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151.
Virender K. Sharma Frank J. Millero Concetta De Stefano Pasquale Crea 《Marine Chemistry》2007,106(3-4):463-470
The dissociation constants (pK1 and pK2) for methionine have been measured in artificial seawater as a function of salinity (S = 5 to 35) and temperature (5 to 45 °C). The seawater pK2 values were lower than the values in NaCl at the same ionic strength while the pK1 values in seawater were lower only at S = 35. In an attempt to understand these differences, we have made measurements of the constants in Na–Mg–Cl solutions at 25 °C. The measured values have been used to determine the formation of Mg2+ complexes and Pitzer interaction parameters for Mg2+ with methionine. The seawater model with the interaction parameters accounts for the differences between the value of pK1 and pK2 between NaCl and seawater. This study demonstrates that it is important to consider all of the ionic interactions in natural waters when examining the dissociation of organic acids. 相似文献
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Along‐strike evolution of folding,stretching and breaching of supra‐salt strata in the Plataforma Burgalesa extensional forced fold system (northern Spain) 下载免费PDF全文
The Plataforma Burgalesa is a partly exposed extensional forced fold system with an intermediate salt layer, which has developed along the southern portion of the Basque‐Cantabrian Basin from Malm to Early Cretaceous as part of the Bay of Biscay‐Pyrenean rift system. Relationships between syn‐ and pre‐rift strata of the supra‐salt cover sequence and distribution of intra‐cover second‐order faults are observed both along seismic sections and at the surface. These relationships indicate an along‐strike variability of the extensional structural style. After a short period of salt mobilization and forced folding, high slip rates in the central portion of the major basement faults have rapidly promoted brittle behaviour of the salt layer, preventing further salt mobilization and facilitating the propagation of the fault across the salt layer. In contrast, at the tip regions of basement faults, slower slip rates have facilitated ductile salt behaviour, ensuring its further evaporite evacuation, preventing fault propagation across the salt layer and, in essence, allowing for a long‐living forced folding process. Our results indicate the important effect of along‐strike variation in displacement and displacement rates in controlling evaporite behaviour in extensional basins. Amount of displacement and displacement rates are key factors controlling the propagation of basement faults across evaporite layers. In addition, growth strata patterns are recognized as a powerful tool for constraining the up‐dip propagation history of basement faults in extensional fault‐related fold systems with intermediate décollement levels. 相似文献
154.
Vinicio Manzi Rocco Gennari Frits Hilgen Wout Krijgsman Stefano Lugli Marco Roveri Francisco J. Sierro 《地学学报》2013,25(4):315-322
We propose a revised age calibration of the Messinian salinity crisis onset in the Mediterranean at 5.971 Ma based on the recognition of an extra gypsum cycle in the transitional interval of the Perales section (Sorbas basin, Spain) and the revision of the magnetostratigraphy of the Monticino section (Vena del Gesso basin, Italy). This age re‐calibration allows to state more accurately that: (i) the interval encompassing the MSC‐onset is continuous, thus ruling out any erosional feature or stratigraphic hiatus related to a major sea‐level fall affecting the Mediterranean; (ii) the first gypsum was deposited during the summer insolation peak at 5.969 Ma associated with an eccentricity minimum and roughly coincident with glacial stage TG32; (iii) the MSC‐onset was preconditioned by the tectonically‐driven reduction of the hydrological exchanges with the Atlantic Ocean and finally triggered by glacial conditions in the northern hemisphere and by arid conditions in northern Africa. 相似文献
155.
Bruna B. Carvalho Omar Bartoli Fabio Ferri Bernardo Cesare Silvio Ferrero Laurent Remusat Luca S. Capizzi Stefano Poli 《Journal of Metamorphic Geology》2019,37(7):951-975
We investigate the inclusions hosted in peritectic garnet from metapelitic migmatites of the Kinzigite Formation (Ivrea Zone, NW Italy) to evaluate the starting composition of the anatectic melt and fluid regime during anatexis throughout the upper amphibolite facies, transition, and granulite facies zones. Inclusions have negative crystal shapes, sizes from 2 to 10 μm and are regularly distributed in the core of the garnet. Microstructural and micro‐Raman investigations indicate the presence of two types of inclusions: crystallized silicate melt inclusions (i.e., nanogranitoids, NI), and fluid inclusions (FI). Microstructural evidence suggests that FI and NI coexist in the same cluster and are primary (i.e., were trapped simultaneously during garnet growth). FI have similar compositions in the three zones and comprise variable proportions of CO2, CH4, and N2, commonly with siderite, pyrophyllite, and kaolinite, suggesting a COHN composition of the trapped fluid. The mineral assemblage in the NI contains K‐feldspar, plagioclase, quartz, biotite, muscovite, chlorite, graphite and, rarely, calcite. Polymorphs such as kumdykolite, cristobalite, tridymite, and less commonly kokchetavite, were also found. Rehomogenized NI from the different zones show that all the melts are leucogranitic but have slightly different compositions. In samples from the upper amphibolite facies, melts are less mafic (FeO + MgO = 2.0–3.4 wt%), contain 860–1700 ppm CO2 and reach the highest H2O contents (6.5–10 wt%). In the transition zone melts have intermediate H2O (4.8–8.5 wt%), CO2 (457–1534 ppm) and maficity (FeO + MgO = 2.3–3.9 wt%). In contrast, melts at granulite facies reach highest CaO, FeO + MgO (3.2–4.7 wt%), and CO2 (up to 2,400 ppm), with H2O contents comparable (5.4–8.3 wt%) to the other two zones. Our results represent the first clear evidence for carbonic fluid‐present melting in the Ivrea Zone. Anatexis of metapelites occurred through muscovite and biotite breakdown melting in the presence of a COH fluid, in a situation of fluid–melt immiscibility. The fluid is assumed to have been internally derived, produced initially by devolatilization of hydrous silicates in the graphitic protolith, then as a result of oxidation of carbon by consumption of Fe3+‐bearing biotite during melting. Variations in the compositions of the melts are interpreted to result from higher T of melting. The H2O contents of the melts throughout the three zones are higher than usually assumed for initial H2O contents of anatectic melts. The CO2 contents are highest at granulite facies, and show that carbon‐contents of crustal magmas are not negligible at high T. The activity of H2O of the fluid dissolved in granitic melts decreases with increasing metamorphic grade. Carbonic fluid‐present melting of the deep continental crust represents, together with hydrate‐breakdown melting reactions, an important process in the origin of crustal anatectic granitoids. 相似文献
156.
Coastal uplift rate at Matanzas (Cuba) inferred from MIS5e phreatic overgrowths on speleothems 下载免费PDF全文
Jo De Waele Ilenia M. D'Angeli Nicola Tisato Paola Tuccimei Michele Soligo Joaquín Ginés Angel Ginés Joan J. Fornós Igor M. Villa Esteban R. Grau González Stefano M. Bernasconi Tomaso R. R. Bontognali 《地学学报》2017,29(2):98-105
Many morphological elements in Cuba's landscape (e.g. marine terraces, tidal notches) demonstrate that coastal uplift has taken place, but the rate at which this occurs is not known. Carbonate phreatic overgrowths on speleothems have been found in a cave in Central North Cuba, ~1 km from the present coastline at 16 m asl. They form exceptional and unique mushroom‐shaped speleothems and balconies decorating the walls of the rooms. These phreatic overgrowths on speleothems (POS) formed at the oscillating air–water interface in sea‐level controlled anchialine lakes. U/Th dating of these overgrowths suggests ages that are compatible with the Marine Isotope Stage 5e (i.e. 130–115 ka). These POS have fixed this sea‐level highstand and demonstrate that this part of Cuba has been subjected to a much lower uplift rate than previously reported, that is, less than 0.1 mm/year since the last interglacial. 相似文献
157.
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159.
Stefano Catalano Giuseppe Grasso Paolo Mazzoleni Carmelo Monaco Luigi Tortorici 《地学学报》2007,19(4):287-293
On the axial zone of the Southern Apennines the major tectonic boundary between the inner platform (Western platform unit) and the pelagic (Lagonegro units) domains is represented by a thick level of highly deformed rock‐assemblage. Structural analysis reveals that this tectonic unit represents an intracontinental melange complex characterized by a block‐in‐matrix fabric that contains blocks from both hangingwall platform and footwall basin units. This unit comprises different sets of structures that, caused by shearing processes, developed at depths ranging from about 8–9 km to the surface. These tectonites represent the product of a crustal shear zone developed at the major boundary between platform‐basin domains of Adria during the thick‐skinned tectonic processes controlling the Southern Apennines mountain building. 相似文献
160.