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81.
An 11-month observation of dissolved and particulate organic matter, chlorophyll a(Chl a), C18 Sep-Pak extractable hydrophobic dissolved organic matter (hDOM) fraction and associated dissolved trace metals (Cd,
Cu, V, Co, Ni, Mo, U) was performed in the Lot–Garonne River system. This system includes the Riou Mort, the Lot River and
the downstream reaches of the Garonne River and represents the fluvial transport path of trace metals between the major point
source of polymetallic pollution, located in the Riou Mort watershed and the Gironde estuary. Spatial and temporal variations
of dissolved and particulate organic carbon and Chl areflect the presence of different types of organic matter and their relation with the hDOM fraction. Maximum Chl a/POC ratios (up to 0.03), indicate intense phytoplankton production from March to May. In the Lot River (Temple), DOC and
POC concentrations were clearly higher and mean Chl a concentration (2.8 mg g−1) was about three times higher than those of the other sites. High Chl a/POC ratios suggest high phytoplankton activity with maxima in spring and late summer. In the Riou Mort River, very high POC
concentrations of up to 40 (mean: 20) occurred, whereas Chl a concentrations were relatively low indicating low phytoplankton activity. High, strongly variable DOC and POC concentrations
suggest important natural (Carboniferous soils, forests) or anthropogenic (e.g., former coal mines, waste areas, agriculture,
sewage) carbon sources within the small Riou Mort watershed. Despite high DOC concentrations in the Riou Mort River, hDOM
metal fractions were generally lower than those at the other sites. The general order of decreasing binding strength between
metals and the organic hydrophobic phase (Cu, U > Co, Ni > V, Mo > Cd) at all four sites was in good agreement with the Irving–William
series of transition element affinity towards organic ligands. Accordingly, the role of the hydrophobic phase in dissolved
Cd transport appeared to be negligible, whereas the hDOM–Cu fraction strongly contributed to dissolved Cu transport. 相似文献
82.
In this study, hydrogeologic and hydrochemical information from the Mersin-Erdemli groundwater system were integrated and
used to determine the main factors and mechanisms controlling the chemistry of groundwaters in the area and anthropogenic
factors presently affecting them. The PHREEQC geochemical modeling demonstrated that relatively few phases are required to
derive water chemistry in the area. In a broad sense, the reactions responsible for the hydrochemical evolution in the area
fall into four categories: (1) silicate weathering reactions; (2) dissolution of salts; (3) precipitation of calcite, amorphous
silica and kaolinite; (4) ion exchange. As determined by multivariate statistical analysis, anthropogenic factors show seasonality
in the area where most contaminated waters related to fertilizer and fungicide applications that occur during early summer
season. 相似文献
83.
Two cases of on-ice and off-ice air flow characterizing the opposite weather situations over the ice-edge zone in the northern Baltic Sea are analysed on the basis of aircraft observations, and modelled using atwo-dimensional mesoscale model. The stable boundary layer (SBL) during theon-ice flow exhibited little thermal modification, but a low-level jet (LLJ) was generated at the 250-m high top of the SBL. In the model, the LLJ was associated with inertial oscillations in space, while the baroclinicity explained the shape of the wind profile well above the SBL. Although the observed LLJ was most pronounced over the ice, the modelling suggests that it was not generated by the ice edge but by the coastline some 400 km upwind of the ice edge, where a much more drastic change in the thermal stratification and surface roughness took place. The generation, maintenance, and strength of the LLJ were very sensitive to the parameterization of turbulent mixing in the SBL. In the case of the off-ice flow, the modification of the air mass and the development of a convective boundary layer (CBL) both over the ice and open sea were reasonably well modelled. Sensitivity runs suggested that it was essential to take into account the effects of subgrid-scale leads, a forest in the archipelago (which was crossed by the air flow), and water vapour condensationinto ice crystals. The heat flux from leads was particularly important for the heatbudget of the CBL, and the observed growth of the CBL was partly due to theeffective mixing over the rough and relatively warm forest. 相似文献
84.
Summary ?Microclimatological data obtained during a field experiment in the nongrowing winter period were used to study the microclimatologically
stable night conditions of a 200 × 150 m miscanthus (Miscanthus cv. giganteus) stand and compared to open field conditions. The microclimatological pattern within the miscanthus canopy
was characterized by long-wave radiative cooling of the plant stand and by an established temperature inversion within the
canopy at calm nights. The results show that there are significant differences in air temperature and energy balance components
between the open field and the miscanthus field during calm and clear nights. In general, net radiation difference during
the cold and calm nights was relatively constant and about 20 W m−2 less negative in miscanthus (because of lower surface temperatures) than at the open field. Air temperature differences also
remained fairly constant and were up to 3 °C lower than at the open field (at the height of 1 m). Through thermal inversion
cold air accumulated in the lower parts of the canopy as shown by the vertical air temperature profiles. They showed a greater
amplitude within the diurnal cycle in the miscanthus stand than in the open field. Through the onset of wind, temperature
profiles changed rapidly and differences diminished. Vertical katabatic air drainage into the canopy layers was estimated
indirectly by using the energy balance approach. It was calculated from the significant energy balance closure gap and showed
a mean air exchange rate of up to 22 m3 m−2 h−1, related to a stand volume of 1 m2 area and 4 m height, during the mostly calm and clear nights, depending on the canopy net radiation and turbulent heat exchange
forced by slight wind spells. Quantitative uncertainties in calculated cold air drainage which are introduced by the measurement
method and certain assumptions in the calculations, were considered in a sensitivity analysis. In spite of these uncertainties
evidence of katabatic cold air flow is given.
Received July 29, 1999; revised June 11, 2001; accepted March 14, 2002 相似文献
85.
Laurent Desmurs Othmar Müntener Gianreto Manatschal 《Contributions to Mineralogy and Petrology》2002,144(3):365-382
Exhumation of subcontinental mantle rocks and its exposure at the seafloor is known from different magma-poor passive continental margins. However, the transition from largely amagmatic passive rifting to seafloor spreading is still poorly documented. In this contribution we use MOR-type gabbroic and basaltic rocks to characterize the magmatism associated with the formation of an ancient ocean-continent transition preserved in the Platta nappe, eastern Switzerland. Gabbros form individual small intrusions into exhumed serpentinized subcontinental mantle rocks. Mineral and bulk-rock chemistry and simple modeling indicate that each gabbro body records different magmatic processes ranging from predominantly fractional crystallization to solidification without fractionation. Mg numbers and Ni contents of equilibrium olivine calculated from basalts and gabbros indicate that few mafic rocks are primary melts but most represent fractionated compositions ranging from T- to N-MORB. Whereas most mafic rocks may be explained by low to moderate degrees of melting of an N-MORB-type mantle, the source of some basalt is enriched in incompatible elements. This compositional variation seems to correlate with the spatial distribution of the mafic rocks within the ocean-continent transition whereby mafic rocks with T-MORB signatures occur close to the continental margin whereas N-MORB signatures are predominantly found oceanwards. As in an opening system time and space are closely linked, the chemical evolution of the mafic rocks along the ocean-continent transitions suggests continuous thinning of the subcontinental mantle and associated uplift of the underlying asthenosphere during the time between the crustal and the lithospheric breakup. 相似文献
86.
87.
88.
Mantle Convection Modeling with Viscoelastic/Brittle Lithosphere: Numerical Methodology and Plate Tectonic Modeling 总被引:1,自引:0,他引:1
--The earth's tectonic plates are strong, viscoelastic shells which make up the outermost part of a thermally convecting, predominantly viscous layer. Brittle failure of the lithosphere occurs when stresses are high. In order to build a realistic simulation of the planet's evolution, the complete viscoelastic/brittle convection system needs to be considered. A particle-in-cell finite element method is demonstrated which can simulate very large deformation viscoelasticity with a strain-dependent yield stress. This is applied to a plate-deformation problem. Numerical accuracy is demonstrated relative to analytic benchmarks, and the characteristics of the method are discussed. 相似文献
89.
The bulk composition of organic matter and saturated and aromatic hydrocarbons extracted from 16 samples collected from two Kuperschiefer profiles in the Rudna mine,Southwest Poland has been analyzed to study the role of organic matter during base metal enrichment in the Kupferschiefer shale.The results indicated that the extract yields and saturated hydrocarbon yields decreased with increasing base metal contents.GC and GC/MS analyses indicated that n -alkanes and alkylated aromatic compounds were depleted and may have served as hydrogen donators for thermochemical sulfate reduction.The enrichment of base metal is closely connected with the destruction of hydrocarbons. 相似文献
90.
An Mw based earthquake Catalogue for central, northern and northwestern Europe using a hierarchy of magnitude conversions 总被引:3,自引:1,他引:3
Data from 25 local catalogues and 30special studies of earthquakes in central,northern and northwestern Europe have beenincorporated into a Databank. The dataprocessing includes discriminating eventtypes, eliminating fake events and dupletsand converting different magnitudes andintensities to Mw if this is not givenby the original source. The magnitudeconversion is a key task of the study andimplies establishment of regressionequations where no local relations exist.The Catalogue contains tectonic events fromthe Databank within the area44°N–72°N,25°W–32°E and the time period1300–1993. The lower magnitude level forthe Catalogue entries is setat Mw == 3.50. The area covered by thedifferent catalogues are associated withpolygons. Within each polygon only datafrom one or a small number of the localcatalogues, supplemented by data fromspecial studies, enter the Catalogue. Ifthere are two or more such catalogues orstudies providing a solution for an event,a priority algorithm selects one entry forthe Catalogue. Then Mw is calculatedfrom one of the magnitude types, or frommacroseismic data, given by the selectedentry according to another priority scheme.The origin time, location, Mw magnitude and reference are specified for eachentry of the Catalogue. So is theepicentral intensity, I0, if providedby the original source. Following thesecriteria, a total of about 5,000earthquakes constitute the Catalogue.Although originally derived for the purposeof seismic hazard calculation within GSHAP,the Catalogue provides a data base for manytypes of seismicity and seismic hazardstudies. 相似文献