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Implications for behavior of volatile elements during impacts—Zinc and copper systematics in sediments from the Ries impact structure and central European tektites 下载免费PDF全文
Zuzana Rodovská Tomáš Magna Karel Žák Chizu Kato Paul S. Savage Frédéric Moynier Roman Skála Josef Ježek 《Meteoritics & planetary science》2017,52(10):2178-2192
Moldavites are tektites genetically related to the Ries impact structure, located in Central Europe, but the source materials and the processes related to the chemical fractionation of moldavites are not fully constrained. To further understand moldavite genesis, the Cu and Zn abundances and isotope compositions were measured in a suite of tektites from four different substrewn fields (South Bohemia, Moravia, Cheb Basin, Lusatia) and chemically diverse sediments from the surroundings of the Ries impact structure. Moldavites are slightly depleted in Zn (~10–20%) and distinctly depleted in Cu (>90%) relative to supposed sedimentary precursors. Moreover, the moldavites show a wide range in δ66Zn values between 1.7 and 3.7‰ (relative to JMC 3‐0749 Lyon) and δ65Cu values between 1.6 and 12.5‰ (relative to NIST SRM 976) and are thus enriched in heavy isotopes relative to their possible parent sedimentary sources (δ66Zn = ?0.07 to +0.64‰; δ65Cu = ?0.4 to +0.7‰). In particular, the Cheb Basin moldavites show some of the highest δ65Cu values (up to 12.5‰) ever observed in natural samples. The relative magnitude of isotope fractionation for Cu and Zn seen here is opposite to oxygen‐poor environments such as the Moon where Zn is significantly more isotopically fractionated than Cu. One possibility is that monovalent Cu diffuses faster than divalent Zn in the reduced melt and diffusion will not affect the extent of Zn isotope fractionation. These observations imply that the capability of forming a redox environment may aid in volatilizing some elements, accompanied by isotope fractionation, during the impact process. The greater extent of elemental depletion, coupled with isotope fractionation of more refractory Cu relative to Zn, may also hinge on the presence of carbonyl species of transition metals and electromagnetic charge, which could exist in the impact‐induced high‐velocity jet of vapor and melts. 相似文献
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Spatial variations of the magnetic field, measured at the Earth's surface, are mainly due to geological inhomogeneities within the crust. The present state of the crust, in turn, reflects its past dynamical processes and evolution. We analyzed the magnetic field intensity along a few but densely sampled profiles in a Tertiary volcanic province near Bonn, Germany. The aim was to find out whether the variation of the magnetic intensity can be related to a deterministic, although chaotic, generating system or to a stochastic one. In the former case, the geodynamical history would depend on a few degrees of freedom, whereas in the latter case, the parameters to take into account were so many that a statistic approach appears to be more suitable. Since strange attractors do not emerge from the analyzed data, we exclude the presence of a chaos generating system. Autocorrelation functions and a rescaled-range analysis, on the other hand, reveal and quantify a certain degree of correlation among successive data points and allow calculation of a range of spectral exponents in log-log diagrams, which are clearly distinct from those of white noise and Brownian motion. Only one of the profiles exhibits similarity to uncorrelated or white noise. In this case, the signal variations do not result from the local geology but from a buried gas pipe-line, aligned subparallel to that profile. If self-organized crustal evolution generally produces signatures that can be described as correlated noise, within a limited bandwidth of spectral exponents, erraneous or disturbed data could eventually be discriminated from records containing purely natural data by applying analysis tools of the dynamic system theory together with autocorrelation tests. 相似文献
15.
Elisabetta?Brizi Sabrina?NazzareniEmail author Francesco?Princivalle Pier?Francesco?Zanazzi 《Contributions to Mineralogy and Petrology》2003,145(5):578-584
Optically homogeneous augite xenocrysts, closely associated with spinel–peridotite nodules, occur in alkali basalts from Hannuoba (Hebei province, China). They were studied by electron and X-ray diffraction to define the occurrence and significance of pigeonite exsolution microtextures. Sub-calcic augite (Wo34) exsolved into En62–62Fs25–21Wo13–17 pigeonite and En46–45Fs14–14Wo40–42 augite, as revealed by TEM through diffuse coarser (001) lamellae (100–300 Å) and only incipient (100) thinner ones (<70 Å). C2/c augite and P21/c pigeonite lattices, measured by CCD-XRD, relate through a(Aug)?a(Pgt), b(Aug)?b(Pgt), c(Aug)≠c(Pgt) [5.278(1) vs 5.189(1)Å] and β(Aug)≠β(Pgt) [106.55(1) vs 108.55(2)°]. Cell and site volumes strongly support the hypothesis that the augite xenocrysts crystallised at mantle depth from alkaline melts. After the augite xenocrysts entered the magma, (001) lamellae first formed by spinodal decomposition at a Tmin of about 1,100 °C, and coarsened during very rapid transport to the surface; in a later phase, possibly on cooling, incipient (100) lamellae then formed. 相似文献
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A. Le Gall M.A. Janssen A.G. Hayes C. Savage R.D. Lorenz R.L. Kirk S. Wall E.R. Stofan the Cassini Radar Team 《Icarus》2011,213(2):608-624
Large expanses of linear dunes cover Titan’s equatorial regions. As the Cassini mission continues, more dune fields are becoming unveiled and examined by the microwave radar in all its modes of operation (SAR, radiometry, scatterometry, altimetry) and with an increasing variety of observational geometries. In this paper, we report on Cassini’s radar instrument observations of the dune fields mapped through May 2009 and present our key findings in terms of Titan’s geology and climate. We estimate that dune fields cover ∼12.5% of Titan’s surface, which corresponds to an area of ∼10 million km2, roughly the area of the United States. If dune sand-sized particles are mainly composed of solid organics as suggested by VIMS observations (Cassini Visual and Infrared Mapping Spectrometer) and atmospheric modeling and supported by radiometry data, dune fields are the largest known organic reservoir on Titan. Dune regions are, with the exception of the polar lakes and seas, the least reflective and most emissive features on this moon. Interestingly, we also find a latitudinal dependence in the dune field microwave properties: up to a latitude of ∼11°, dune fields tend to become less emissive and brighter as one moves northward. Above ∼11° this trend is reversed. The microwave signatures of the dune regions are thought to be primarily controlled by the interdune proportion (relative to that of the dune), roughness and degree of sand cover. In agreement with radiometry and scatterometry observations, SAR images suggest that the fraction of interdunes increases northward up to a latitude of ∼14°. In general, scattering from the subsurface (volume scattering and surface scattering from buried interfaces) makes interdunal regions brighter than the dunes. The observed latitudinal trend may therefore also be partially caused by a gradual thinning of the interdunal sand cover or surrounding sand sheets to the north, thus allowing wave penetration in the underlying substrate. Altimetry measurements over dunes have highlighted a region located in the Fensal dune field (∼5° latitude) where the icy bedrock of Titan is likely exposed within smooth interdune areas. The hemispherical assymetry of dune field properties may point to a general reduction in the availability of sediments and/or an increase in the ground humidity toward the north, which could be related to Titan’s asymmetric seasonal polar insolation. Alternatively, it may indicate that either the wind pattern or the topography is less favorable for dune formation in Titan’s northern tropics. 相似文献
18.
Observing Entrainment Processes Using a Small Unmanned Aerial Vehicle: A Feasibility Study 总被引:1,自引:0,他引:1
Measurement flights with the meteorological mini aerial vehicle (M $^2$ AV) were performed in spring 2011 to assess the capability of an unmanned aerial vehicle (UAV) to measure the structure of the transition zone between the convective boundary layer and the stably stratified free atmosphere. The campaign took place at the Meteorological Observatory Lindenberg/Richard-Aßmann-Observatory of the German Meteorological Service. Besides the M $^2$ AV flights, observations were made from a 12-m and a 99-m tower, a sodar, two ceilometers, radiosondes, and a tethered balloon with sensor packages at six different levels. M $^2$ AV measurements were intentionally combined with remote sensing systems. The height range of the entrainment zone as well as its diurnal cycle were provided by the remote sensing instruments. The UAV provided the high-resolution in situ data of temperature and wind for the study of turbulent processes. It is shown that the M $^2$ AV is able to maintain constant altitude with very small deviations—a pre-requisite to study processes inside the often quite thin entrainment zone and that M $^2$ AV high-resolution wind and temperature measurements allow for very detailed studies of the fine structure of the atmosphere and thus for the identification of quite local and/or short-duration processes such as overshooting thermals or downward intrusions of warm air. Spatial series measured by the M $^2$ AV during horizontal flights show turbulent exchange of heat in short turbulent bursts at heights close to and within the entrainment zone. Scaled vertical profiles of vertical velocity, potential temperature variance, and sensible heat flux confirm the general shape found by previous measurements and numerical studies. 相似文献
19.
Azzurra Zucchini Paola Comodi Sabrina Nazzareni Michael Hanfland 《Physics and Chemistry of Minerals》2014,41(10):783-793
Synchrotron single-crystal X-ray diffraction experiments at high-pressure and high-temperature conditions were performed up to 20 GPa and 573.0(2) K on a fully ordered stoichiometric dolomite and a partially disordered stoichiometric dolomite [order parameter, s = 0.26(6)]. The ordered dolomite was found to be stable up to approximately 14 GPa at ambient temperature and up to approximately 17 GPa at T = 573.0(2) K. The P–V data from the ambient temperature experiments were analysed by a second-order Birch–Murnaghan equation-of-state giving K 0 = 92.7(9) GPa for the ordered dolomite and K 0 = 92.5(8) GPa for the disordered dolomite. The high-temperature data, collected for the ordered sample, were fitted by a third-order Birch–Murnaghan equation-of-state resulting in K 0 = 95(6) GPa and K′ = 2.6(7). In order to compare the three experiments results, a third-order Birch–Murnaghan equation-of-state was also calculated for the ambient temperature experiments giving K 0 = 93(3) GPa, K′ = 3.9(6) for the ordered dolomite and K 0 = 92(3) GPa, K′ = 4.0(4) for the disordered dolomite. The derived axial moduli show that dolomite compresses very anisotropically, being the c-axis approximately three times more compressible than the a-axis. The axial compressibility increases as T increases, and the a-axis is the most temperature-influenced axis. On the contrary, axial compressibility is not influenced by disordering. Structural refinements at different pressures show that Ca and Mg octahedra are almost equally compressible in the ordered dolomite with K(CaO6) = 109(4) GPa and K(MgO6) = 103(3) GPa. On the contrary, CaO6 compressibility is reduced and MgO6 compressibility is increased in the disordered crystal structure where K(CaO6) = 139(4) GPa and K(MgO6) = 89(4) GPa. Disordering is found to increase CaO6 and to decrease MgO6 bond strengths, thus making stiffer the Ca octahedron and softer the Mg octahedron. Cation polyhedra are distorted in both ordered and disordered dolomites and they increase in regularity as P increases. Ordered dolomite approaches regularity at approximately 14 GPa. The increase in regularity of octahedra in the disordered dolomite is strongly affected by the very slow regularization of MgO6 with respect to CaO6. The phase transition to the high-pressure polymorph of dolomite (dolomite-II), which is driven by a significant increase in the regularity of both cations polyhedra and mineral crystal structure, occurs in the ordered dolomite at ambient temperature at approximately 14 GPa; whereas no clear evidences of phase transition were observed as regards the disordered crystal structure. 相似文献
20.
Ken Kobayashi Jonathan Cirtain Amy R. Winebarger Kelly Korreck Leon Golub Robert W. Walsh Bart De Pontieu Craig DeForest Alan Title Sergey Kuzin Sabrina Savage Dyana Beabout Brent Beabout William Podgorski David Caldwell Kenneth McCracken Mark Ordway Henry Bergner Richard Gates Sean McKillop Peter Cheimets Simon Platt Nick Mitchell David Windt 《Solar physics》2014,289(11):4393-4412
The High-Resolution Coronal Imager (Hi-C) was flown on a NASA sounding rocket on 11 July 2012. The goal of the Hi-C mission was to obtain high-resolution (≈?0.3?–?0.4′′), high-cadence (≈?5 seconds) images of a solar active region to investigate the dynamics of solar coronal structures at small spatial scales. The instrument consists of a normal-incidence telescope with the optics coated with multilayers to reflect a narrow wavelength range around 19.3 nm (including the Fe xii 19.5-nm spectral line) and a 4096×4096 camera with a plate scale of 0.1′′?pixel?1. The target of the Hi-C rocket flight was Active Region 11520. Hi-C obtained 37 full-frame images and 86 partial-frame images during the rocket flight. Analysis of the Hi-C data indicates the corona is structured on scales smaller than currently resolved by existing satellite missions. 相似文献