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81.
82.
Matthew R. M. IZAWA Roberta L. FLEMMING Penelope L. KING Ron C. PETERSON Phil J. A. McCAUSLAND 《Meteoritics & planetary science》2010,45(4):675-698
Abstract– We have carried out a sample‐correlated spectroscopic and mineralogical investigation of samples from seven different collection sites of the Tagish Lake C2 chondrite. Rietveld refinement of high‐resolution powder X‐ray diffraction (XRD) data was used to determine quantitative major mineral abundances. Thermal infrared (400–4500 cm−1, 2.2–25.0 μm) spectra of the same samples were obtained using diffuse (biconical) reflectance infrared Fourier transform spectroscopy (DRIFTS). Our results are in good agreement with previous studies of the mineralogy of the Tagish Lake meteorite; we find however that Tagish Lake is more varied in major mineralogy than has previously been reported. In particular, we observed two new distinct lithologies, an inclusion‐poor magnetite‐ and sulfide‐rich lithology, and a carbonate‐rich, siderite‐dominated lithology in addition to the previously documented carbonate‐rich and carbonate‐poor lithologies. Grain density for each Tagish Lake sample was calculated from the measured mineral modal abundances and known mineral densities. For powders from three originally intact inclusion‐rich samples, the calculated grain density is 2.77 ± 0.05 g cm−3, in excellent agreement with those reported in the literature for other intact inclusion‐rich Tagish Lake samples. Tagish Lake disaggregated samples have a significantly higher calculated grain density due to their lower saponite‐serpentine content, likely a result of mineral separation in the meltwater holes from which they were collected; the disaggregated samples may not therefore adequately represent bulk samples of the Tagish Lake meteorite. The predominance of very fine‐grained material in the Tagish Lake samples investigated in this study is expected to produce infrared spectra representative of asteroidal regolith. Gypsum and talc have been found by XRD in powders from the inclusion‐rich, intact Tagish Lake samples in this study, and may have been present in the parent body; if present, these hydrous sulfates would complicate the interpretation of possible hydrated mineral features in asteroid infrared spectra. 相似文献
83.
Insights into Li and Li isotope cycling and sub-arc metasomatism from veined mantle xenoliths,Kamchatka 总被引:3,自引:2,他引:1
Ralf Halama Ivan P. Savov Roberta L. Rudnick William F. McDonough 《Contributions to Mineralogy and Petrology》2009,158(2):197-222
Harzburgitic xenoliths cut by pyroxenite veins from Avachinsky volcano, Kamchatka, are derived from the sub-arc mantle and
record element transfer from the slab to the arc. Olivine and orthopyroxene in the harzburgites have Li isotopic compositions
(δ7Li = +2.8 to +5.6) comparable to estimates of the upper mantle (δ7Li ~ +4 ± 2). The pyroxenite veins, which represent modal metasomatism and may therefore provide information about the metasomatic
agent, have mantle-normalized trace element characteristics that suggest overprinting of their mantle source by an aqueous,
slab-derived fluid. These include relative enrichments of Pb over Ce, U over Th and Sr over Nd. Li is enriched relative to
the HREE, and ortho- and clinopyroxene from the veins are in Li elemental and isotopic equilibrium with each other and the
surrounding harzburgite. Vein samples (δ7Li = +3.0 to +5.0) do not record a significant slab-derived δ7Li signature. These observations can be reconciled if slab Li diffusively re-equilibrates in the mantle wedge. Modeling demonstrates
that Li equilibration of small (1–2 cm width) veins or melt conduits is achieved at mantle wedge temperatures within 101–105 years. We conclude that strongly fractionated Li isotopic signatures cannot be sustained for long periods in the sub-arc
mantle, at least at shallow (<70 km) depths.
Electronic supplementary material The online version of this article (doi:) contains supplementary material, which is available to authorized users. 相似文献
84.
Susan P Proctor Sucharita Gopal Asuka Imai Jessica Wolfe David Ozonoff Roberta F White 《Transactions in GIS》2005,9(3):381-396
Spatial autocorrelation analysis was used to identify spatial patterns of 1991 Gulf War (GW) troop locations in relationship to subsequent postwar diagnosis of chronic multisymptom illness (CMI). Criteria for the diagnosis of CMI include reporting from at least two of three symptom clusters: fatigue, musculoskeletal pain, and mood and cognition. A GIS‐based methodology was used to examine associations between potential hazardous exposures or deployment situations and postwar health outcomes using troop location data as a surrogate. GW veterans from the Devens Cohort Study were queried about specific symptoms approximately four years after the 1991 deployment to the Persian Gulf. Global and local statistics were calculated using the Moran's I and G statistics for six selected date periods chosen a priori to mark important GW‐service events or exposure scenarios among 173 members of the cohort. Global Moran's I statistics did not detect global spatial patterns at any of the six specified data periods, thus, indicating there is no significant spatial autocorrelation of locations over the entire Gulf region for veterans meeting criteria for severe postwar CMI. However, when applying local G* and local Moran's I statistics, significant spatial clusters (primarily in the coastal Dammam/Dharhan and the central inland areas of Saudi Arabia) were identified for several of the selected time periods. Further study using GIS techniques, coupled with epidemiological methods, to examine spatial and temporal patterns with larger sample sizes of GW veterans is warranted to ascertain if the observed spatial patterns can be confirmed. 相似文献
85.
Massimo Civita Adriano Fiorucci Roberta Miè 《Geostandards and Geoanalytical Research》2001,25(2-3):431-439
Aluminium was determined in surface and ground waters in the Alba region of NW Italy to provide information on natural and anthropogenic sources of contamination. Determinations were made by a spectrophotometric method based on the aluminium-pyrocatechol complex. The total aluminium content of waters was determined as well as the toxic form of monomeric aluminium, obtained from samples that had been passed through 0.20 μm cellulose filters to remove colloidal and particulate material. Results were correlated with mortality data associated with Alzheimer's disease. There appeared to be a correlation between mortality data and areas having the highest aluminium content of water. 相似文献
86.
Rossano Piazza Ana Carolina Ruiz-Fernández Mauro Frignani Roberta Zangrando Luca Giorgio Bellucci Ivo Moret Federico Páez-Osuna 《Environmental Geology》2008,54(7):1537-1545
Concentrations of polychlorinated biphenyls (PCBs) and polycyclic aromatic hydrocarbons (PAHs) were measured in 13 surficial
sediment samples collected at three lacustrine locations in the surroundings of Mexico City and four coastal areas of the
States of Sinaloa, Sonora, Oaxaca and Veracruz. Total PCB concentrations span the interval 3.18–621 ng g−1. The highest values (63.7–621 ng g−1) were found in Mexico City, which is a highly anthropogenically impacted area, whereas low concentrations (3.18–12.9 ng g−1) were characteristic of seven places, some of them subject to intense hydrodynamics. In these latter cases, values increase
by 18–73 times if normalised against the fine fraction (silt plus clay) content in sediment. Two samples from Mexico City
exceed the ERM (Effect Range Median) guidelines and are likely to cause adverse effects. Samples contain only lower chlorinated
PCBs (mainly 2-, 3- and 4-CB), thus suggesting that the most used PCB commercial mixture was Aroclor 1242. The homologue composition
of the sample taken close to the nuclear power plant of Laguna Verde is identical to this commercial mixture. PAHs in the
same samples have relatively low concentrations (14.9–287 ng g−1), well below ERL (Effect Range Low) guidelines. The composition of PAH mixtures accounts for the influence of both petrogenic
and pyrolitic sources, with these latter prevailing at some places in Mexico City. 相似文献
87.
Arden D. Davis Cathleen J. Webb Jenifer L. Sorensen David J. Dixon Roberta Hudson 《Environmental Earth Sciences》2018,77(2):37
Limestone-based material can reduce concentrations of cadmium below 0.001 mg/L (1 ppb) in water, resulting in > 99% removal efficiency. Thermodynamic constraints appear to be favorable for reactions involving the formation of otavite during cadmium removal. Thermodynamic values for these reactions yield a theoretical removal limit of 0.0015 mg/L or better for cadmium, in reasonable agreement with tests on laboratory and field samples that show cadmium removal at levels less than 0.001 mg/L. 相似文献
88.
Caterina Gozzi Roberta Sauro Graziano Francesco Frondini Antonella Buccianti 《Environmental Earth Sciences》2018,77(16):579
Chemical reactions in aqueous geochemical systems are driven by nonequilibrium conditions, and their dynamics can be deduced through the distributional analysis (identification of probability laws) of complex compositional indices. In this perspective, compositional data analysis offers the possibility to investigate the behavior of the composition as a whole instead of isolated chemical species, with the awareness that multispecies systems are characterized by the simultaneous interactions among all their parts. We addressed this problem using D???1 isometric log-ratio coordinates describing the D compositional dataset of the river chemistry of the Alpine region (D number of variables), thus working in the \({{\mathbb{R}}^{D - 1}}\) statistical sample space. The D???1 coordinates were chosen using the decreasing variance criterion so that each one could provide information about different space–time properties for the investigated geochemical system. Coordinates dominated by heterogeneity appear to be able to capture regime shifts only on a long-time period and monitor processes on a very wide scale. On the other hand, coordinates characterized by lower variability present multimodality, thus capturing the presence of alternative states in the analyzed spatial domain also for the current time. Further developments are needed to determine the ranges of conditions for which variability and other statistics can be useful indicators of regime shifts on different time–space scales in geochemical systems. 相似文献
89.
90.
Isabella Moro Roberta Paccagnella Carlo Barbante Carlo Andreoli 《Marine Ecology》2000,21(3-4):233-245
Abstract. During the austral summer 1993 – 94, microalgal density and biomass were investigated in the sea ice, in the underlying water column, in the melt water and during the formation of the sea ice. Of the 96 taxa identified, 59 were diatoms and 32 were dinoflagellates. Among the remaining five species, Pseudopleurochloris antarctica was very abundant both in the sea ice and in the ice-free waters. Cell densities and biomass of microalgae were higher in the bottom of the sea ice and during the formation of the ice than in the seawater, and diatoms were the dominant group at higher microalgal biomass. Among these, Entomoneis kufferathii , Chaetoceros dichaeta and Fragilariopsis species were the most common taxa. 相似文献