more enriched (−22 to −21‰) offshore. The spatial distribution of lignin in shelf sediments mirrors that of OC, with high lignin yields found inshore relative to that found offshore (water depth > 10 m).The isotopic and biomarker data indicate that at least two types of terrigenous OM are deposited within the study area. Relatively undegraded, C3 plant debris is deposited close to the mouth of the AR, whereas more degraded, isotopically enriched, soil-derived OM appears to be deposited along the remainder of the shelf. An important input from marine carbon is found at the stations offshore from the 10-m isobath. Quantification of the terrigenous component of sedimentary OM is complicated by the heterogeneous composition of the terrigenous end-member. A three-end-member mixing model is therefore required to more accurately evaluate the sources of OM deposited in the study area. The results of the mixing calculation indicate that terrigenous OM (soil-derived OM and vascular plant debris) accounts for ∼79% of the OM deposited as inshore sediments and 66% of OM deposited as offshore sediments. Importantly, the abundance of terrigenous OM is 40% higher in inshore sediments and nearly 85% higher in offshore sediments than indicated by a two-end-member mixing model. Such a result highlights the need to reevaluate the inputs and cycling of soil-derived OM in the coastal ocean. 相似文献
153.
Tim?M.?O’BrienEmail author Elizabeth?L.?Miller 《Contributions to Mineralogy and Petrology》2014,168(4):1071
Microtextural, U–Pb, trace element and Lu–Hf analyses of zircons from gneisses dredged from the Chukchi Borderland indicate a long-lived, Cambrian–Ordovician, granulite facies metamorphism. These results reveal a complete prograde, peak and cooling history of zircon growth during anatexis. Early increasing temperatures caused modification and Pb-loss of Precambrian zircons by recrystallization and dissolution/re-precipitation of existing grains. Small variations in initial 176Hf/177Hf results (0.282325–0.282042) and flat HREE patterns of these zircons indicate that they grew by dissolution/re-precipitation in the presence of garnet. Zircons subsequently crystallized from a partial melt during peak to post-peak metamorphism from 530 to 485 Ma. A broad range of initial 176Hf/177Hf ratios (0.282693–0.282050) and mineral inclusions within zircons suggest that this phase of growth incorporated Zr and Hf obtained from the breakdown of Zr-enriched phases. Microtextural evidence along with trace element and isotopic data suggests that final growth of metamorphic rims on zircon occurred during slow cooling and crystallization of residual partial melts during the early Ordovician (485–470 Ma). Younger, late Ordovician–Silurian (420–450 Ma) euhedral, oscillatory-zoned, trace element-enriched zircons crystallized within leucocratic veins that intrude the gneisses. Their age corresponds to granitoids dated from this same dredge. The intrusives and veins provide evidence that the Chukchi Borderland rifted from a position near Pearya and northwest Svalbard, which represent the northern continuation of the Caledonian orogen. Evidence for earlier Cambrian metamorphism has not been reported from this region. The age of granulite facies metamorphism reported here represents the earliest phase of deformation in the Arctic Caledonides. 相似文献
154.
María Teresa Rodríguez-Salazar Ofelia Morton-Bermea Elizabeth Hernández-Álvarez Rufino Lozano Victor Tapia-Cruz 《Environmental Earth Sciences》2011,62(5):899-905
This research presents and discusses information concerning the spatial distribution of heavy metals (Pb, Cu, Zn, Ba, Co,
Cr, Ni and V) in the urban environments of Mexico City using geographical information system and statistical analysis. Superficial
soil samples (n = 146) were analyzed. The highest contamination indices were found in the north and center zone of the metropolitan area.
In contrast, the surrounding rural fields show a lower impact grade. The higher concentrations of Pb, Cu, Zn and Ba were observed
as being related to high vehicular traffic, nevertheless other elements such as Co, Cr, Ni and V do not show anthropogenic
influence and their content can be attributed to the parental rock. The results are compared with previous surveys carried
out in 2003 in order to evaluate temporal deposition trends. No changes were found on reported concentrations except for Cu
and Zn, whose concentration has increased in later years. The results suggest that spatial distribution analysis and results
in comparison with previous studies could be useful for the management and sustainable development of the metropolitan area
of Mexico City. 相似文献
155.
156.
The effect of El Niño Southern Oscillation cycles on the decadal scale suspended sediment behavior of a coastal dry‐summer subtropical catchment
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Andrew B. Gray Gregory B. Pasternack Elizabeth B. Watson Jonathan A. Warrick Miguel A. Goñi 《地球表面变化过程与地形》2015,40(2):272-284
Rivers display temporal dependence in suspended sediment–water discharge relationships. Although most work has focused on multi‐decadal trends, river sediment behavior often displays sub‐decadal scale fluctuations that have received little attention. The objectives of this study were to identify inter‐annual to decadal scale fluctuations in the suspended sediment–discharge relationship of a dry‐summer subtropical river, infer the mechanisms behind these fluctuations, and examine the role of El Niño Southern Oscillation climate cycles. The Salinas River (California) is a moderate sized (11 000 km2), coastal dry‐summer subtropical catchment with a mean discharge (Qmean) of 11.6 m3 s?1. This watershed is located at the northern most extent of the Pacific coastal North America region that experiences increased storm frequency during El Niño years. Event to inter‐annual scale suspended sediment behavior in this system was known to be influenced by antecedent hydrologic conditions, whereby previous hydrologic activity regulates the suspended sediment concentration–water discharge relationship. Fine and sand suspended sediment in the lower Salinas River exhibited persistent, decadal scale periods of positive and negative discharge corrected concentrations. The decadal scale variability in suspended sediment behavior was influenced by inter‐annual to decadal scale fluctuations in hydrologic characteristics, including: elapsed time since small (~0.1 × Qmean), and moderate (~10 × Qmean) threshold discharge values, the number of preceding days that low/no flow occurred, and annual water yield. El Niño climatic activity was found to have little effect on decadal‐scale fluctuations in the fine suspended sediment–discharge relationship due to low or no effect on the frequency of moderate to low discharge magnitudes, annual precipitation, and water yield. However, sand concentrations generally increased in El Niño years due to the increased frequency of moderate to high magnitude discharge events, which generally increase sand supply. Copyright © 2014 John Wiley & Sons, Ltd. 相似文献
157.
The Role of Planetary Boundary-Layer Parameterizations in the Air Quality of an Urban Area with Complex Topography 总被引:2,自引:1,他引:2
Elizabeth Bossioli Maria Tombrou Aggeliki Dandou Eleni Athanasopoulou Kostas V. Varotsos 《Boundary-Layer Meteorology》2009,131(1):53-72
The effect of different planetary boundary-layer (PBL) parameterization schemes on the spatial distribution of atmospheric
pollution over the complex topography of the greater Athens area is investigated. Four PBL schemes originally implemented
in a numerical meteorological model and a fifth one simulating the urban effect are examined. Two different atmospheric conditions
are analyzed; a typical summer and a typical winter pollution episode. The relative importance of chemical and physical processes
of the pollution predictions is discussed using process analysis. It is revealed that, for primary pollutants, a local scheme
seems more adequate to represent the maximum observed concentrations while, completely different in structure, a non-local
scheme reproduces the mean observed values in the basin. Concerning secondary pollutants, peak concentration differences,
due to the different PBL schemes, are smoothed out. Nevertheless, the PBL scheme selection shapes the horizontal and the vertical
extension of maximum values. The non-local and semi non-local schemes are superior to the others, favouring strong vertical
mixing and transport towards the surface. The stronger turbulence accommodated effectively by the semi non-local urban scheme
enhances ozone production along the sea-breeze axis and preserves the high ozone concentrations during the nighttime hours
in the urban core. 相似文献
158.
159.
Abandoned mining operations continue to severely degrade many ecosystems worldwide by releasing acidic water and/or heavy metals into surface and groundwater. Contaminant concentrations in affected streams vary with discharge in patterns that reflect both geochemical reactions and variable mixing of contaminated and non-contaminated waters. However, controls on concentration-discharge (C-Q) patterns remain unclear, particularly for constituents that experience changing solubility across redox and pH gradients. Understanding the C-Q behaviour of contaminants aids in predicting both downstream transport and effects on aquatic life under variable flow. Here, we examined the C-Q behaviours of non-reactive (Na, K, Ca, Mg, Cl−) and reactive (Fe, Mn, Al, H+, SO42−) solutes in a stream contaminated with acid mine drainage in northeastern Ohio, USA. Concentration-discharge patterns at the watershed outlet primarily reflected mixing of contaminated baseflow with intermittent inputs of high pH water draining from a passive limestone treatment system into the stream. The treatment system acted as an ephemeral tributary that mitigated contamination in the stream by diluting solutes, raising pH, and driving metal precipitation, but only when flow was present during wet seasons. Consequently, AMD-derived reactive solutes (H+, Fe, Mn, Al) decreased with increasing stream discharge while relatively conservative solutes (e.g., Ca, Mg, K, Na) decreased only slightly or were chemostatic. This study highlights both the unique C-Q patterns of reactive solutes when compared to those of non-reactive solutes and the potential for intermittent streams to control C-Q behaviour in headwater catchments. 相似文献
160.