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81.
Asfaw Zegeye Cédric Carteret Martine Mullet Frédéric Jorand 《Geochimica et cosmochimica acta》2007,71(22):5450-5462
Microbiological reduction of a biogenic sulfated green rust , was examined using a sulfate reducing bacterium (Desulfovibrio alaskensis). Experiments investigated whether could serve as a sulfate source for D. alaskensis anaerobic respiration by analyzing mineral transformation. Batch experiments were conducted using lactate as the electron donor and biogenic as the electron acceptor, at circumneutral pH in unbuffered medium. transformation was monitored with time by X-ray diffraction (XRD), Transmission Mössbauer Spectroscopy (TMS), Diffuse Reflectance Infrared Fourier Transform Spectroscopy (DRIFTS), Transmission Electron Microscopy (TEM) and X-ray Photoelectron Spectroscopy (XPS). The reduction of sulfate anions and the formation of iron sulfur mineral were clearly identified by XPS analyses. TMS showed the formation of additional mineral as green rust (GR) and vivianite. XRD analyses discriminated the type of the newly formed GR as GR1. The formed GR1 was as indicated by DRIFTS analysis. Thus, the results presented in this study indicate that D. alaskensis cells were able to use as an electron acceptor. , vivianite and an iron sulfur compound were formed as a result of reduction by D. alaskensis. Hence, in environments where geochemical conditions promote biogenic formation, this mineral could stimulate the anaerobic respiration of sulfate reducing bacteria. 相似文献
82.
M. Paterne F. Guichard J.C. Duplessy G. Siani R. Sulpizio J. Labeyrie 《Journal of Volcanology and Geothermal Research》2008
A detailed tephrochronological study was undertaken in three deep-sea cores collected in the Tyrrhenian and Ionian Seas. The age and the origin of the marine tephra were inferred from oxygen isotope records of foraminifera and from major element compositions of glass-shards. Seventy-one eruptions were detected in the time interval 90,000–200,000 yrs during which the volcanoes of the Roman and Campanian regions and of the southern Italy were in activity. This is attested by the consistency of the geochemical compositions of both marine and terrestrial deposits. Most of the marine tephra consisted in trachytes and phonolites characterizing a Roman and Campanian origin. Several tephra were proposed as key-horizons for proximal and distal sediments. Among them, one tephra originating from Mount Etna (149,300 yrs) and five tephra from Pantelleria island (130,000 yrs, 163,600 yrs, 192,500 yrs, 197,400 yrs and 198,400 yrs) were northerly dispersed. Several other key horizons originated from the Campanian or Roman provinces were detected as far as 1000 km from the vents. 相似文献
83.
Links between bacterial communities in marine sediments and trace metal geochemistry as measured by in situ DET/DGT approaches 总被引:1,自引:0,他引:1
Gillan DC Baeyens W Bechara R Billon G Denis K Grosjean P Leermakers M Lesven L Pede A Sabbe K Gao Y 《Marine pollution bulletin》2012,64(2):353-362
Our current view about the relationship between metals and bacteria in marine sediments might be biased because most studies only use ex situ approaches to quantify metals. The aim of the present research was to compare ex situ and in situ methods of metal measurement (DET and DGT--diffusive equilibration or diffusive gradients in thin-films) and relate the results with two commonly used microbiological variables (bacterial biomass and bacterial diversity as revealed by DGGE). No previous studies have used such in situ approaches in microbial ecology. For biomass and most of the investigated trace metals (Ag, Cd, Sn, Cr, Ni, Cu, Pb, and Al) no significant correlations were found. The exceptions were Fe, Mn, Co, and As which behave like micronutrients. For bacterial diversity, no relevant relationships were found. We conclude that in situ methods are more adapted tools for microbial ecologists but that ex situ approaches are still necessary. 相似文献
84.
Charpy L Rodier M Fournier J Langlade MJ Gaertner-Mazouni N 《Marine pollution bulletin》2012,65(10-12):471-477
The environmental characteristics of Ahe deep lagoon (Tuamotu Archipelago, French Polynesia) were studied over 3 years with the aim of explaining the spatial and temporal variability of the natural food available for pearl oysters with a special focus on phytoplankton biomass and global photosynthesis/respiration ratio of the lagoon. Chlorophyll averaged 0.34±0.01 μg L(-1) and our findings did not confirm increased phytoplankton biomass in deep lagoonal waters. Phytoplankton production appears to be limited firstly by nitrogen and respiratory processes overpass photosynthetic processes at least in the north-eastern edge of the atoll. Grazing by pearl oysters in culture seems to decrease the POC concentration but not the phytoplankton biomass. Oysters graze mainly on non chlorophyllian particles. 相似文献
85.
(Ca x ,Sr1?x )ZrO3 and Ca(Sn y ,Zr1-y )O3 solid solutions were synthesized by solid-state reaction at high temperature before to be studied by powder X-ray diffraction and Raman Spectroscopy. Diffraction data allow the distortion of the ABO3 perovskite structure to be investigated according to cations substitution on A and B-sites. It is shown that distortion, characterized by Φ, the tilt angle of BO6 octahedra, slightly increases with decreasing y content in Ca(Sn y ,Zr1?y )O3 compounds and strongly decreases with decreasing x content in (Ca x ,Sr1?x )ZrO3 compounds. Such results are discussed in view of the relative A and B cation sizes. Raman data show that vibrational spectra are strongly affected by the cation substitution on A-site; the frequencies of most vibrational modes increase with increasing x content in (Ca x ,Sr1?x )ZrO3 compounds, i.e. with the decreasing mean size of the A-cation; the upper shift is observed for the 358 cm?1 mode (?ν/?r = ?60.1 cm?1/Å). On the other hand, the cation substitution on B-sites, slightly affect the spectra; it is shown that in most cases, the frequency of vibrational modes increases with increasing y content in Ca(Sn y ,Zr1?y )O3 compounds, i.e. with the decreasing mean size of the B-cation, but that two modes (287 and 358 cm?1) behave differently: their frequencies decrease with the decreasing mean size of the B-cation, with a shift respectively equal to +314 and +162 cm?1/Å. Such results could be used to predict the location of different elements such as trivalent cations or radwaste elements on A- or B-site, in the perovskite structure. 相似文献
86.
Ahuva Almogi-Labin Miryam Bar-Matthews Dan Shriki Elina Kolosovsky Martine Paterne Bettina Schilman Avner Ayalon Zeev Aizenshtat Alan Matthews 《Quaternary Science Reviews》2009,28(25-26):2882-2896
The influence of the northern Atlantic and tropical monsoonal systems, as recorded by the River Nile, on the climate variability of the southeastern Mediterranean was studied in two cores taken by the R/V Marion Dufresne: one core taken SE of Cyprus representing the northern Levantine Basin (core 9501, 980 m water depth) and the other located ˜380 km further south, represents the southeastern Levantine Basin in an area influenced by the River Nile plume (core 9509, 884 m water depth). The study was performed at relatively high resolution using several proxies: δ18O of Globigerinoides ruber, sediment characteristics and index colour parameters in core sections representing the last 86 ka. A low-resolution alkenone sea surface temperature record was also measured. The time frame in both cores was mostly constrained by ‘wiggle’ matching with the nearby well-dated δ18O and δ13C record of the Soreq Cave, which is mainly influenced by the eastern Mediterranean water vapor. The sedimentary record of the southern core is strongly influenced by the River Nile contribution throughout the last 86 ka, as evidenced by the higher sedimentation rates compared with the northern core (20 cm/ka vs. 5 cm/ka), continuously darker sediment colour, and higher TOC values (0.6–0.9 vs. 0.25 wt% not including sapropels). During sapropels S1 and S3, present in both cores, the influence of the River Nile became more widespread, reaching as far as Cyprus. Yet, the influence of the River Nile remained stronger in the south, as evident by the higher TOC values in the southern core throughout the entire 90 ka period and the longer duration of S1 in the southern core. An anomalous low δ18O interval that is not recorded in western Mediterranean occurred between 58 and 49 ka in the Levantine Basin and is more developed in the northern core. This period correlates with D-O interstadial 14 and maximum northern hemisphere insolation during the lastglacial cycle, suggesting that the warming mainly impacted the northern Levant.The Eastern Mediterranean Sea and land area was considerably warmer than the western Mediterranean throughout the LGM – Holocene transition, and the δ18OG. ruber drop of 4.5‰ is significantly greater than the 3‰ shift found for the western Mediterranean δ18OG. bulloides, both differences reflecting an increased continental effect from the western to eastern Mediterranean. Comparison between the marine and the land δ18O records suggests that the origin of rain over the land is composed of mixed signal from the southern and northern Levantine Basin. The study of Δδ18Osea–land variations demonstrates that various factors have influenced the sea–land relationship during the last 90 ka. The ‘amount effect’ has an important influence on rainfall δ18O during interglacial periods (particularly sapropel periods), whereas during glacial periods, increased land distances and elevation differences arising from decrease in sea level may have brought about decrease in δ18O of rainfall due to Rayleigh distillation processes. These influences were superimposed on those of sea surface water δ18O changes brought about by continental ice melting, and the strong effects felt in the southern Levantine Basin of the high River Nile input during periods of enhanced monsoonal activity. 相似文献
87.
van den Brink NW Riddle MJ van den Heuvel-Greve M van Franeker JA 《Marine pollution bulletin》2011,62(1):128-132
We demonstrate that pelagic Antarctic seabirds show significant decreases in concentrations of some persistent organic pollutants. Trends in Adélie penguins and Southern fulmars fit in a general pattern revealed by a broad literature review. Downward trends are also visible in pelagic fish, contrasting sharply with steady or increasing concentrations in Antarctic benthic organisms. Transfer of contaminants between Antarctic pelagic and benthic food webs is associated with seasonal sea-ice dynamics which may influence the balance between the final receptors of contaminants under different climatic conditions. This complicates the predictability of future trends of emerging compounds in the Antarctic ecosystem, such as of the brominated compounds that we detected in Antarctic petrels. The discrepancy in trends between pelagic and benthic organisms shows that Antarctic biota are still final receptors of globally released organic contaminants and it remains questionable whether the total environmental burden of contaminants in the Antarctic ecosystem is declining. 相似文献
88.
89.
A Compilation of Silicon and Thirty One Trace Elements Measured in the Natural River Water Reference Material SLRS-4 (NRC-CNRC) 总被引:1,自引:0,他引:1
Delphine Yeghicheyan Jean Carignan Michel Valladon Martine Bouhnik Le Coz Florence Le Cornec Maryse Castrec-Rouelle Michel Robert Luc Aquilina Emmanuel Aubry Carine Churlaud Aline Dia Samuel Deberdt Bernard Dupré Rémi Freydier Gérard Gruau Odile Hénin Anne-Marie de Kersabiec Joël Macé Luc Marin Nicole Morin Patrice Petitjean Elodie Serrat 《Geostandards and Geoanalytical Research》2001,25(2-3):465-474
The natural river water certified reference material SLRS-4 (NRC-CNRC, National Research Council-Conseil National de Recherches Canada) has been routinely analysed for major and trace elements by six French laboratories. Most measurements were made using inductively coupled plasma-mass spectrometry. For silicon and thirty one trace elements (rare earth elements, Ag, B, Br, Cs, Ga, Ge, Li, P, Pd, Rb, Se, Th, Ti, Tl, W, Y and Zr), no certified values are assigned by NRC-CNRC. We propose some compilation values and related uncertainties according to the results obtained by the different laboratories. 相似文献
90.
Summary The status of nutation theory in the computation of the Earth Rotation Parameters from the different observational techniques
is reviewed. The impact on the combined solution of the Bureau International de l'Heure is evaluated. In view of the improvement
brought by the IAU 1980 Nutation Theory, its introduction in the BIH publications, without waiting for the adoption by the
astronomical ephemerides (1984 Jan. 1) is decided. 相似文献