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601.
602.
利用微滤和超滤技术研究了九龙江河口区表层水中铀及其同位素组成的粒级分布和地球化学行为.结果表明,溶解态(<0.4μm)中低分子量组分(<10 000 u)占主要份额,胶体态(10 000 u~0.4μm)238U所占比例不足1%,且随盐度的增加其所占份额逐渐降低.溶解态、低分子量组分和胶体态238U的比活度与盐度之间存在良好的线性正相关关系,证实它们在九龙江河口区呈现保守行为.在颗粒态(>0.4μm)中,各粒级组分238U所占份额主要受控于相应颗粒物的浓度,在盐度小于20的区域,各粒级颗粒组分238U占颗粒态的份额有如下变化次序:10~53μm>2~10μm>0.4~2μm>大于53μm,而在盐度大于30的近外海站位,该次序发生一些变化:0.4~2μm>10~53μm>2~10μm>大于53μm,最小粒级颗粒组分238U的贡献有所增加,反映了自生铀贡献的加强.九龙江河口区表层水中溶解态(包括低分子量组分和胶体态)的234U/238U)A.R.均大于1,显示出234U过剩的特征,而各粒级颗粒组分中的234U/238U)A.R.则接近于平衡值(1.0).这一现象与陆地岩石风化过程中水体对铀的淋滤释出量及234U的优先浸出有关.对232Th/238U质量比的研究显示,溶解态及其所包括的低分子量组分和胶体态的232Th/238U质量比均小于1,而颗粒态及其所包括的4个粒级组分中的232Th/238U质量比均大于1,反映了向外海输送过程中铀、钍地球化学行为的差异. 相似文献
603.
生物制氢研究进展 总被引:1,自引:0,他引:1
目前, 世界上利用的能源90%以上都是“化石能源”(如石油、煤炭和天然气等)。随着人类不断利用这些不可再生的“化石能源”, 它将会逐渐枯竭, 且其燃烧形成的产物(如CO2和SO2等)造成的严重环境污染(如温室效应和酸雨), 也有害于人类健康。因此, 人类正面临着能源紧缺和环境污染的双重压力。为满足能源需求量日益增长和环境保护的需要, 我们必须寻找环保型的可再生能源来替代“化石能源” 以满足人类对能源的需求。
在各种可再生能源中氢能将有可能替代“化石能源”,成为未来能源利用的主要形式。氢能具有许多优点:①氢能燃烧时只生成水, 不产生任何污染物, 甚至连CO2也不会产生, 实现真正的“零污染” 和“零排放”;②氢能的能量密度高, 放热高达122 kJ/g, 是焦炭放热的4.5倍, 汽油的2.68倍;③氢能可经济有效的输送和储存, 可以利用已有的天然气管道输送, 输送成本低, 甚至优于输电, 因为输送氢能不会产生如电能输送过程中所产生的能量损耗;氢能的存储也比较简便, 其中储氢合金材料就是一种非常理想的储氢方法, 该方法储氢能力强、运输方便、操作容易, 且安全可靠。在利用储氢合金进行储氢时, 还可用以进行制冷或采暖(Kulkova et al., 2006), 因为储氢材料在吸氢时放热, 在放氢时吸热。正因为氢能具有如此多的优点, 许多大的跨国公司开始对制氢技术高度关注, 如主要汽车制造商(通用、福特、戴姆勒-克莱斯勒等)对开发以氢能作为燃料的汽车投入大量的人力和物力;宝马公司从20世纪70年代就开始研制以氢能为能源的汽车, 宝马公司现在已拥有了时速达240km的氢能汽车(Munro,2003)。同时, 一些发达国家的科研院所的科学家们对氢能的制备方法、制氢机制以及提高产氢量等进行了大量的研究。 相似文献
604.
Starting from the widespread phenomena of porous bottoms in the near shore region, considering fully the diversity of bottom topography and wave number variation, and including the effect of evanescent modes, a general linear wave theory for water waves propagating over uneven porous bottoms in the near shore region is established by use of Green‘s scond identity. This theory can be reduced to a number of the most typical mild-slope equations curreutly in use and provide a reliable research basis for follow-up development of nonlinear water wave theory involving porous bottoms. 相似文献
605.
Based on Hong‘s theory, previous random models, and a generalized expression suitable for FIT calculation, the interaction between irregular waves and vertical walls is numerically simulated. The results of simulation demonstrate that the wave energy changes with the incidence angle and the distance from the wall. Particularly, the Mach effect and the combined wave spectrum characteristics are analyzed in detail, which are significant in both theory and practice. 相似文献
606.
More and more researches show that neither the critical downward acceleration nor the critical slope of water waves is a universal constant. On the contrary, they vary with particular wave conditions. This fact moders the models either for the probability of wave breaking B or for the whitecap coverage W based on these criteria difficult to apply. In this paper and the one which follows we seek to develop models for the prediction of both B and W based on the kinematical criterion. First, several joint probabihstic distribution functions (PDFs) of wave characteristics are derived, based on which the breaking properties B and W are estimated. The estimation is made on the assumption that a wave breaks ff the horizontal velocity of water particles at its crest exceeds the local wave celerity, and whitecapping occurs in regions of fluid where water particles travel faster than the waves. The consequent B and W depend on wave spectral moments of orders 0 to 4.Then the JONSWAP spectrum is used to represent the fetch-limited sea waves in deep water, so as to relate the probahility of wave breaking and the whitecap coverage with wind parameters. To this end, the time-averaging technique proposed by Glazman (1986) is applied to the estimation of the spectral moments involved, and furthermore, the theoretical models are compared with available observations collected from published literature. From the comparison, the averaging time scale is determined. The final models show that the probability of wave breaking as well as the whitecap coverage depends on the dimensionless fetch. The agreement between these models and the database is reasonable. 相似文献
607.
Analysis of Dynamic Characteristics of Submarine Free Spanning Pipelines by Complex Damping Method 总被引:2,自引:0,他引:2
Considering the effect of the internal flowing fluid and the external marine environmental condition, the differential equation for the vortex-induced vibration (V1V) of the free spanning pipeline is derived and is discretized by the Hermit interpolation function. The free vibration equation with the damping term is solved by the complex damping method for the natural frequency, and then the effect of fluid damping on the natural frequency of the free spanning pipeline is analyzed.The results show that fluid damping has a significant influence on the damped natural frequency of the free spanning pipeline in the lock-in state, while it has little influence when the pipeline is out of the lock-in state. In the meantime,the change of the free span length has the same effect on the damped natural frequency and the undamped natural frequency. 相似文献
608.
An optimization mathematical model of the pile forces for piled breasting dolphins in the open sea under various loading conditions is presented. The optimum layout with the well distributed pile forces and the least number of piles is achieved by the multiplier penalty function method. Several engineering cases have been calculated and compared with the result of the conventional design method. It is shown that the number of piles can be reduced at least by 10%—20% and the piles‘ bearing state is improved greatly. 相似文献
609.
Chunfang Cai Zengye Xie Richard H. Worden Guoyi Hu Lansheng Wang Hong He 《Marine and Petroleum Geology》2004,21(10):1265-1279
New sour pools have recently found in the Lower Triassic Feixianguan Fm carbonate reservoirs in the East Sichuan Basin in China with H2S up to 17.4% by volume. A recent blowout from a well drilled into this formation killed hundreds of people as a result of the percentage concentrations of H2S. In order to assess the origin of fatal H2S as well as the cause of petroleum alteration, H2S concentrations and the isotopes, δ34S and δ13C have been collected and measured in gas samples from reservoirs. Anhydrite, pyrite and elemental sulphur δ34S values have been measured for comparison. The high concentrations of H2S gas are found to occur at depths >3000 m (temperature now at 100 °C) in evaporated platform facies oolitic dolomite or limestone that contains anhydrite nodule occurrence within the reservoirs. Where H2S concentrations are greater than 10% its δ34S values lie between +12.0 and +13.2‰ CDT. This is within the range of anhydrite δ34S values found within the Feixianguan Fm (+11.0 to +21.7‰; average 15.5±3.5‰ CDT). Thus H2S must have been generated by thermochemical sulphate reduction (TSR) locally within the reservoirs. Burial history analysis and fluid inclusion data reveal that the temperature at which TSR occurred was greater than about 130–140 °C, suggesting that the present depth-temperature minimum is an artifact of post-TSR uplift. Both methane and ethane were actively involved in TSR since the petroleum became almost totally dry (no alkanes except methane) and methane δ13C values become significantly heavier as TSR proceeded. Methane δ13C difference thus reflects the extent of TSR. While it is tempting to use a present-day depth control (>3000 m) to predict the distribution of H2S in the Feixianguan Fm, this is an invalid approach since TSR occurred when the formation was buried some 1000–2000 m deeper than it is at present. The likelihood of differential uplift across the basin means that it is important to develop a basinal understanding of the thermal history of the Feixianguan Fm so that it is possible to determine which parts of the basin have been hotter than 130–140 °C. 相似文献
610.