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31.
J.Michael Moldowan Wolfgang K. Seifert Edward Arnold Jon Clardy 《Geochimica et cosmochimica acta》1984,48(8):1651-1661
Two C28H48-pentacyclic triterpanes were isolated from Monterey shale. X-ray crystallography of a crystal containing both compounds proved their structures as 17β,18α,21α(H)-28,30-bisnorhopane and 17β,18α,21β(H)-28,30-bisnorhopane. Several differences are found between 28,30-bisnorhopanes and the regular hopanes. Unlike the regular hopane epimers, for practical purposes the three epimeric 28,30-bisnorhopanes [17α,21β(H)-, 17β,21α(H)-, and 17β,21β(H)-]cannot be distinguished by their mass spectra. Special conditions are needed to separate them by gas chromatography. The diagenetically first-formed epimer is thought to be 17α,21β(H)- because it predominates in immature shales. The order of thermodynamic stability is 17β,2lα(H) < > 17α,21β(H) > 17β,21β(H), and all three epimers are present in petroleum. 25,28,30-Trisnorhopanes can be analyzed in similar fashion and are found to have similar thermodynamic characteristics. The percent of the ring D/E cis epimer of 28,30-bisnorhopane and/or 25,28,30-trisnorhopane is a useful maturation parameter similar to the 20S/20R sterane ratio. Evidence indicates 25-demethylation of 28,30-bisnorhopane to 25,28,30-trisnorhopane during advanced stages of biodegradation. Hence, percent ring cis 25,28,30-trisnorhopane has an application to maturation assessment in heavily biodegraded oils. 相似文献
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33.
Matthew J. Genge Luke Alesbrook Natasha V. Almeida Helena C. Bates Phil A. Bland Mark R. Boyd Mark J. Burchell Gareth S. Collins Luke T. Cornwell Luke Daly Hadrien A. R. Devillepoix Matthias van Ginneken Ansgar Greshake Daniel Hallatt Christopher Hamann Lutz Hecht Laura E. Jenkins Diane Johnson Rosie Jones Ashley J. King Haithem Mansour Sarah McMullan Jennifer T. Mitchell Gavyn Rollinson Sara S. Russell Christian Schröder Natasha R. Stephen Martin D. Suttle Jon D. Tandy Patrick Trimby Eleanor K. Sansom Vassilia Spathis Francesca M. Willcocks Penelope J. Wozniakiewicz 《Meteoritics & planetary science》2024,59(5):948-972
Fusion crusts form during the atmospheric entry heating of meteorites and preserve a record of the conditions that occurred during deceleration in the atmosphere. The fusion crust of the Winchcombe meteorite closely resembles that of other stony meteorites, and in particular CM2 chondrites, since it is dominated by olivine phenocrysts set in a glassy mesostasis with magnetite, and is highly vesicular. Dehydration cracks are unusually abundant in Winchcombe. Failure of this weak layer is an additional ablation mechanism to produce large numbers of particles during deceleration, consistent with the observation of pulses of plasma in videos of the Winchcombe fireball. Calving events might provide an observable phenomenon related to meteorites that are particularly susceptible to dehydration. Oscillatory zoning is observed within olivine phenocrysts in the fusion crust, in contrast to other meteorites, perhaps owing to temperature fluctuations resulting from calving events. Magnetite monolayers are found in the crust, and have also not been previously reported, and form discontinuous strata. These features grade into magnetite rims formed on the external surface of the crust and suggest the trapping of surface magnetite by collapse of melt. Magnetite monolayers may be a feature of meteorites that undergo significant degassing. Silicate warts with dendritic textures were observed and are suggested to be droplets ablated from another stone in the shower. They, therefore, represent the first evidence for intershower transfer of ablation materials and are consistent with the other evidence in the Winchcombe meteorite for unusually intense gas loss and ablation, despite its low entry velocity. 相似文献
34.
Various approaches have been used to establish marine protected areas (MPAs) in different countries. In this paper we compare and review three processes to establish MPAs within the United States and Australia. These two countries share many similarities in their cultures, but their approaches to managing marine resources differ considerably. Each of these efforts to establish or review MPAs was motivated by concern about declines of targeted marine species or habitats. However, the government actions varied because of differences in governance, planning process including public input, and the role of science. Comparing these processes highlights effective approaches for protecting marine ecosystems and gaining public support. 相似文献
35.
New Pb-, Sr-, and Nd-isotopic data have been obtained for the rocks of volcanoes overlying a wide range of depths (100–580 km) to the Wadati-Benioff Zone (WBZ) in the New Britain island arc, Papua New Guinea. Well-defined trends consistent with two-component mixing are observed in combined Pb-isotope/trace-element plots. One of the components is believed to represent a slab contribution whose isotopic signature, unlike those noted for several other arcs, appears to be dominated by subducted, altered, oceanic crust rather than by sediment. This conclusion is consistent with the results of a recent Be–B study of New Britain rocks. The influence of the slab component is considered to decrease as depth to the WBZ increases. Higher abundances of high-field-strength elements correlate with increasing depths to the WBZ, and may be indicative of smaller degrees of partial melting of the mantle wedge as WBZ depths increase. Abundances of other incompatible elements appear to reflect a complex interplay between the slab-derived flux and melting process. 相似文献
36.
Abstract. This report summarizes results of monitoring programs for volatile synthetic organic chemicals (VOCs) in Nebraska's private and public water-supply wells conducted by two State agencies. Of 97 community water-supply systems sampled as of June 1984, 16.5 percent (16 systems) showed quantifiable levels of at least one VOC. Detectable amounts of one or more VOCs were measured in samples from 15.9 percent (10) of 63 private wells sampled in 1982. These percentages are consistent with results of other State and national surveys. 相似文献
37.
Jon D. Woodhead Russell S. Harmon Donald G. Fraser 《Earth and Planetary Science Letters》1987,83(1-4)
Quaternary lavas from the Northern Mariana Islands have respective O- and S-isotope ranges ofδ18O = +5.7 to +6.6 (‰ SMOW) andδ34S = +2.0to+20.7 (‰ CDT). Chemically evolved andesites and dacites with meanδ18O = +6.3 ± 0.2 are slightly enriched in18O with respect to unfractionated basalts of<53%SiO2 with meanδ18O = +6.0 ± 0.1. This18O enrichment can be explained in terms of differentiation of parental mafic magmas havingδ18O values between +5.7 to +6.2‰ through closed-system crystal fractionation because the lavas from all nine islands of the arc define a coherentδ18OSiO2 trend. The S-isotope composition of oxidized magmas is not modified extensively through the degassing of SO2; therefore, the meanδ34S value of ca. +11‰ for the Mariana lavas is considered to be representative of their source region.The enrichment of18O and34S in Mariana Arc parental magmas relative to ocean floor basalts withδ18O ca. + 5.7‰ andδ34S = ca.0.3‰ is attributed to the recycling of18O- and34S-rich crustal components (sediment withδ18O = ca. + 25‰ and seawater sulfate withδ34S = ca. +20‰ into the upper mantle source region for these arc magmas. This interpretation is consistent with enrichments of radiogenic Sr and Pb in the same lavas relative to ocean-floor basalts erupted either side of the arc, which are presumed to share a common upper mantle source. This enrichment is considered to reflect the mixing of two components, one having a typical upper mantle composition and the other having a more radiogenic character similar to that of western Pacific pelagic sediments. 相似文献
38.
Mineral-scale Sr-isotope constraints on magma evolution and chamber dynamics in the Rum layered intrusion,Scotland 总被引:1,自引:0,他引:1
Frank?J.?TepleyIIIEmail author Jon?P.?Davidson 《Contributions to Mineralogy and Petrology》2003,145(5):628-641
Sr isotopic zoning within single plagioclase crystals from rocks from Unit 9 of the Rum layered intrusion is used to infer events during crystal growth in a magma undergoing contamination. The 87Sr/86Sr diversity among minerals and between cores and rims of plagioclase crystals increases as the boundary between unit 9 and the overlying Unit 10 peridotite is approached. Models of near-solidus interaction of the cumulate with a fluid or melt, or large scale textural re-equilibration, cannot easily account for the systematic differences in 87Sr/86Sr between small crystals and the rims of larger crystals.We propose a simple interpretation in which crystal growth is concentrated along the cool margins of the reservoir. Crystals are subsequently advected to a site of accumulation at the base of the reservoir, probably by episodic plume-like dense downwellings allowing mixing of isotopically zoned and unzoned crystals.If the core-rim isotope variations are inherited from primary magmatic growth, then the small distances over which they are now preserved (1–2 mm) place constraints on the minimum cooling rate of the intrusion. Although the length scale of diffusive equilibration is influenced by a number of poorly-constrained variables (starting temperature, feldspar composition, temperature-time path) cooling was clearly very rapid with cooling to effective closure (~1,000 °C) within a few thousand years.Editorial responsibility: I. Parsons 相似文献
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40.
An apparatus is described which permits precise, versatile control of simulated tidal flux in laboratory microcosms. A key component of the system, a programmable electronic control unit, can closely imitate any natural tidal function and is readily adaptable to other experimental applications that utilize timed switching capability. The programmable control unit is also cheaper and easier to operate than computer-based systems. 相似文献