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21.
The Multi frequency Scanning Microwave Radiometer (MSMR) onboard Oceasat-1 was used to develop a retrieval method fornear-surface specific humidity by means of multivariate regressiontechnique. The MSMR measures the microwaveradiances in 8 channels at the frequencies of 6.6, 10.7, 18 and 21 GHzfor both vertical and horizontal polarizations. Regression coefficients were derived using the ship reports of the Comprehensive Ocean-Atmosphere Data Set (COADS) for the months of July, October and December, in 1999. Daily near-surface specific humidity data from COADS in 2° × 2° latitude/longitude bins and collocated brightness temperature data from MSMR were used to derive the coefficients. The derived coefficients werevalidated with humidity given in COADS.A linear relationship is established to determine the near-surface specifichumidity from MSMR brightness temperature (Tb) with an rms error of 1.2 g kg-1 for individual situations and an rms errorof 0.84 g kg-1 for monthly time scales over global oceans.The retrieval algorithm is validonly for the open sea regions. 相似文献
22.
Methane-rich fluid inclusions in skarn near the giant REE–Nb–Fe deposit at Bayan Obo, Northern China
We report fluid inclusion data for skarn, formed at the contact between Hercynian granitoids and dolomite of the Proterozoic Bayan Obo Group, in the vicinity of Bayan Obo REE–Nb–Fe deposit, Inner Mongolia, China. Three types of fluid inclusions are identified: two-phase CH4-rich, three-phase liquid–vapour–solid and two-phase aqueous inclusions. Using microthermometry and laser Raman microprobe analysis to calculate isochores for CH4-bearing inclusions, we estimate fluid trapping conditions at T=280 to 344 °C and P<1 to 2.3 kbar. Such conditions are compatible with formation of CH4 inclusions as a result of reaction between graphite in the country rocks (black slate sequence) and fluids derived from magma. The lack of carbonaceous material in the inclusions supports the hypothesis that CH4 was generated during fluid migration rather than by in situ reaction. In contrast to the skarn, and despite the fact that similar graphite-bearing slates are found in the host rocks, no CH4-bearing inclusions have been so far reported from Bayan Obo REE ores. We therefore conclude that the skarn-forming fluids in the contact aureole of the Hercynian granitoids were not involved at any stage in the formation of the Bayan Obo deposit. 相似文献
23.
Fu-yuan Wu Simon A. Wilde Guang-liang Zhang De-you Sun 《Journal of Asian Earth Sciences》2004,23(5):781
Northeastern (NE) China is a well-documented example of a collisional zone characterized by widespread post-orogenic granites and mafic–ultramafic complexes. Based on a study of the Hongqiling and Piaohechuan Cu–Ni sulfide-bearing mafic–ultramafic complexes in central Jilin province, we present geological, petrological, geochemical and geochronological data which indicates their post-orogenic origin.The Hongqiling complex comprises pyroxenite, olivine websterite, lherzolite, gabbro and leucogabbro. Zircon U–Pb SHRIMP analyses on a leucogabbro of the Hongqiling complex yield a weighted mean 206Pb–238U age of 216±5 Ma. The Piaohechuan complex is composed of gabbro, pyroxenite and dolerite, exposed as dikes. A plagioclase-bearing pyroxenite has a U–Pb zircon weighted mean 206Pb–238U age of 217±3 Ma, identical to that of the Hongqiling complex. These ages are coeval with the emplacement of A-type granites in the area, but slightly younger than the regional metamorphism (240 Ma) and syn-orogenic granitic magmatism (246±4 Ma). This suggests that these mafic–ultramafic complexes are post-orogenic in origin. The age data also indicated a short period of lithospheric stabilization of about 30 Ma after cessation of orogenic activity.Geochemical investigation indicates that the primary mafic magma was a lithospheric mantle-derived basalt resulting from the upwelling of asthenosphere due to lithospheric delamination during post-orogenic processes. The magmatic source was contaminated by a small amount of crustal material, and subsequent crystal fractionation resulted in the Cu–Ni mineralization.The widespread occurrence of mafic–ultramafic complexes in the Xing'an–Mongolian Orogenic Belt of NE China and in the Altay–Tianshan–Junggar Orogenic Belt of Northern Xinjiang indicates that mafic intrusions are an important magmatic suite that evolved during post-orogenic processes. Portions of this mafic magma could have underplated the lower crust, and served as the heat source for associated late-stage granitic magmas. 相似文献
24.
Early results from the 2001 census of England allow a preliminary analysis of joblessness. People in the prime working ages (25–49) are more likely to be in work than those in their 50s, but the differences are quite subtle: in particular, men without qualifications are not much more likely to be in work when they are younger, despite the suggestions that too many men cease working in their 50s. The evidence supports the view that there is a national shortfall of demand for labour, that the low-skilled are the least able to compete for scarce jobs, and older people are the most likely to be unqualified. Moreover there is a strong spatial clustering of areas where job availability has declined or grown least, undermining the government's claim that there were often available jobs near to concentrations of people without work. 相似文献
25.
Postglacial topographic evolution of glaciated valleys: a stochastic landscape evolution model 总被引:1,自引:0,他引:1
The retreat of valley glaciers has a dramatic effect on the stability of glaciated valleys and exerts a prolonged influence on the subsequent fluvial sediment transport regime. We have studied the evolution of an idealized glaciated valley during the period following retreat of ice using a numerical model. The model incorporates a stochastic process to represent deep‐seated landsliding, non‐linear diffusion to represent shallow landsliding and an approximation of the Bagnold relation to represent fluvial sediment transport. It was calibrated using field data from several recent surveys within British Columbia, Canada. We present ensemble model results and compare them with results from a deterministic linear‐diffusion model to show that explicit representation of large landslides is necessary to reproduce the morphology and channel network structure of a typical postglacial valley. Our model predicts a rapid rate of fluvial sediment transport following deglaciation with a subsequent gradual decline, similar to that inferred for Holocene time. We also describe how changes in the model parameters affect the estimated magnitude and duration of the paraglacial sediment pulse. Copyright © 2005 John Wiley & Sons, Ltd. 相似文献
26.
27.
Sediment concentration changes in runoff pathways from a forest road network and the resultant spatial pattern of catchment connectivity 总被引:6,自引:0,他引:6
Hydrological connectivity is a term often used to describe the internal linkages between runoff and sediment generation in upper parts of catchments and the receiving waters. In this paper, we identify two types of connectivity: direct connectivity via new channels or gullies, and diffuse connectivity as surface runoff reaches the stream network via overland flow pathways. Using a forest road network as an example of a landscape element with a high runoff source strength, we demonstrate the spatial distribution of these two types of linkages in a 57 km2 catchment in southeastern Australia. Field surveys and empirical modelling indicate that direct connectivity occurs primarily due to gully development at road culverts, where the average sediment transport distance is 89 m below the road outlet. The majority of road outlets were characterised by dispersive flow pathways where the maximum potential sediment transport distance is measured as the available hillslope length below the road outlet. This length has a mean value of 120 m for this catchment. Reductions in sediment concentration in runoff plumes from both pathways are modelled using an exponential decay function and data derived from large rainfall simulator experiments in the catchment. The concept of the volume to breakthrough is used to model the potential delivery of runoff from dispersive pathways. Of the surveyed road drains (n=218), only 11 are predicted to deliver runoff to a stream and the greatest contributor of runoff occurs at a stream crossing where a road segment discharges directly into the stream. The methodology described here can be used to assess the spatial distribution and likely impact of dispersive and gullied pathways on in-stream water quality. 相似文献
28.
Julieta Massaferro Stephen J. Brooks Simon G. Haberle 《Quaternary Science Reviews》2005,24(23-24):2510-2522
We compare high-resolution pollen and chironomid records from the last 15,000 yr in Laguna Facil, southern Chile. Major vegetation and chironomid changes are recorded between ca 14,900 and 14,700 cal. yr BP. During the Lateglacial, changes in the chironomid stratigraphy lag behind changes in the pollen stratigraphy suggesting that the chironomids are responding to changes in the tree canopy or in soil chemistry brought about by vegetational development. At about 7200 cal. yr BP there is a change in the chironomid stratigraphy in advance of changes in the vegetation. This suggests that the response is to regional climatic change. The relatively close correlation of the chironomid and pollen stratigraphies with changes in charcoal concentrations also implicates the importance of fire and/or vulcanism in influencing the dynamics of forest and limnological systems. There is no clear evidence of cooling during the Younger Dryas chronozone in Laguna Facil. 相似文献
29.
Isotope fractionation of electroplated Fe was measured as a function of applied electrochemical potential. As plating voltage was varied from −0.9 V to 2.0 V, the isotopic signature of the electroplated iron became depleted in heavy Fe, with δ56Fe values (relative to IRMM-14) ranging from −0.18(±0.02) to −2.290(±0.006) ‰, and corresponding δ57Fe values of −0.247(±0.014) and −3.354(±0.019) ‰. This study demonstrates that there is a voltage-dependent isotope fractionation associated with the reduction of iron. We show that Marcus’s theory for the kinetics of electron transfer can be extended to include the isotope effects of electron transfer, and that the extended theory accounts for the voltage dependence of Fe isotope fractionation. The magnitude of the electrochemically-induced fractionation is similar to that of Fe reduction by certain bacteria, suggesting that similar electrochemical processes may be responsible for biogeochemical Fe isotope effects. Charge transfer is a fundamental physicochemical process involving Fe as well as other transition metals with multiple isotopes. Partitioning of isotopes among elements with varying redox states holds promise as a tool in a wide range of the Earth and environmental sciences, biology, and industry. 相似文献
30.
Gold partitioning in melt-vapor-brine systems 总被引:5,自引:0,他引:5
Adam C. Simon Mark R. Frank Philip A. Candela Christoph A. Heinrich 《Geochimica et cosmochimica acta》2005,69(13):3321-3335
We used laser-ablation inductively coupled plasma mass spectrometry to measure the solubility of gold in synthetic sulfur-free vapor and brine fluid inclusions in a vapor + brine + haplogranite + magnetite + gold metal assemblage. Experiments were conducted at 800°C, oxygen fugacity buffered at Ni-NiO (NNO), and pressures ranging from 110 to 145 MPa. The wt% NaCl eq. of vapor increases from 2.3 to 19 and that of brine decreases from 57 to 35 with increasing pressure. The composition of the vapors and brines are dominated by NaCl + KCl + FeCl2 + H2O. Gold concentrations in vapor and brine decrease from 36 to 5 and 50 to 28 μg/g, respectively, and the calculated vapor:brine partition coefficients for gold decrease from 0.72 to 0.17 as pressure decreases from 145 to 110 MPa. These data are consistent with the thermodynamic boundary condition that the concentration of gold in the vapor and brine must approach a common value as the critical pressure is approached along the 800°C isotherm in the NaCl-KCl-FeCl2-HCl-H2O system.We use the equilibrium constant for gold dissolution as AuOH0, extrapolated from lower temperature and overlapping pressure range, to calculate expected concentrations of AuOH0 in our experimental vapors. These calculations suggest that a significant quantity of gold in our experimental vapors is present as a non-hydroxide species. Possible chloridogold(I) species are hypothesized based on the positively correlated gold and chloride concentrations in our experimental vapors. The absolute concentration of gold in our synthetic vapor, brine, and melt and calculated mass partition coefficients for gold between these physicochemically distinct magmatic phases suggests that gold solubility in aqueous fluids is a function of aqueous phase salinity, specifically total chloride concentration, at magmatic conditions. However, though we highlight here the effect of salinity, the combination of our data with data sets from lower temperatures evinces a significant decrease in gold solubility as temperature drops from 800°C to 600°C. This decrease in solubility has implications for gold deposition from ascending magmatic fluids. 相似文献