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991.
Tidal variability in the water quality of an urbanized estuary 总被引:1,自引:0,他引:1
J.?L.?DiLorenzoEmail author R.?J.?Filadelfo C.?R.?Surak H.?S.?Litwack V.?K.?Gunawardana T.?O.?Najarian 《Estuaries and Coasts》2004,27(5):851-860
Tide and water quality data were collected concurrently in the Hackensack River estuary (HRE), a tidal tributary of the New
York-new Jersey Harbor estuary. Harmonic analyses of tidal elevation data indicate that HRE tides are predominantly semidiurnal,
though modulated by diurnal and fortnightly components. Nearly uniform tidal ranges (averaging approximately 1.6 m) were observed
at three stations within the HRE. Periodogram estimates reveal significant tidal variability for the water quality parameter
NH4−N under dry-weather conditions. Lag correlation analyses associate NH4−N concentration variations with water level fluctuations. Longitudinal profile plots for NH4−N reveal a consistent pattern of tidal translations, with peak concentrations oscillating about a major wastewater discharger.
These analyses suggest that the distribution of NH4−N concentrations in the HRE is controlled primarily by major point source loadings and horizontal advection. A simplified,
one-dimensional model is used to describe this distribution. Effects of tidal variability in masking water quality status
and waak trends are also analyzed. These analyses highlight the potential importance of short-term water quality variability
in tidal estuaries where concentration gradients are large. 相似文献
992.
A. Horneman A. van Geen P.E. Mathe R.K. Dhar M.A. Hoque M. Shamsudduha K.M. Ahmed 《Geochimica et cosmochimica acta》2004,68(17):3459-3473
This study reexamines the notion that extensive As mobilization in anoxic groundwater of Bangladesh is intimately linked to the dissolution of Fe oxyhydroxides on the basis of analyses performed on a suite of freshly collected samples of aquifer material. Detailed sediment profiles extending to 40 to 70 m depth below the surface were obtained at six sites where local groundwater As concentrations were known to span a wide range. The sediment properties that were measured include (1) the proportion of Fe(II) in the Fe fraction leached in hot 1.2 N HCl, (2) diffuse spectral reflectance, and (3) magnetic susceptibility.In parallel with local concentrations of dissolved As ranging from <5 to 600 μg/L, Fe(II)/Fe ratios in shallow (gray) Holocene sands tended to gradually increase with depth from values of 0.3 to 0.5 to up to 0.9. In deeper (orange) aquifers of presumed Pleistocene age that were separated from shallow sands by a clay layer and contained <5 μg/L dissolved As, leachable Fe(II)/Fe ratios averaged ∼0.2. There was no consistent relation between sediment Fe(II)/Fe and dissolved Fe concentrations in groundwater in nearby wells. The reflectance measurements indicate a systematic linear relation (R2 of 0.66; n = 151) between the first derivative transform of the reflectance at 520 nm and Fe(II)/Fe. The magnetic susceptibility of the shallow aquifer sands ranged from 200 to 3600 (x 10−9 m3/kg SI) and was linearly related (R2 of 0.75; n = 29) to the concentrations of minerals that could be magnetically separated (0.03 to 0.79% dry weight). No systematic depth trends in magnetic susceptibility were observed within the shallow sands, although the susceptibility of deeper low-As aquifers was low (up to ∼200 × 10−9 m3/kg SI).This set of observations, complemented by incubation results described in a companion paper by van Geen et al. (this volume), suggests that the release of As is linked to the transformation of predominantly Fe (III) oxyhydroxide coatings on sand particles to Fe(II) or mixed Fe(II/III) solid phases with a flatter reflectance spectrum such as siderite, vivianite, or magnetite, without necessarily resulting in the release of Fe to groundwater. The very low As/Fe ratio of magnetically separated minerals compared to the As/Fe of bulk acid leachate (2 vs. 40 10−6, respectively) suggests that such a transformation could be accompanied by a significant redistribution of As to a mobilizable phase on the surface of aquifer particles. 相似文献
993.
P. Ma K. Aggrey C. Tonzola C. Schnabel P. de Nicola J.T. Wasson L. Brown R. Middleton 《Geochimica et cosmochimica acta》2004,68(19):3883-3896
By using accelerator mass spectrometry we have measured the 10Be concentrations of 86 Australasian tektites. Corrected to the time of tektite production ∼0.8 My ago, the 10Be concentrations (106 atom/g) range from 59 for a layered tektite from Huai Sai, Thailand, to 280 for an australite from New South Wales, Australia. The average value is 143 ± 50. When tektites are sorted by country, their average measured 10Be concentrations increase slowly with increasing distance from Southeast Asia, the probable location of the tektite producing event, from 59 ± 9 for 6 layered tektites from Laos to 136 ± 20 for 20 splash-form tektites from Australia. The lowest 10Be concentrations for tektites fall on or within a contour centered off the shore of Vietnam, south of the Gulf of Tonkin (107°E; 17°N), but also encompassing two other locations in the area of northeastern Thailand previously proposed for the site of a single tektite-producing impact. The 10Be concentrations of layered tektites show only a weak anticorrelation (R ∼ −0.3) with the numbers of relict crystalline inclusions.Loosely consolidated, fine-grained terrestrial sediments or recently consolidated sedimentary rocks are the most likely precursor materials. Dilution of sediments with other kinds of rock raises problems in mixing and is not supported by petrographic data. Sedimentary columns that have the right range of 10Be concentrations occur off the coasts of places where sedimentation rates are high relative to those in the deep sea. A single impact into such a region, 15 to 300 m thick, could have propelled near-surface, high-10Be material farthest—to Australia—while keeping the deeper-lying, low-10Be layers closer to home. We do not rule out, however, other proposed mechanisms for tektite formation. 相似文献
994.
S.?PetitEmail author A.?Decarreau F.?Martin R.?Buchet 《Physics and Chemistry of Minerals》2004,31(9):585-592
The aim of this paper is to determine a relationship between the wavenumbers of the first OH-stretching overtones (W2OH) and the wavenumbers of the OH-stretching fundamentals (WOH) to help to interpret the near-infrared (NIR) spectra. The first overtone (2OH) bands appear at wavenumbers less than twice those of the fundamental bands (OH), due to the anharmonic character of vibrations, X = W2OH/2 - WOH, with X being the anharmonicity constant. Talc samples with various crystal chemistries are used to solve the equation and the experimental data are well fitted with X = –85.6 cm–1. As far as the authors are aware, it is the first time that the anharmonicity constant for the OH-stretching vibrations is determined for phyllosilicates. The anharmonicity constant remains almost unchanged for several types of clay samples. Therefore the relation, established from talc samples because their absorption bands are narrow and their wavenumber range of OH vibrations is wide, can be used for any other clay minerals. 相似文献
995.
Lake Balboa is a deep sinkhole lake in south Georgia. Subbottom acoustic profiling and long sediment cores reveal four stratigraphic units within >20 m of lacustrine fill above acoustically stratified and faulted Miocene/Pliocene overburden and basement Eocene limestone which hosts the Floridan Aquifer system (FAS). Fill consists of thin, rhythmically bedded, peaty sediments (Unit I), indicative of slow sedimentation in a shallow swamp until 13,110–12,680 cal BP, a mix of desiccated and over-consolidated clay and silty sand (Unit II) implying periodic subaerial exposure of the lake bed until 9470–9025 cal BP, and gyttja associated with a rapid 8 m rise in water level by 9120–9020 cal BP (Unit III), as well as an additional rise of 10 m to modern lake levels (Unit IV). Accumulation of nearly 4.5 m of low permeability gyttja, and higher lake levels have fundamentally changed exchange between surface water and groundwater, reducing by 40% or more the rate of vertical leakage to the FAS and increasing shallow aquifer discharge to the lake. 相似文献
996.
Using density functional theory, we perform ab initio calculations of the behaviour of calaverite, AuTe2, at high pressures. Calaverite has a distorted CdI2 structure, that presents a pronounced two-dimensional character and a rather anisotropic response to pressure. Increasing the pressure, we predict an isosymmetrical phase transition between 55 and 60 GPa, that is accompanied by an important distortion of the structure, observed in all its geometrical parameters, especially the c lattice parameter. Relaxing the pressure, the reverse phase transition is observed between 30 and 25 GPa. 相似文献
997.
Alessandro Beghini Zdeněk P. Bažant R. Chambon D. Kolymbas I. Herle 《国际地质力学数值与分析法杂志》2004,28(4):365-372
998.
A microearthquake survey in the Sikkim Himalaya raised a question whether the north–south segment of the Main Central Thrust (MCT) in this part of the Himalaya is seismically active(?). Fault-plane solution of a cluster of events occurred below this segment of the MCT shows right-lateral strike-slip motion. The seismic observations and the geological evidences suggest that a NNE–SSW trending strike-slip fault, beneath this segment, caused right lateral movement on the MCT, and is seismically active. 相似文献
999.
B.R. Goleby R.S. Blewett R.J. Korsch D.C. Champion K.F. Cassidy L.E.A. Jones P.B. Groenewald P. Henson 《Tectonophysics》2004,388(1-4):119
Deep seismic reflection data across the Archaean Eastern Goldfields Province, northeastern Yilgarn Craton, Western Australia, have provided information on its crustal architecture and on several of its highly mineralised belts. The seismic reflection data allow interpretation of several prominent crustal scale features, including an eastward thickening of the crust, subdivision of the crust into three broad layers, the presence of a prominent east dip to the majority of the reflections and the interpretation of three east-dipping crustal-penetrating shear zones. These east-dipping shear zones are major structures that subdivide the region into four terranes. Major orogenic gold deposits in the Eastern Goldfields Province are spatially associated with these major structures. The Laverton Tectonic Zone, for example, is a highly mineralised corridor that contains several world-class gold deposits plus many smaller deposits. Other non crustal-penetrating structures within the area do not appear to be as well endowed metallogenically as the Laverton structure. The seismic reflection data have also imaged a series of low-angle shear zones within and beneath the granite–greenstone terranes. Where the low-angle shear zones intersect the major crustal-penetrating structures, a wedge shaped geometry is formed. This geometry forms a suitable fluid focusing wedge in which upward to subhorizontal moving fluids are focused and then distributed into the nearby complexly deformed greenstones. 相似文献
1000.
Shear deformation of hot pressed plagioclase–olivine aggregates was studied in the presence and absence of mineral reaction. Experiments were performed at 900 °C, 1500 MPa, and a constant shear strain rate of 5×10−5 s−1 in a solid medium apparatus. Whether the mineral reaction between plagioclase and olivine takes place or not is controlled by choosing the appropriate plagioclase composition; labradorite (An60) does not react, anorthite (An92) does. Labradorite–olivine aggregates deformed without reaction are very strong and show strain hardening throughout the experiment. Syndeformational reaction between olivine and anorthite causes a pronounced strain weakening. The reaction produces fine-grained opx–cpx–spinel aggregates, which accommodate a large fraction of the finite strain. Deformation and reaction are localised within a 0.5-mm-wide sample. Three representative samples were analysed for their fabric anisotropy R* and shape-preferred orientation α* (fabric angle with the shear plane) using the autocorrelation function (ACF). Fabric anisotropy can be calibrated to quantify strain variations across the sheared samples. In the deformed and reacted anorthite–olivine aggregate, there is a strong correlation between reaction progress and strain; regions of large shear strain correspond to regions of maximum reaction progress. Within the sample, the derived strain rate variations range up to almost one order of magnitude. 相似文献