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71.
Alexandre Raphael Cabral Orlando Garcia Rocha Filho Richard David Jones 《Journal of Geochemical Exploration》2008,96(1):69-76
Mercury contents in Precambrian banded iron formation-hosted hematite ores are virtually unknown. In an attempt to provide information on the abundance and distribution of Hg in Fe ore, we present analyses for Hg in samples of high-grade soft hematite ore from Gongo Soco, Minas Gerais, Brazil. Bulk samples contain from < 5 to 25 ppb Hg without obvious correlation with major elements. Granulometric fractions of follow-up samples have amounts of Hg from 6 to 48 ppb and display positive linear correlations with total Mn as MnO (r = 0.87), LOI (r = 0.87) and SiO2 (r = 0.76), as well as a negative linear correlation with total Fe as Fe2O3 (r = − 0.87). The correlations suggest that Hg is associated with a hydrated ferruginous groundmass bearing residual Mn, Al and Si, which replaced gangue minerals in itabirite in the process of formation of the Gongo Soco soft hematite ore. 相似文献
72.
Measurements of NOx,y were made at Alert, Nunavut, Canada (82.5° N, 62.3° W) during surface layer ozone depletion events. In spring 1998, depletion events were rare and occurred under variable actinic flux, ice fog, and snowfall conditions. NOy changed by less than 10% between normal, partially depleted, and nearly completely depleted ozone air masses. The observation of a diurnal variation in NOx under continuous sunlight supports a source from the snowpack but with rapid conversion to nitrogen reservoirs that are primarily deposited to the surface or airborne ice crystals. It was unclear whether NOx was reduced or enhanced in different stages of the ozone depletion chemistry because of variations in solar and ambient conditions. Because ozone was depleted from 15–20 ppbv to less than 1 ppbv in just over a day in one event it is apparent that the surface source of NOx did not grossly inhibit the removal of ozone. In another case ozone was shown to be destroyed to less than the 0.5 ppbv detection limit of the instrument. However, simple model calculations show that the rate of depletion of ozone and its final steady-state abundance depend sensitively on the strength of the surface source of NOx due to competition from ozone production involving NOx and peroxy radicals. The behavior of the NO/NO2 ratio was qualitatively consistent with enhanced BrO during the period of active ozone destruction. The model is also used to emphasize that the diurnal partitioning of BrOx during ozone depletion events is sensitive to even sub ppbv variations in O3. 相似文献
73.
The origin of thermal waters from the eastern flank of the Dead Sea Rift Valley (western Jordan) 总被引:1,自引:0,他引:1
Bruno Capaccioni Orlando Vaselli Elvio Moretti Franco Tassi Roberto Franchi 《地学学报》2003,15(3):145-154
Thermal waters emerging along the eastern flank of the northernmost part of the Dead Sea Rift Valley close to the Yarmuk river are dilute, Ca–SO4–(HCO3) and Na–Cl water types with measured temperatures of 35–60 °C and estimated teperatures, according to silica solubility, of 60–110 °C. They are fed only by present‐day recharged meteoric waters (Wadi Hasa, Al Himma and North Shuna thermal baths) and by meteoric waters contaminated with saline waters (El Ma'in thermal Bath). Although they have been known for a long time, there is still dispute about their origins and the source of heat. On the basis of new chemical and isotopic analyses, the saline waters could represent residual pockets of groundwater in equilibrium with those filling the Dead Sea depression before the last retreat of Lake Lisan at 17–15 kyr bp or with the ancient seawaters of the Sedom Lagoon in the early Pleistocene, in both cases unaffected by significant evaporation processes but chemically and isotopically modified by water/rock interaction. 相似文献
74.
Factors affecting habitat occupancy of fish assemblage in the Gulf of Trieste (Northern Adriatic Sea) 总被引:3,自引:0,他引:3
Species composition, richness and abundance of the fish assemblage were studied over six different inshore macrohabitats in the southern part of the Gulf of Trieste (Northern Adriatic Sea) using the visual counts technique. Fifteen environmental variables were taken into consideration in order to determine microhabitat preferences of fish species, using canonical correspondence analysis and electivity indices. The results suggest that the structure of the fish assemblage in shallow habitats is affected by a large number of interplaying factors. Depth, type of bottom and vegetation cover – incorporating both abiotic and biotic variables – are some of the factors responsible for coastal fish distribution. Microhabitat preferences for 29 fish species are presented in the depth range from 0.5 to 3 m. 相似文献
75.
Thresholds and relations for soil‐hydraulic and soil‐physical properties as a function of burn severity 4 years after the 2011 Las Conchas Fire,New Mexico,USA
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Wildfire effects on soil‐physical and ‐hydraulic properties as a function of burn severity are poorly characterized, especially several years after wildfire. A stratified random sampling approach was used in 2015 to sample seven sites representing a spectrum of remotely sensed burn severity in the area impacted by the 2011 Las Conchas Fire in New Mexico, USA. Replicate samples from each site were analysed in the laboratory. Linear and linear indicator regression were used to assess thresholds in soil‐physical and ‐hydraulic properties and functional relations with remotely sensed burn severity. Significant thresholds were present for initial soil‐water content (θi) at 0–6 cm depth between the change in the Normalized Burn Ratio (dNBR) equal to 618–802, for bulk density (ρb) at 3–6 cm between dNBR equal to 416–533, for gravel fraction at 0–1 cm between dNBR equal to 416–533, for fines (the silt + clay fraction) at 0–1 cm for dNBR equal to 416–533, and for fines at 3–6 cm for dNBR equal to 293–416. Significant linear relations with dNBR were present between ρb at 0–1 cm, loss on ignition (LOI) at 0–1 cm, gravel fraction at 0–1 cm, and the large organic fraction at 1–3 cm. No thresholds or effects on soil‐hydraulic properties of field‐saturated hydraulic conductivity or sorptivity were observed. These results suggest that ρb and LOI at 0–1 cm have residual direct impacts from the wildfire heat impulse. The θi threshold is most likely from delayed groundcover/vegetation recovery that increases evaporation at the highest burn severity sites. Gravel and silt + clay thresholds at 0–1 cm at the transition to high burn severity suggest surface gravel lag development from hydraulic erosion. Thresholds in ρb from 3 to 6 cm and in silt + clay fraction from 3 to 6 cm appear to be the result of soil variability between sites rather than wildfire impacts. This work suggests that gravel‐rich soils may have increased resilience to sustained surface runoff generation and erosion following wildfire, with implications for assessments of postwildfire hydrologic and erosion recovery potential. 相似文献
76.
Measurements of the Henry's Law Coefficients of 2-Methyl-3-buten-2-ol, Methacrolein, and Methylvinyl Ketone 总被引:1,自引:0,他引:1
Laura T. Iraci Bradly M. Baker Geoffrey S. Tyndall John J. Orlando 《Journal of Atmospheric Chemistry》1999,33(3):321-330
Using an equilibrium headspace technique, Henry's law coefficients were measured for methacrolein (H = 6.5 ± 0.7 M atm-1) and methylvinyl ketone (41 ± 7.0 M atm-1) in water at 25 °C. In addition, 2-methyl-3-buten-2-ol was studied at 30 °C in water and in an aqueous ionic solution representative of plant tissue. Similar values were found in deionized water (65 ± 3.5 M atm-1) and in a 0.05 mol kg-1 Ca2+, K+, NO3-, SO42- solution (62 ± 0.8 M atm-1). These Henry's Law coefficients are too small to allow for significant partitioning of methacrolein, methylvinyl ketone or methylbutenol into cloud water under equilibrium conditions. 相似文献
77.
Cubellis Elena Luongo Giuseppe Obrizzo Francesco Sepe Vincenzo Tammaro Umberto 《Natural Hazards》2020,100(3):955-994
Natural Hazards - This paper analyses data regarding the seismicity and ground deformations of the island of Ischia. The goal is to describe these phenomena as a space–time process, exploring... 相似文献
78.
79.
Dissolution experiments on a serpentinite were performed at 70 °C, 0.1 MPa, in H2SO4 solution, in open and closed systems, in order to evaluate the overall dissolution rate of mineral components over different times (4, 9 and 24 h). In addition, the serpentinite powder was reacted with a NaCl-bearing aqueous solution and supercritical CO2 for 24 h at higher pressures (9-30 MPa) and temperatures (250-300 °C) either in a stirred reactor or in an externally-heated pressure vessel to assess both the dissolution rate of serpentinite minerals and the progress of the carbonation reaction. Results show that, at 0.1 MPa, MgO extraction from serpentinite ranges from 82% to 98% and dissolution rate varies from 8.5 × 10−10 mole m−2 s−1 to 4.2 × 10−9 mole m−2 s−1. Attempts to obtain carbonates from the Mg-rich solutions by increasing their pH failed since Mg- and NH4- bearing sulfates promptly precipitated. On the other hand, at higher pressures, significant crystallization (5.0-10.4 wt%) of Ca- and Fe-bearing magnesite was accomplished at 30 MPa and 300 °C using 100 g L−1 NaCl aqueous solutions. The corresponding amount of CO2 sequestered by crystallization of carbonates is 9.4-15.9 mole%. Dissolution rate (from 6.3 × 10−11 mole m−2 s−1 to 1.3 × 10−10 mole m−2 s−1) is lower than that obtained at 0.1 MPa and 70 °C but it is related to pH values much higher (3.3-4.4) than that (−0.65) calculated for the H2SO4 solution.Through a thorough review of previous experimental investigations on the dissolution kinetics of serpentine minerals the authors propose adopting: (i) the log rate [mole m−2 s−1] value of −12.08 ± 0.16 (1σ), as representative of the neutral dissolution mechanism at 25 °C and (ii) the following relationship for the acidic dissolution mechanism at 25 °C:
log rate=-0.45(±0.09)×pH-10.01(±0.30). 相似文献
80.
Nathan E. Bramall Richard Quinn Andrew Mattioda Kathryn Bryson Julie D. Chittenden Amanda Cook Cindy Taylor Giovanni Minelli Pascale Ehrenfreund Antonio J. Ricco David Squires Orlando Santos Charles Friedericks David Landis Nykola C. Jones Farid Salama Louis J. Allamandola Søren V. Hoffmann 《Planetary and Space Science》2012,60(1):121-130
The Space Environment Viability of Organics (SEVO) experiment is one of two scientific payloads aboard the triple-cube satellite Organism/ORganic Exposure to Orbital Stresses (O/OREOS). O/OREOS is the first technology demonstration mission of the NASA Astrobiology Small Payloads Program. The 1-kg, 1000-cm3 SEVO cube is investigating the chemical evolution of organic materials in interstellar space and planetary environments by exposing organic molecules under controlled conditions directly to the low-Earth orbit (LEO) particle and electromagnetic radiation environment. O/OREOS was launched on November 19, 2010 into a 650-km, 72°-inclination orbit and has a nominal operational lifetime of six months. Four classes of organic compounds, namely an amino acid, a quinone, a polycyclic aromatic hydrocarbon (PAH), and a metallo-porphyrin are being studied. Initial reaction conditions were established by hermetically sealing the thin-film organic samples in self-contained micro-environments. Chemical changes in the samples caused by direct exposure to LEO radiation and by interactions with the irradiated microenvironments are monitored in situ by ultraviolet/visible/near-infrared (UV/VIS/NIR) absorption spectroscopy using a novel compact fixed-grating CCD spectrometer with the Sun as its light source. The goals of the O/OREOS mission include: (1) demonstrating key small satellite technologies that can enable future low-cost astrobiology experiments, (2) deploying a miniature UV/VIS/NIR spectrometer suitable for in-situ astrobiology and other scientific investigations, (3) testing the capability to establish a variety of experimental reaction conditions to enable the study of astrobiological processes on small satellites, and (4) measuring the chemical evolution of organic molecules in LEO under conditions that can be extrapolated to interstellar and planetary environments. In this paper, the science and technology development of the SEVO instrument payload and its measurements are described. 相似文献