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181.
Farid Juillot Delphine Jouvin Philipe Telouk Philippe Ildefonse Steve Sutton Gordon E. Brown Jr. 《Geochimica et cosmochimica acta》2011,75(9):2295-2308
Zinc isotopes have been studied along two smelter-impacted soil profiles sampled near one of the largest Pb and Zn processing plants in Europe located in northern France, about 50 km south of Lille. Mean δ66Zn values along these two soil profiles range from +0.22 ± 0.17‰ (2σ) to +0.34 ± 0.17‰ (2σ) at the lowest horizons and from +0.38 ± 0.45‰ (2σ) to +0.76 ± 0.14‰ (2σ) near the surface. The δ66Zn values in the lowest horizons of the soils are interpreted as being representative of the local geochemical background (mean value +0.31 ± 0.38‰), whereas heavier δ66Zn values near the surface of the two soils are related to anthropogenic Zn. This anthropogenic Zn occurs in the form of franklinite (ZnFe2O4)-bearing slag grains originating from processing wastes at the smelter site and exhibiting δ66Zn values of +0.81 ± 0.20‰ (2σ). The presence of franklinite is indicated by EXAFS analysis of the topsoil samples from both soil profiles as well as by micro-XANES analysis of the surface horizon of a third smelter-impacted soil from a distant site. These results indicate that naturally occurring Zn and smelter-derived Zn exhibit significantly different δ66Zn values, which suggests that zinc isotopes can be used to distinguish between geogenic and anthropogenic sources of Zn in smelter-impacted soils. In addition to a possible influence of additional past sources of light Zn (likely Zn-sulfides and Zn-sulfates directly emitted by the smelter), the light δ66Zn values in the surface horizons compared to smelter-derived slag materials are interpreted as resulting mainly from fractionation processes associated with biotic and/or abiotic pedological processes (Zn-bearing mineral precipitation, Zn complexation by organic matter, and plant uptake of Zn). This conclusion emphasizes the need for additional Zn isotopic studies before being able to use Zn isotopes to trace sources and pathways of this element in surface environments. 相似文献
182.
This study investigates the isotopic composition (C, O, S and Sr) of carbonates, sulphates and sulphide cements in the rock
matrix and fracture fillings in geological formations of the Southeast basin of France, using core samples collected during
the Deep Geology of France programme (GPF Ardèche theme). The Southeast basin belongs to the Alpine Tethyan margin. It is
one of the thickest sedimentary basins in Europe, reaching upwards of 9 km in certain locations. The main fluid transfer from
the basin is related to the large Pb–Zn Mississippi Valley-type district along the southern margin of the Massif Central block.
A synthesis of the tectonic, mineralogical and petrographic investigations on the GPF boreholes shows that a major fluid circulation
event occurred across the Alpine margin of Tethys during the Early Jurassic (Hettangian–Bathonian). It produced a general
cementation of the rock porosity through precipitation of dolomite, sulphate and barite. Fracture fillings yield isotopic
signatures distinct from the matrix cements. Matrix cements have particular characteristics, i.e. δ34S and δ13C that agree with a marine origin. The δ34S values of Permo-Carboniferous to Triassic sulphides from fracture cements are interpreted as resulting from the thermo-chemical
reduction of sulphates. Fracture sulphates in the same geological formations yield δ34S values that define a relatively homogeneous end-member, whose composition is similar to sulphates in the Largentière Pb–Zn
ore deposit. The source of S is attributed to the Permo-Carboniferous succession. The borehole fracture fillings are attributed
to a major fluid circulation stage compatible with the Early Jurassic stage identified from the geological investigation of
the boreholes. The formation of the Largentière deposit is considered as resulting from the mixing of this Early Jurassic
fluid with continental hydrothermal fluids circulating in a basement horst, along its margin with the sedimentary basin. Other
Pb–Zn deposits may also be related to fluid migration along the basement/sedimentary cover interface in the eastern and western
parts of the Massif Central. This regional fluid circulation event may represent a geodynamic marker of the Jurassic extensional
phase. 相似文献
183.
Alexandre Forest Jean-Éric Tremblay Yves Gratton Johannie Martin Jonathan Gagnon Gérald Darnis Makoto Sampei Louis Fortier Mathieu Ardyna Michel Gosselin Hiroshi Hattori Dan Nguyen Roxane Maranger Dolors Vaqué Cèlia Marrasé Carlos Pedrós-Alió Amélie Sallon Christine Michel Colleen Kellogg Jody Deming Elizabeth Shadwick Helmuth Thomas Heike Link Philippe Archambault Dieter Piepenburg 《Progress in Oceanography》2011,91(4):410-436
Major pathways of biogenic carbon (C) flow are resolved for the planktonic food web of the flaw lead polynya system of the Amundsen Gulf (southeast Beaufort Sea, Arctic Ocean) in spring-summer 2008. This period was relevant to study the effect of climate change on Arctic marine ecosystems as it was characterized by unusually low ice cover and warm sea surface temperature. Our synthesis relied on a mass balance estimate of gross primary production (GPP) of 52.5 ± 12.5 g C m−2 calculated using the drawdown of nitrate and dissolved inorganic C, and a seasonal f-ratio of 0.64. Based on chlorophyll a biomass, we estimated that GPP was dominated by phytoplankton (93.6%) over ice algae (6.4%) and by large cells (>5 μm, 67.6%) over small cells (<5 μm, 32.4%). Ancillary in situ data on bacterial production, zooplankton biomass and respiration, herbivory, bacterivory, vertical particle fluxes, pools of particulate and dissolved organic carbon (POC, DOC), net community production (NCP), as well as selected variables from the literature were used to evaluate the fate of size-fractionated GPP in the ecosystem. The structure and functioning of the planktonic food web was elucidated through inverse analysis using the mean GPP and the 95% confidence limits of every other field measurement as lower and upper constraints. The model computed a net primary production of 49.2 g C m−2, which was directly channeled toward dominant calanoid copepods (i.e. Calanus hyperboreus 20%, Calanus glacialis 10%, and Metridia longa 10%), other mesozooplankton (12%), microzooplankton (14%), detrital POC (18%), and DOC (16%). Bacteria required 29.9 g C m−2, a demand met entirely by the DOC derived from local biological activities. The ultimate C outflow comprised respiration fluxes (82% of the initial GPP), a small sedimentation (3%), and a modest residual C flow (15%) resulting from NCP, dilution and accumulation. The sinking C flux at the model limit depth (395 m) supplied 60% of the estimated benthic C demand (2.8 g C m−2), suggesting that the benthos relied partly on other C sources within the bottom boundary layer to fuel its activity. In summary, our results illustrate that the ongoing decline in Arctic sea ice promotes the growth of pelagic communities in the Amundsen Gulf, which benefited from a ∼80% increase in GPP in spring-summer 2008 when compared to 2004 – a year of average ice conditions and relatively low GPP. However, 53% of the secondary production was generated within the microbial food web, the net ecological efficiency of zooplankton populations was not particularly high (13.4%), and the quantity of biogenic C available for trophic export remained low (6.6 g C m−2). Hence it is unlikely that the increase in lower food web productivity, such as the one observed in our study, could support new harvestable fishery resources in the offshore Beaufort Sea domain. 相似文献
184.
Structural controls on the formation of BSR over a diapiric anticline from a dense MCS survey offshore southwestern Taiwan 总被引:1,自引:0,他引:1
Philippe Schnürle Char-Shine Liu Andrew T. Lin Saulwood Lin 《Marine and Petroleum Geology》2011,28(10):1932-1942
A dense seismic reflection survey with up to 250-m line-spacing has been conducted in a 15 × 15 km wide area offshore southwestern Taiwan where Bottom Simulating Reflector is highly concentrated and geochemical signals for the presence of gas hydrate are strong. A complex interplay between north–south trending thrust faults and northwest–southeast oblique ramps exists in this region, leading to the formation of 3 plunging anticlines arranged in a relay pattern. Landward in the slope basin, a north–south trending diapiric fold, accompanied by bright reflections and numerous diffractions on the seismic profiles, extends across the entire survey area. This fold is bounded to the west by a minor east-verging back-thrust and assumes a symmetric shape, except at the northern and southern edges of this area, where it actively overrides the anticlines along a west-verging thrust, forming a duplex structure. A clear BSR is observed along 67% of the acquired profiles. The BSR is almost continuous in the slope basin but poorly imaged near the crest of the anticlines. Local geothermal gradient values estimated from BSR sub-bottom depths are low along the western limb and crest of the anticlines ranging from 40 to 50 °C/km, increase toward 50–60 °C/km in the slope basin and 55–65 °C/km along the diapiric fold, and reach maximum values of 70 °C/km at the southern tip of the Good Weather Ridge. Furthermore, the local dips of BSR and sedimentary strata that crosscut the BSR at intersections of any 2 seismic profiles have been computed. The stratigraphic dips indicated a dominant east–west shortening in the study area, but strata near the crest of the plunging anticlines generally strike to southwest almost perpendicular to the direction of plate convergence. The intensity of the estimated bedding-guided fluid and gas flux into the hydrate stability zone is weaker than 2 in the slope basin and the south-central half of the diapiric fold, increases to 7 in the northern half of the diapiric fold and plunging anticlines, and reaches a maximum of 16 at the western frontal thrust system. Rapid sedimentation, active tectonics and fluid migration paths with significant dissolved gas content impact on the mechanism for BSR formation and gas hydrate accumulation. As we begin to integrate the results from these studies, we are able to outline the regional variations, and discuss the importance of structural controls in the mechanisms leading to the gas hydrate emplacements. 相似文献
185.
Philippe Favre 《Geodinamica Acta》2013,26(2):59-81
RésuménUn résumé de la cinématique du Rif externe central et occidental, de la période de rifting aux événements tectoniques récents, est proposé. L’évolution du Rif externe est abordée sur le plan quantitatif par le biais des principaux mécanismes physiques qui ont pu affecter cette partie de la marge nord-africaine durant le Jurassique, le Crétacé et le Paléocène (processus de dilatation thermique lors du rifting et de contraction thermique lors du refroidissement de la lithosphère, effondrement par flexure de la marge nord-africaine lors de la collision). Les géométries et densités obtenues sont comparées avec les données gravimétriques et de sismique réfraction.Un des aspects du modèle de Wernicke (1985), la dissymétrie du rifting de la marge africaine, semble se vérifier par l’analyse et à la modélisation de la subsidence. Mais celle-ci montre l’existence d’une fusion adiabatique tardive du manteau supérieur dont le modèle de cisaillement simple ne tient pas compte. Le soulèvement de la marge à la fin du rifting ne serait pas dû uniquement à une dilatation thermique car les données de terrain montrent des discordances angulaires importantes sur la marge africaine. Ce soulèvement est attribué localement à la poussée des rides médio-océaniques naissantes de l’Atlantique et du sillon transformant nord-africain.La modélisation de la subsidence tectonique permet d’expliquer l’absence d’intumescence sous le Rif. Elle est attribuée aux taux d’amincissement crustaux élevés durant les phases d’extension triasico-jurassiques. Cette approche quantitative confirme l’existence d’un bassin intra-continental avorté au sud-ouest et d’une marge continentale sensu stricto au nord-est. Si l’océanisation paraît plus tardive dans la partie rifaine du sillon transformant nord-africain (Callovien) que dans l’Atlantique Central (Bajocien), la subsidence post-rift ne se distingue pas de celle d’une marge passive classique. 相似文献
186.
We develop an analytical Hamiltonian formalism adapted to the study of the motion of two planets in co-orbital resonance. The Hamiltonian, averaged over one of the planetary mean longitudes, is expanded in power series of eccentricities and inclinations. The model, which is valid in the entire co-orbital region, possesses an integrable approximation modeling the planar and quasi-circular motions. First, focusing on the fixed points of this approximation, we highlight relations linking the eigenvectors of the associated linearized differential system and the existence of certain remarkable orbits like the elliptic Eulerian Lagrangian configurations, the anti-Lagrange (Giuppone et al. in MNRAS 407:390–398, 2010) orbits and some second sort orbits discovered by Poincaré. Then, the variational equation is studied in the vicinity of any quasi-circular periodic solution. The fundamental frequencies of the trajectory are deduced and possible occurrence of low order resonances are discussed. Finally, with the help of the construction of a Birkhoff normal form, we prove that the elliptic Lagrangian equilateral configurations and the anti-Lagrange orbits bifurcate from the same fixed point $L_4$ L 4 . 相似文献
187.
Delphine Bosch Janne Blichert-Toft Frédéric Moynier Bruce K. Nelson Philippe Telouk Pierre-Yves Gillot Francis Albarède 《Earth and Planetary Science Letters》2008,265(3-4):748-765
Pb, Hf, Nd and Sr isotopes of basaltic lavas from the two Réunion Island volcanoes are reported in order to examine the origin of the sources feeding these volcanoes and to detect possible changes through time. Samples, chosen to cover the whole lifetime of the two volcanoes (from 2 Ma to present), yield a chemically restricted (compared to OIB lavas) but complex distribution. Réunion plume isotopic characteristics have been defined on the basis of the composition of uncontaminated shield-building lavas from the Piton de la Fournaise volcano. The average ?Nd, ?Hf, 87Sr/86Sr and 206Pb/204Pb, 207Pb/204Pb, and 208Pb/204Pb isotope ratios calculated for this component are + 4.4, + 9.1, 0.70411, 18.97, 15.59 and 39.03, respectively. In Pb–Pb isotope space, each volcano defines a distinct linear trend but slight variations are also detected within the various volcanic sequences. The Piton des Neiges volcano yields a distinct and significantly more scattered isotopic distribution than Piton de la Fournaise for both Pb, Hf and Nd isotope tracers. A principal component analysis of the Pb isotope data from Piton de la Fournaise reveals a major contribution of the C and EM-1 components (with a clear Dupal flavor) as main components for the modern Réunion plume. The same components have been identified for Piton des Neiges but with a stronger participation of a depleted mantle component and a weaker EM-1 contribution. The compositional change of the lavas erupted by the Piton des Neiges and Piton de la Fournaise volcanoes is attributed to the impingement of two small-scale blobs of plume material at the base of the Réunion lithosphere. Compared to other hot-spots worldwide, in particular Hawaii and Kerguelen, magmas beneath Réunion are generated from a considerably more homogeneous, compositionally more primitive plume higher in 206Pb. Although shallow-level contamination processes have been locally detected they did not alter significantly the composition of the plume magmas. This is tentatively attributed to mantle dynamics producing small, high-velocity blobs that ascend rapidly through the lithosphere, and to the lack of a well-developed magma chamber at depth in the lithosphere. 相似文献
188.
Larroudé P 《Marine pollution bulletin》2008,57(1-5):47-52
A modified 2DH morphodynamical model was employed to simulate the evolution of large-scale features with major implications for beach nourishment. The study was focused on modelling the evolution of material artificially placed in different parts of the profile, extracting or adding material to the natural bars, and quantifying how the profile responds to different wave climates and nourishment placements. The simulated results were compared with field data from a Mediterranean beach. 相似文献
189.
Jhan Carlo Espinoza Villar Jean Loup Guyot Josyane Ronchail Grard Cochonneau Naziano Filizola Pascal Fraizy David Labat Eurides de Oliveira Juan Julio Ordoez Philippe Vauchel 《Journal of Hydrology》2009,375(3-4):297-311
Former hydrological studies in the Amazon Basin generally describe annual discharge variability on the main stem. However, the downstream Amazon River only represents the mean state of the Amazonian hydrological system. This study therefore uses a new data set including daily discharge in 18 sub-basins to analyze the variability of regional extremes in the Amazon basin, after recalling the diversity of the hydrological annual cycles within the Amazon basin. Several statistical tests are applied in order to detect trends and breaks in the time series. We show that during the 1974–2004 period, the stability of the mean discharge on the main stem in Óbidos is explained by opposite regional features that principally involve Andean rivers: a decrease in the low stage runoff, particularly important in the southern regions, and an increase in the high stage runoff in the northwestern region. Both features are observed from the beginning of the nineties. These features are also observed in smaller meridian sub-basins in Peru and Bolivia. Moreover we show that the changes in discharge extremes are related to the regional pluriannual rainfall variability and the associated atmospheric circulation as well as to tropical large-scale climatic indicators. 相似文献
190.
Jaouher Kerrou Philippe Renard Harrie-Jan Hendricks Franssen Ivan Lunati 《Advances in water resources》2008
The performances of kriging, stochastic simulations and sequential self-calibration inversion are assessed when characterizing a non-multiGaussian synthetic 2D braided channel aquifer. The comparison is based on a series of criteria such as the reproduction of the original reference transmissivity or head fields, but also in terms of accuracy of flow and transport (capture zone) forecasts when the flow conditions are modified. We observe that the errors remain large even for a dense data network. In addition some unexpected behaviours are observed when large transmissivity datasets are used. In particular, we observe an increase of the bias with the number of transmissivity data and an increasing uncertainty with the number of head data. This is interpreted as a consequence of the use of an inadequate multiGaussian stochastic model that is not able to reproduce the connectivity of the original field. 相似文献