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91.
92.
Joseph A. Shacat William J. Green Eric H. Decarlo Silvia Newell 《Aquatic Geochemistry》2004,10(3-4):325-352
Lake Joyce is one of the least studied lakes of the McMurdo Dry Valleys. Similar to other lakes in this region, Lake Joyce is a closed-basin, permanently ice-covered, meromictic lake. We present here a detailed investigation of major ions, nutrients, and dissolved trace elements for Lake Joyce. Specifically, we investigate the role of iron and manganese oxides and hydrous oxides in trace metal cycling.Lake Joyce is characterized by fresh, oxic waters overlying an anoxic brine, primarily Na–Cl. Surface waters have a maximum nitrate concentration of 26M with a molar dissolved inorganic nitrogen to phosphorus ratio of 477. The supply of nitrogen is attributed to atmospheric deposition, possibly from polar stratospheric clouds. Dissolved phosphorus is scavenged by hydrous iron oxides. The pH is highest (10.15) just beneath the 7-m thick ice cover and decreases to a minimum of 7.29 in the redox transition zone. Dissolved Al exceeds 8M in surface waters, and appears to be controlled by equilibrium with gibbsite. In contrast, concentrations of other trace elements in surface waters are quite low (e.g., 5.4nM Cu, 0.19nM Co, <20pM La). Dissolved Fe, Mn, Ni and Cd were below our detection limits of 13 nM, 1. 8 nM, 4.7 nM and 15pM (respectively) in surface waters. There was a 6-m vertical separation in the onset of Mn and Fe reduction, with dissolved Mn appearing higher in the water column than Fe. Based on thermodynamic calculations, dissolved Mn appears to be controlled by equilibrium with hausmannite (Mn3 O4 ). Co tracks the Mn profile closely, suggesting Co(III) is bound in the lattice of Mn oxides, whereas the Ce profile is similar, yet the Ce anomaly suggests oxidative scavenging of Ce. Release of Cu, Ni, Cd and trivalent REE appears to be controlled by pH-induced desorption from Fe and Mn oxides, although Cu (and perhaps Ni) may be scavenged by organic matter in surface waters. 相似文献
93.
William J. Green Brian R. Stage Bonnie Jo Bratina Shannon Wagers Adam Preston Kevin O’bryan Joseph Shacat Silvia Newell 《Aquatic Geochemistry》2004,10(3-4):303-323
Lake Vanda is a closed-basin, permanently ice-covered lake located in the Wright Valley of Antarctica. The lakes more important geochemical features include the fact that it is fed by a single glacial melt water stream for only 6–8weeks out of the year; that it has remained stratified for more than a millennium; and that, like other lakes in the region, it is remote from anthropogenic influence. These, together with the fact that it is among the least biologically productive lakes in the world, make it an ideal system for examining the transport, cycling and fate of trace metals in the aquatic environment. Like others before us, we view this lake as a natural geochemical laboratory, a flask in the desert. This paper presents the first set of closely spaced, vertical, profiles for dissolved and particulate Mn, Fe, Ni, Cu, Zn and Cd in the water column. Despite the absence of an outflow, metals in the fresh upper waters of the lake have extremely low concentrations, in the pico-molar to nano-molar range, and are partitioned largely into dissolved rather than particulate phases. Efficient metal scavenging by particles from these oxygen-rich waters is indicated. Significant increases in metal concentrations begin to appear at depth, between 57 and 60m, and these increases coincide with the onset of manganese oxide dissolution in oxic, but lower pH waters. Vertical profiles suggest that the entire suite of trace metals (Ni, Cu, Zn, and Cd) is being released from manganese oxide carrier phases. Thermodynamic analysis indicates that Mn3 O4 (i.e., the mineral hausmannite) may be important in metal sequestration and recycling in the deeper waters of Lake Vanda. Manganese-reducing organisms reported by Bratina etal. (1998) are active in the zone of metal release and these could also contribute to the observed cycling. 相似文献
94.
Andrew?SwalesEmail author Iain?T.?MacDonald Malcolm?O.?Green 《Estuaries and Coasts》2004,27(2):225-243
Isolated patches ofSpartina anglica (cordgrass) at two sites on a wave-exposed mid-intertidal flat of the 340 km2 Manukau Harbor (Auckland, New Zealand) have developed very differently since being planted in the mid-1970s. Although the
two sites are only 0.5 km apart and at the same intertidal elevation,Spartina patches at the easternmost site (site 1) have as much as an order of magnitude higher biomass and accumulated sediment volume
thanSpartina patches at site 2. A field experiment was conducted to characterize waves and associated sediment dynamics at each site,
which might explain whySpartina patches at the two sites have developed so differently over the past 25 yr or so. Suspended sediments were measured and wave
characteristics were inferred from subsurface pressure data measured for 5 wk at bothSpartina sites and at an intermediate location. Bed-orbital speeds and frictional wave-energy dissipation were consistently lower
at the easternmost site with the largerSpartina patches. The west-to-east reduction in wave energy is due to the spatial arrangement of theSpartina sites relative to the predominant wind fetches. The wave-energy gradient is maintained by tidal-cycle variations in fetch
and bed friction and results in a west-to-east reduction in sand suspension. Silt, which is largely resuspended under southwest
winds, is redeposited in the low wave-energy conditions in and around the larger site 1Spartina patches. Shell accumulation bySpartina patches at site 1 occurs infrequently, during southwest winds >10 m s−1 and water depths >0.7 m, when waves are least attenuated by bed friction. Large between-site differences in the growth of
and sediment accumulation by theSpartina patch are consistent with the observed wave-energy gradient. The resulting spatial patterns of silt, sand, and shell resuspension
and deposition directly influence the rate of sediment accumulation bySpartina patches and the composition of accumulated sediment on this wave-exposed intertidal flat. 相似文献
95.
The Sørfjord (Western Norway) has a long history of industry and pollution, and has been monitored for several decades. The environmental monitoring has comprised analyses of different contaminants in sea water, mussel, fish, seaweed and sediments. Measurements of polychlorinated biphenyls (PCBs) in blue mussels (Mytilus edulis) some 17 years ago indicated a local source. In 2001 severe concentrations were measured in blue mussels and further investigations disclosed the primary source of PCBs in the Sørfjord. In 2002, extreme PCB-concentrations were found in cod (Gadus morhua) from the same area. However, no induction of EROD activity was detected, indicating the limitations of this assay as marker for PCB contamination. A future scientific challenge will be to understand the specific mechanisms and effects of such PCB accumulation in fish. 相似文献
96.
Indigenous Australians’ knowledge of weather and climate 总被引:1,自引:1,他引:0
Although the last 200 years of colonisation has brought radical changes in economic and governance structures for thousands
of Aboriginal and Torres Strait Islanders living in remote areas of northern Australia, many of these Indigenous people still
rely upon, and live closely connected to, their natural environment. Over millennia, living ‘on country’, many of these communities
have developed a sophisticated appreciation of their local ecosystems and the climatic patterns associated with the changes
in them. Some of this knowledge is recorded in their oral history passed down through generations, documented in seasonal
weather calendars in local languages and, to a limited degree, transcribed and translated into English. This knowledge is
still highly valued by these communities today, as it is used to direct hunting, fishing and planting as well as to inform
many seasonally dependant cultural events. In recent years, local observations have been recognised by non-Indigenous scientists
as a vital source of environmental data where few historic records exist. Similar to the way that phenological observations
in the UK and US provide baseline information on past climates, this paper suggests that Indigenous observations of seasonal
change have the potential to fill gaps in climate data for tropical northern Australia, and could also serve to inform culturally
appropriate adaptation strategies. One method of recording recent direct and indirect climate and weather observations for
the Torres Strait Islands is documented in this paper to demonstrate the currency of local observations of climate and its
variability. The paper concludes that a comprehensive, participatory programme to record Aboriginal and Torres Strait Islander
knowledge of past climate patterns, and recent observations of change, would be timely and valuable for the communities themselves,
as well as contributing to a greater understanding of regional climate change that would be useful for the wider Australian
population. 相似文献
97.
Timothy Garn David A. Green Julia M. Riley Paul Alexander 《Monthly notices of the Royal Astronomical Society》2009,397(2):1101-1112
We probe the relationship between star formation rate (SFR) and radio synchrotron luminosity in galaxies at 0 < z < 2 within the northern Spitzer Wide-area Infrared Extragalactic survey (SWIRE) fields, in order to investigate some of the assumptions that go into calculating the star formation history of the Universe from deep radio observations. We present new 610-MHz Giant Metrewave Radio Telescope (GMRT) observations of the European Large-Area ISO Survey-North 2 (ELAIS-N2) field, and using this data, along with previous GMRT surveys carried out in the ELAIS-N1 (North 1) and Lockman Hole regions, we construct a sample of galaxies which have redshift and SFR information available from the SWIRE survey. We test whether the local relationship between SFR and radio luminosity is applicable to z = 2 galaxies, and look for evolution in this relationship with both redshift and SFR in order to examine whether the physical processes which lead to synchrotron radiation have remained the same since the peak of star formation in the Universe. We find that the local calibration between radio luminosity and star formation can be successfully applied to radio-selected high-redshift, high-SFR galaxies, although we identify a small number of sources where this may not be the case; these sources show evidence for inaccurate estimations of their SFR, but there may also be some contribution from physical effects such as the recent onset of starburst activity, or suppression of the radio luminosity within these galaxies. 相似文献
98.
J.G. Blank S.J. Green D. Blake J.W. Valley N.T. Kita A. Treiman P.F. Dobson 《Planetary and Space Science》2009,57(5-6):533-540
Mars appears to have experienced little compositional differentiation of primitive lithosphere, and thus much of the surface of Mars is covered by mafic lavas. On Earth, mafic and ultramafic rocks present in ophiolites, oceanic crust and upper mantle that have been obducted onto land, are therefore good analogs for Mars. The characteristic mineralogy, aqueous geochemistry, and microbial communities of cold-water alkaline springs associated with these mafic and ultramafic rocks represent a particularly compelling analog for potential life-bearing systems. Serpentinization, the reaction of water with mafic minerals such as olivine and pyroxene, yields fluids with unusual chemistry (Mg–OH and Ca–OH waters with pH values up to ~12), as well as heat and hydrogen gas that can sustain subsurface, chemosynthetic ecosystems. The recent observation of seeps from pole-facing crater and canyon walls in the higher Martian latitudes supports the hypothesis that even present conditions might allow for a rock-hosted chemosynthetic biosphere in near-surface regions of the Martian crust. The generation of methane within a zone of active serpentinization, through either abiogenic or biogenic processes, could account for the presence of methane detected in the Martian atmosphere. For all of these reasons, studies of terrestrial alkaline springs associated with mafic and ultramafic rocks are particularly timely. This study focuses on the alkaline Adobe Springs, emanating from mafic and ultramafic rocks of the California Coast Range, where a community of novel bacteria is associated with the precipitation of Mg–Ca carbonate cements. The carbonates may serve as a biosignature that could be used in the search for evidence of life on Mars. 相似文献
99.
100.
Naomi Murdoch Patrick Michel Derek C. Richardson Kerstin Nordstrom Christian R. Berardi Simon F. Green Wolfgang Losert 《Icarus》2012,219(1):321-335
Surfaces of planets and small bodies of our Solar System are often covered by a layer of granular material that can range from a fine regolith to a gravel-like structure of varying depths. Therefore, the dynamics of granular materials are involved in many events occurring during planetary and small-body evolution thus contributing to their geological properties.We demonstrate that the new adaptation of the parallel N-body hard-sphere code pkdgrav has the capability to model accurately the key features of the collective motion of bidisperse granular materials in a dense regime as a result of shaking. As a stringent test of the numerical code we investigate the complex collective ordering and motion of granular material by direct comparison with laboratory experiments. We demonstrate that, as experimentally observed, the scale of the collective motion increases with increasing small-particle additive concentration.We then extend our investigations to assess how self-gravity and external gravity affect collective motion. In our reduced-gravity simulations both the gravitational conditions and the frequency of the vibrations roughly match the conditions on asteroids subjected to seismic shaking, though real regolith is likely to be much more heterogeneous and less ordered than in our idealised simulations. We also show that collective motion can occur in a granular material under a wide range of inter-particle gravity conditions and in the absence of an external gravitational field. These investigations demonstrate the great interest of being able to simulate conditions that are to relevant planetary science yet unreachable by Earth-based laboratory experiments. 相似文献