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111.
Thomas E. Young Harry W. Green II Anne M. Hofmeister David Walker 《Physics and Chemistry of Minerals》1993,19(6):409-422
Wadsleyite (β-(Mg,Fe)2SiO4) is a major constituent of the Earth's transition zone and is known to accommodate OH. The portion of the transition zone between 400–550 km could be an important source or sink for hydroxyl in plumes and slabs intersecting this region. Micro-infrared spectroscopy has been carried out on the β-phase and coexisting metastable olivine synthesized in a multianvil apparatus at 14 GPa and 1550–1650 K under hydrous conditions. Single-crystal and polycrystal specimens of both phases were analyzed in the 1800–8500 cm?1 frequency region to determine the speciation, abundances, and partitioning behavior of the hydrous components in coexisting β-phase and olivine. β-phase spectra consistently show three distinct OH bands at 3329, 3580, and 3615 cm?1. OH concentrations range from 10000–65000 H/106 Si. A strong positive correlation of grain size and extent of transformation with OH concentration in the β-phase indicates that grain-growth and transformation rates are enhanced in a hydrous environment. Olivine spectra are variable, but consistently show a prominent broad-band absorbance representing molecular H2O, consistent with the infrared signature of the starting material. OH concentrations in olivine range from <300–1400 H/106 Si. The highest OH concentrations measured for olivine and the β-phase may represent solubility limits, in which case the OH solubility ratio between these two phases is approximately 1∶40. Where both phases coexist and are undersaturated with OH, the partitioning ratio of OH between them is about 1∶100. The large solubility contrast between olivine and the β-phase suggests a mechanism for hydrating the transition zone via olivine carried down in subducting slabs. Plumes impinging on an OH-rich upper transition region could cause H2 or H2O to be released upon transformation of the β-phase to olivine, resulting in initiation of secondary upwellings. If dissolution of OH weakens the β-phase, and if OH is present in the mantle, the region between 400–550 km could be a zone of low viscosity. 相似文献
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Early fill of the Western Irish Namurian Basin: a complex relationship between turbidites and deltas 总被引:1,自引:0,他引:1
The Western Irish Namurian Basin developed in Early Carboniferous times as a result of extension across the Shannon Lineament which probably coincides with the lapetus Suture. During the late Dinantian, axial areas of the NE-SW elongate trough became deep, whilst shallow-water limestones were deposited on the flanks. This bathymetry persisted into the Namurian when carbonate deposition ceased. In axial areas, a relatively thick mudstone succession spans earliest Namurian to Chokierian whilst on the northwestern marginal shelf, a thin, condensed Namurian mudstone sequence, in which pre-Chokierian sediments are apparently absent, rests unconformably on the Dinantian. From late Chokierian to early Kinderscoutian, the basin was filled by sand-dominated clastic sediments. Sand deposition began in the axial area with deposition of a thick turbidite sequence, the Ross Formation, which is largely equivalent to the condensed mudstone succession on the flanks. Turbidity currents flowed mainly axially towards the north-east and deposited a sequence lacking well-defined patterns of vertical bed-thickness change. Channels and slide sheets occur towards the top of the formation. The turbidite system seems to have lacked well-defined lobes and stable distributary channels. Overlying the Ross Formation, the Gull Island Formation shows a decreasing incidence of turbidite sandstones at the expense of increasing siltstones. This formation is characterized by major slides and slumps interbedded with undisturbed strata. In the flanking areas of the basin, the formation is thinner, has only a few turbidites in the sequence above the condensed mudstones and contains only one slide sheet. Overall the formation is interpreted as the deposit of a major prograding slope, the lower part representing a ramp upon which turbidites were deposited, the upper part a highly unstable muddy slope lacking any conspicuous feeder channels through which sand might have been transferred to deeper water. Progradation of the slope appears to have been increasingly from the northwestern flank of the trough which is similar to the direction deduced for the overlying deltaic Tullig cyclothem which completes the initial basin fill. Whilst several features of the succession can be explained by envisaging the whole sequence as the product of one linked depositional system, the shifting directions of palaeocurrents and palaeoslope raise problems. The switch from axial to lateral supply casts doubt on the strict application of Walther's Law to the total sequence and seems to demand large avulsive shifts of the delta system on the shelf area to the west. 相似文献
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This study presents the results from precipitation experiments carried out to investigate the partitioning of the alkaline earth cations Mg2+, Ca2+, Sr2+, and Ba2+ between abiogenic aragonite and seawater as a function of temperature. Experiments were carried out at 5 to 75 °C, using the protocol of Kinsman and Holland [Kinsman, D.J.J., Holland, H.D., 1969. The coprecipitation of cations with CaCO3 IV. The coprecipitation of Sr2+ with aragonite between 16 and 96 °C. Geochim. Cosmochim. Acta33, 1-17.] The concentrations of Mg Sr and Ba were determined in the fluid from each experiment by inductively coupled plasma-mass spectrometry, and in individual aragonite grains by secondary ion mass spectrometry. The experimentally produced aragonite grains are enriched in trace components (“impurities”) relative to the concentrations expected from crystal-fluid equilibrium, indicating that kinetic processes are controlling element distribution. Our data are not consistent with fractionations produced kinetically in a boundary layer adjacent to the growing crystal because Sr2+, a compatible element, is enriched rather than depleted in the aragonite. Element compatibilities, and the systematic change in partitioning with temperature, can be explained by the process of surface entrapment proposed by Watson and Liang [Watson, E.B., Liang, Y., 1995. A simple model for sector zoning in slowly grown crystals: implications for growth rate and lattice diffusion, with emphasis on accessory minerals in crustal rocks. Am. Mineral.80, 1179-1187] and Watson [Watson, E.B., 1996. Surface enrichment and trace-element uptake during crystal growth. Geochim. Cosmochim. Acta60, 5013-5020; Watson, E.B., 2004. A conceptual model for near-surface kinetic controls on the trace-element and stable isotope composition of abiogenic calcite crystals. Geochim. Cosmochim. Acta68, 1473-1488]. This process is thought to operate in regimes where the competition between crystal growth rate and diffusivity in the near-surface region limits the extent to which the solid can achieve partitioning equilibrium with the fluid. A comparison of the skeletal composition of Diploria labyrinthiformis (brain coral) collected on Bermuda with results from precipitation calculations carried out using our experimentally determined partition coefficients indicate that the fluid from which coral skeleton precipitates has a Sr/Ca ratio comparable to that of seawater, but is depleted in Mg and Ba, and that there are seasonal fluctuations in the mass fraction of aragonite precipitated from the calcifying fluid (“precipitation efficiency”). The combined effects of surface entrapment during aragonite growth and seasonal fluctuations in “precipitation efficiency” likely forms the basis for the temperature information recorded in the aragonite skeletons of Scleractinian corals. 相似文献
117.
This study undertakes a multi‐disciplinary approach (sedimentology, carbon isotopes, magnetic susceptibility and thickness distribution) to improve understanding of a major Palaeozoic carbonate platform, the Frasnian platform of Belgium. These combined techniques are used to reconstruct the platform history, which evolved in two main steps. During the first phase, the basin was strongly influenced by faulting, producing notable thickness and facies variations, with open ocean conditions, with good water circulation and no/or limited barrier reef. The second phase of platform development was less influenced by differential subsidence, as indicated by homogeneous facies distribution. However, this platform developed under restricted waters, with low circulation which is likely related to the development of a barrier reef. 相似文献
118.
The Livelihood Vulnerability Index: A pragmatic approach to assessing risks from climate variability and change—A case study in Mozambique 总被引:3,自引:0,他引:3
We developed the Livelihood Vulnerability Index (LVI) to estimate climate change vulnerability in the Mabote and Moma Districts of Mozambique. We surveyed 200 households in each district to collect data on socio-demographics, livelihoods, social networks, health, food and water security, natural disasters and climate variability. Data were aggregated using a composite index and differential vulnerabilities were compared. Results suggest that Moma may be more vulnerable in terms of water resources while Mabote may be more vulnerable in terms of socio-demographic structure. This pragmatic approach may be used to monitor vulnerability, program resources for assistance, and/or evaluate potential program/policy effectiveness in data-scarce regions by introducing scenarios into the LVI model for baseline comparison. 相似文献
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Ocean Dynamics - Coastal waters are globally challenging areas to monitor not only because of the high resolution needed to resolve the scales at stake but also because most satellites are not yet... 相似文献