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131.
Saioa Suárez Hazel M. Prichard Francisco Velasco Peter C. Fisher Iain McDonald 《Mineralium Deposita》2010,45(4):331-350
The distribution, mineralogy and mobility of the platinum-group elements (PGE) in the surface environment are poorly understood.
This study of the lower, less altered and upper, more altered gossan, overlying the Aguablanca Ni–Cu-(PGE) magmatic deposit
(Spain), has shown that the platinum-group minerals (PGM) are progressively oxidised and dispersed into iron oxides that form
the gossan. A combination of the characterization of PGE in host PGM, using a scanning electron microscope, and measurement
of PGE at lower concentrations in host iron oxides, using laser ablation-inductively coupled plasma-mass spectrometry (LA-ICP-MS),
has for the first time allowed the total distribution of the PGE within a gossan to be documented. This study has revealed
a complete in situ alteration and dispersion sequence of the PGM including (1) breakdown of both the more stable Pt-arsenides,
Pt/Pd-tellurides and the less stable bismuthotellurides, (2) formation of partially oxidised PGM, (3) development of a wide
range of oxidised Pt- and Pd-bearing phases, (4) subsequent formation of Fe–PGE-oxides and PGE-hydroxides, (5) incorporation
of PGE into ferruginous supergene products and lastly (6) concentration of PGE at the edges of veins and iron oxides. Dispersion
of Pd is greater than for the other PGE with Pd being widely distributed throughout the iron oxides. This oxidising environment
produced PGE-oxides rather than PGE-alloys, also commonly found in the surface environment, especially in placers. These results
provide critical evidence for the stages of mineralogical change from PGE host mineralogy in magmatic ores to surface weathering
producing PGE-oxides. 相似文献
132.
William R. Hyde Adam A. Garde Nynke Keulen Sebastian N. Malkki Steven J. Jaret Tod Waight Pierre Beck Iain McDonald Nicolaj K. Larsen 《Meteoritics & planetary science》2023,58(6):789-814
Impact melt rocks formed during hypervelocity impact events are ideal for studying impact structures. Here, we describe impact melt rock samples collected proximal to the 31 km wide 58 Ma Hiawatha impact structure, northwest Greenland, which is completely covered by the Greenland Ice Sheet. The melt rocks contain diagnostic shock indicators (e.g., planar deformation features [PDF] in quartz and shocked zircon) and form three groups based on melt textures and chemistry: (i) hypocrystalline, (ii) glassy, and (iii) carbonate-based melt rocks. The exposed foreland directly in front of the structure consists of metasedimentary successions and igneous plutons; however, the carbonate-based impactites indicate a mixed target sequence with a significant carbonate-rich component. Well-preserved organic material in some melt rocks indicates that North Greenland at the time of impact was host to abundant organic material, likely a dense high-latitude temperate forest. Geochemical signatures of platinum-group elements in selected samples indicate an extraterrestrial component and support previous identification of a highly fractionated iron impactor in glaciofluvial sand. Our results illustrate the possibility to study impact structures hidden beneath a thick ice sheet based on transported samples and this opens a new avenue for identifying other potential impact craters in Greenland and Antarctica. 相似文献