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381.
Franziska D.H. Wilke Mónica Vásquez Thomas Wiersberg Rudolf Naumann Jörg Erzinger 《Applied Geochemistry》2012
The aim of this experimental study was to evaluate and compare the geochemical impact of pure and impure CO2 on rock forming minerals of possible CO2 storage reservoirs. This geochemical approach takes into account the incomplete purification of industrial captured CO2 and the related effects during injection, and provides relevant data for long-term storage simulations of this specific greenhouse gas. Batch experiments were conducted to investigate the interactions of supercritical CO2, brine and rock-forming mineral concentrates (albite, microcline, kaolinite, biotite, muscovite, calcite, dolomite and anhydrite) using a newly developed experimental setup. After up to 42 day (1000 h) experiments using pure and impure supercritical CO2 the dissolution and solution characteristics were examined by XRD, XRF, SEM and EDS for the solid, and ICP–MS and IC for the fluid reactants, respectively. Experiments with mixtures of supercritical CO2 (99.5 vol.%) and SO2 or NO2 impurities (0.5 vol.%) suggest the formation of H2SO4 and HNO3, reflected in pH values between 1 and 4 for experiments with silicates and anhydrite and between 5 and 6 for experiments with carbonates. These acids should be responsible for the general larger amount of cations dissolved from the mineral phases compared to experiments using pure CO2. For pure CO2 a pH of around 4 was obtained using silicates and anhydrite, and 7–8 for carbonates. Dissolution of carbonates was observed after both pure and impure CO2 experiments. Anhydrite was corroded by approximately 50 wt.% and gypsum precipitated during experiments with supercritical CO2 + NO2. Silicates do not exhibit visible alterations during all experiments but released an increasing amount of cations in the reaction fluid during experiments with impure CO2. Nonetheless, precipitated secondary carbonates could not be identified. 相似文献
382.
Thomas Kalbacher Jens-Olaf Delfs Haibing Shao Wenqing Wang Marc Walther Luis Samaniego Christoph Schneider Rohini Kumar Andreas Musolff Florian Centler Feng Sun Anke Hildebrandt Rudolf Liedl Dietrich Borchardt Peter Krebs Olaf Kolditz 《Environmental Earth Sciences》2012,65(5):1367-1380
Numerical modeling of interacting flow and transport processes between different hydrological compartments, such as the atmosphere/land surface/vegetation/soil/groundwater systems, is essential for understanding the comprehensive processes, especially if quantity and quality of water resources are in acute danger, like e.g. in semi-arid areas and regions with environmental contaminations. The computational models used for system and scenario analysis in the framework of an integrated water resources management are rapidly developing instruments. In particular, advances in computational mathematics have revolutionized the variety and the nature of the problems that can be addressed by environmental scientists and engineers. It is certainly true that for each hydro-compartment, there exists many excellent simulation codes, but traditionally their development has been isolated within the different disciplines. A new generation of coupled tools based on the profound scientific background is needed for integrated modeling of hydrosystems. The objective of the IWAS-ToolBox is to develop innovative methods to combine and extend existing modeling software to address coupled processes in the hydrosphere, especially for the analysis of hydrological systems in sensitive regions. This involves, e.g. the provision of models for the prediction of water availability, water quality and/or the ecological situation under changing natural and socio-economic boundary conditions such as climate change, land use or population growth in the future. 相似文献
383.
384.
Rudolf Brázdil 《GeoJournal》1994,32(3):199-205
On the basis of documentary evidence, proxy-data and instrumental observations, the climatic fluctuation during the last millennium in the Czech Lands is analysed. According to narrative sources, the warmest period falls between the 1260s–1380s, documents for Lamb's (1984) Medieval Warm Epoch in 1150–1300 are missing. The prevalence of extremely cold and also rainy periods, as an expression of the Little Ice Age, is most conspicuous in the 15th century, in the 1590s and, with three interruptions, between the 1730s–1850s. Since the latter half of the 19th century a rising temperature trend has manifested itself. A regional climatic scenario for the model of global warming is discussed in relation to the observed trends in the Czech Lands. 相似文献
385.
386.
Rudolf Tschpe 《Astronomische Nachrichten》1995,316(5):368-368