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621.
Molecular characterization of dissolved organic matter associated with the Greenland ice sheet 总被引:1,自引:0,他引:1
Maya P. Bhatia Krista Longnecker Elizabeth B. Kujawinski 《Geochimica et cosmochimica acta》2010,74(13):3768-9950
Subsurface microbial oxidation of overridden soils and vegetation beneath glaciers and ice sheets may affect global carbon budgets on glacial-interglacial timescales. The likelihood and magnitude of this process depends on the chemical nature and reactivity of the subglacial organic carbon stores. We examined the composition of carbon pools associated with different regions of the Greenland ice sheet (subglacial, supraglacial, proglacial) in order to elucidate the type of dissolved organic matter (DOM) present in the subglacial discharge over a melt season. Electrospray ionization (ESI) Fourier transform ion cyclotron resonance (FT-ICR) mass spectrometry coupled to multivariate statistics permitted unprecedented molecular level characterization of this material and revealed that carbon pools associated with discrete glacial regions are comprised of different compound classes. Specifically, a larger proportion of protein-like compounds were observed in the supraglacial samples and in the early melt season (spring) subglacial discharge. In contrast, the late melt season (summer) subglacial discharge contained a greater fraction of lignin-like and other material presumably derived from underlying vegetation and soil. These results suggest (1) that the majority of supraglacial DOM originates from autochthonous microbial processes on the ice sheet surface, (2) that the subglacial DOM contains allochthonous carbon derived from overridden soils and vegetation as well as autochthonous carbon derived from in situ microbial metabolism, and (3) that the relative contribution of allochthonous and autochthonous material in subglacial discharge varies during the melt season. These conclusions are consistent with the hypothesis that, given sufficient time (e.g., overwinter storage), resident subglacial microbial communities may oxidize terrestrial material beneath the Greenland ice sheet. 相似文献
622.
Urban and suburban storm water runoff as a source of polycyclic aromatic hydrocarbons (PAHs) to Massachusetts estuarine and coastal environments 总被引:1,自引:0,他引:1
Charles A. Menzie Susanne S. Hoeppner Jerome J. Cura Jonathan S. Freshman Elizabeth N. LaFrey 《Estuaries and Coasts》2002,25(2):165-176
Urban and suburban storm water runoff from ten locations in eastern Massachusetts was analyzed for 39 polycyclic aromatic hydrocarbons (PAHs) compounds. Similar profiles in PAH composition were observed for groups of samples and appear to reflect land use. The largest group includes, urban storm water from areas with a mix of industrial, commercial, and residential use. Fluoranthene, phenanthrene, pyrene, chrysene, and benzo (b) fluoranthene were the predominant compounds in this group, but lighter molecular weight PAHs were also present. Sources of PAHs to storm water include a combination of petroleum and combustion. The profile of PAH compounds in local atmospheric deposition was similar to urban storm water, but differed in several of the predominant compounds. PAHs in storm water could increase the levels of these compounds in nearshore sediments and may be the most important source of high molecular weight PAHs to these environments. 相似文献
623.
An Attempt to Close the Daytime Surface Energy Balance Using Spatially-Averaged Flux Measurements 总被引:1,自引:0,他引:1
Matthias Mauder Raymond L. Desjardins Elizabeth Pattey Devon Worth 《Boundary-Layer Meteorology》2010,136(2):175-191
Single-tower eddy-covariance measurements represent the complete surface flux of a scalar only under idealized conditions.
Therefore, we often find an underestimation of energy fluxes expressed as a lack of energy balance closure at many sites.
In this study, a multi-tower approach to measure atmospheric energy fluxes based on spatial averaging is evaluated and possible
mechanisms causing a lack of energy balance closure are analysed, focussing on daytime data only. It is shown that the multi-tower
technique is also unable to measure the entire flux for our site, likely because the assumption of horizontal homogeneity
is violated. Heterogeneity-induced and buoyancy-driven quasi-stationary circulations are probably the dominant processes causing
the underestimation of energy fluxes. A dependence of the energy balance residual on stability is found, with residuals close
to zero for stable stratification, a maximum under unstable to near-neutral conditions and still relatively large residuals
for stronger instability. Assuming the processes transporting energy and CO2 are similar, the implications on long-term CO2 flux measurements are analysed. Accordingly, the resulting selective systematic error of cumulative net ecosystem exchange
estimates for agricultural regions such as ours can be of the order of more than 100%, since mainly the fluxes during periods
of net CO2 uptake are underestimated while periods of net CO2 release are much less affected by this bias. Further investigations about this issue are highly warranted. 相似文献
624.
625.
Abandoned channel fill sequences in the tidal estuary of a small mountainous,dry‐summer river
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Andrew B. Gray Gregory B. Pasternack Elizabeth B. Watson Miguel A. Goñi 《Sedimentology》2016,63(1):176-206
This study proposes a modification of the current model for abandoned channel fill stratigraphy produced in unidirectional flow river reaches to incorporate seasonal tidal deposition. Evidence supporting this concept came from a study of two consecutive channel abandonment sequences in Ropers Slough of the lower Eel River Estuary in northern California. Aerial photographs showed that Ropers Slough was abandoned around 1943, reoccupied after the 1964 flood, and abandoned again in 1974 with fill continuing to the present. Planform geomorphic characteristics derived from these images were used in conjunction with sub‐centimetre resolution stratigraphic analyses to describe depositional processes and their resultant sedimentary deposits. Both abandonment sequences recorded quasi‐annual scale fluvial/tidal deposition couplets. In both cases, tidal deposits contained very little sand, were higher in organic and inorganic carbon content than the sandier, fluvially dominated deposits, and possessed millimetre‐scale horizontal laminations. The two abandonment fills differed significantly in terms of the temporal progression of channel narrowing and fluvial sediment deposition characteristics. Aerial photographic analysis showed that the first abandonment sequence led to a more rapid narrowing of Ropers Slough and produced deposits with a positive relationship between grain size/deposit thickness and discharge. The second abandonment resulted in a much slower narrowing of Ropers Slough and generally thinner fluvial deposits with no clear relationship between grain size/deposit thickness and discharge. The δ13C values and organic nitrogen to organic carbon ratios of deposits from the first phase overlapped with Eel River suspended sediment characteristics found for low flows (one to five times mean discharge), while those of the second phase were consistent with suspended sediment from higher flows (seven to ten times mean discharge). When considered together, the results indicate that the early fill sequence recorded a reach experiencing regular fluvial deposition through flow conditions during the wet season, while the latter fill sequence records a reach more disconnected from the main stem in terms of flow and sediment. The major factor affecting the difference in sedimentation between the two fill periods appears to have been the morphology of the upstream river bend in relation to the position of the bifurcation node. During the first fill period, the upstream entrance to Ropers Slough seems to have remained open, in part due to the placement of its entrance on the outside of the mainstem river bend, and despite stronger tidal effects caused by a larger tidal prism and closer proximity to the tidal inlet. By the second fill sequence, the upstream bend morphology had altered, placing the entrance to Ropers Slough on the inner bank of the mainstem bend, which resulted in more rapid plug bar formation. The role of tidal effects in the geomorphic trajectory of the two abandonment sequences is unclear, but appears to have been less important than local bifurcation geometry. 相似文献
626.
Ocean Dynamics - This study investigates the rapid weakening of super-cyclone Amphan (2020) over the Bay of Bengal. Shortly after reaching its super-cyclone status, Amphan experienced rapid... 相似文献