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151.
Christine Baus HsuWen Hung Frank Sacher Michael Fleig Heinz‐Jürgen Brauch 《洁净——土壤、空气、水》2005,33(2):118-132
In Germany, the gasoline additive methyl tert‐butyl ether (MTBE) is almost constantly detected in measurable concentrations in surface waters and is not significantly removed during riverbank filtration. The removal of MTBE from water has been the focus of many studies that mostly were performed at high concentration levels and centred in understanding the mechanisms of elimination. In order to assess the performance of conventional and advanced water treatment technologies for MTBE removal in the low concentration range further studies were undertaken. Laboratory experiments included aeration, granulated activated carbon (GAC) adsorption, ozonation and advanced oxidation processes (AOP). The results show that the removal of MTBE by conventional technologies is not easily achieved. MTBE is only removed by aeration at high expense. Ozonation at neutral pH values did not prove to be effective in eliminating MTBE at all. The use of ozone/H2O2 (AOP) may lead to a partly elimination of MTBE. However, the ozone/H2O2 concentrations required for a complete removal of MTBE from natural waters is much higher than the ozone levels applied nowadays in waterworks. MTBE is only poorly adsorbed on activated carbon, thus GAC filtration is not efficient in eliminating MTBE. A comparison with real‐life data from German waterworks reveals that if MTBE is detected in the raw water it is most often found in the corresponding drinking water as well due to the poor removal efficiency of conventional treatment steps. 相似文献
152.
A high resolution (3–8 km grid), 3D numerical ocean model of the West Caribbean Sea (WCS) is used to investigate the variability
and the forcing of flows near the Meso-American Barrier Reef System (MBRS) which runs along the coasts of Mexico, Belize,
Guatemala and Honduras. Mesoscale variations in velocity and temperature along the reef were found in seasonal model simulations
and in observations; these variations are associated with meandering of the Caribbean current (CC) and the propagation of
Caribbean eddies. Diagnostic calculations and a simple assimilation technique are combined to infer the dynamically adjusted
flow associated with particular eddies. The results demonstrate that when a cyclonic eddy (negative sea surface height anomaly
(SSHA)) is found near the MBRS the CC shifts offshore, the cyclonic circulation in the Gulf of Honduras (GOH) intensifies,
and a strong southward flow results along the reef. However, when an anticyclonic eddy (positive SSHA) is found near the reef,
the CC moves onshore and the flow is predominantly westward across the reef. The model results help to explain how drifters
are able to propagate in a direction opposite to the mean circulation when eddies cause a reversal of the coastal circulation.
The effect of including the Meso-American Lagoon west of the Belize Reef in the model topography was also investigated, to
show the importance of having accurate coastal topography in determining the variations of transports across the MBRS. The
variations found in transports across the MBRS (on seasonal and mesoscale time scales) may have important consequences for
biological activities along the reef such as spawning aggregations; better understanding the nature of these variations will
help ongoing efforts in coral reef conservation and maintaining the health of the ecosystem in the region. 相似文献
153.
Global ocean circulation models usually lack an adequate consideration of high-latitude processes due to a limited model domain
or insufficient resolution. Without the processes in key areas of the global thermohaline circulation, the characteristics
and flow of deep and bottom waters cannot be modeled realistically. In this study, a high-resolution (~20 km) ocean model
focused on the Weddell Sea sector of the Southern Ocean is combined with a low-resolution (2° × 2°) global ocean model applying the state estimation technique. Temperature, salinity, and velocity data on two Weddell Sea
sections from the regional model are used as constraints for the large-scale model in addition to satellite altimetry and
sea-surface temperatures. The differences between the model with additional constraints and without document that the Weddell
Sea circulation exerts significant influence on the course of the Antarctic Circumpolar Current with consequences for Southern
Ocean water mass characteristics and the spreading of deep and bottom waters in the South Atlantic. Furthermore, a warming
trend in the period 1993–2001 was found in the Weddell Sea and adjacent basins in agreement with float measurements in the
upper Southern Ocean. Teleconnections to the North Atlantic are suggested but need further studies to demonstrate their statistical
significance. 相似文献
154.
M. Roy-Barman C. Jeandel M. Souhaut M. Rutgers van der Loeff I. Voege N. Leblond R. Freydier 《Earth and Planetary Science Letters》2005,240(3-4):681-693
230Th, 232Th and 234Th were analyzed in sinking particles collected by moored and drifting sediment traps in the NE Atlantic Ocean (POMME experiment) in order to constrain the phase(s) carrying Th isotopes in the water column. It reveals a contrasted behaviour between 234Th and 230Th. 234Th is correlated to the particulate organic carbon suggesting that it is primarily scavenged by organic compounds in the surface waters. 230Thxs is correlated with Mn, Ba and the lithogenic fraction that are enriched in small suspended particles and incorporated in the sinking particulate flux throughout the water column. The lack of correlation between 230Thxs and CaCO3 or biogenic silica (bSi) indicates that CaCO3 and bSi are not responsible for 230Th scavenging in the deep waters of this oceanic region. 230Th is generally correlated with the lithogenic content of the trapped material but this correlation disappears in winter during strong atmospheric dust inputs suggesting that lithogenic matter is not directly responsible for 230Th scavenging in the deep waters or that sufficient time is required to achieve particle–solution equilibration. MnO2 could be the prevalent 230Thxs-bearing phase. The narrow range of Kd_MnO2Th obtained for very contrasted oceanic environments supports a global control of 230Thxs scavenging by MnO2 and raises the possibility that the 230Th–231Pa fractionation is controlled by the amount of colloidal MnO2 in seawater. 相似文献
155.
156.
Relief-rejuvenation and topographic length scales in a fluvial drainage basin, Napf area, Central Switzerland 总被引:2,自引:2,他引:2
This paper explores how, and to what extent, a phase of relief-rejuvenation modifies the mode of surface erosion in an approximately 63 km2 drainage basin located at the northern border of the Swiss Alps (Luzern area). In the study area, the retreat of the Alpine glaciers at the end of the Last Glacial Maximum (LGM) caused base level to lower by approximately 80 m. The fluvial system adapted to the lowered base level by headward erosion. This is indicated by knickzones in the longitudinal stream profiles and by the continuous upstream narrowing of the width of the valley floor towards these knickzones. In the headwaters above these knickzones, processes are still to a significant extent controlled by the higher base level of the LGM. There, frequent exposure of bedrock in channels and especially on hillslopes implies that sediment flux is to a large extent limited by weathering rates. In the knickzones, however, exposure of bedrock in channels implies that sediment flux is supply-limited, and that erosion rates are controlled by stream power.The morphometric analysis reveals the existence of length scales in the topography that result from distinct geomorphic processes. Along the tributaries where the upstream sizes of the drainage basins exceed 100,000–200,000 m2, the mode of sediment transport and erosion changes from predominantly hillslope processes (i.e., landsliding, creep of regolith, rock avalanches and to some extent debris flows) to processes in channels (fluvial processes and debris flows). This length scale reflects the minimum size of the contributing area for channelized processes to take over in the geomorphic development (i.e., threshold size of drainage basin). This threshold size depends on the ratio between production rates of sediment on hillslopes, and export rates of sediment by processes in channels. Consequently, in the headwaters, erosion rates and sediment flux, and hence landscape evolution rates, are to a large extent limited by weathering processes. In contrast, in the lower portion of the drainage basin that adjusts to the lowered base-level, rates of channelized erosion and relief formation are controlled mainly by stream power. Hence, this paper shows that base-level lowering, headward erosion and establishment of knickzones separate drainage basins in two segments with different controls on rates of surface erosion, sediment flux and relief formation. 相似文献
157.
The Wilhelmine Alpe section near Immenstadt (Allgäu, south Germany), which represents one of the best continuously exposed outcrops within the northern Alpine foreland basin, has been analyzed for magnetostratigraphic and palynostratigraphic signals. The section comprises the marine-to-terrestrial transition from Lower Marine (UMM) to Lower Freshwater Molasse (USM) sediments. Based on the correlation of the local magnetic pattern with the geomagnetic polarity timescale (GPTS) and palynostratigraphic data, an age of about 31 Ma is suggested for the UMM–USM transition in the Wilhelmine Alpe section. A comparison with coeval magnetostratigraphic sections from central and eastern Switzerland indicates that the regression of the UMM sea along the southern margin of the Molasse basin occurred strongly heterochronously between 31.5 and 30 Ma. The heterochroneity is attributed to the deposition of fan-delta and alluvial fan sediments which document that the overall marine conditions during the UMM were accompanied by strong clastic input derived from the rising Alps. This clastic contribution had a much stronger influence on the depositional pattern than previously thought. 相似文献
158.
159.
A. Demoulin J. Campbell A. De. Wulf A. Muls R. Arnould B. Görres D. Fischer T. Kötter M. Brondeel D. Van. Damme J. M. Jacqmotte 《International Journal of Earth Sciences》2005,94(4):515-524
We present the HARD project of GPS monitoring of vertical ground motion in NE Ardenne and Eifel (western Europe). Its main purposes are to get a better insight into the present-day rates of vertical ground motion in intraplate settings and to identify the various causes of these motions. Since 1999, we have carried out yearly campaigns of simultaneous GPS measurements at 12 sites situated so as to sample the different tectonic subunits of the study area and especially to record potential displacements across the seismogenic Hockai fault zone. Five campaigns (1999–2003) have been processed currently. Key issues of the data processing with the Gamit software are discussed and first results are presented. Though temporally consistent in many cases, the obtained vertical motion rates are spatially highly variable. They are also much too high (several mm/year) to support a tectonic interpretation, and a long-term influence of groundwater level variations is proposed to account for the observed motions. This influence should be distinguished from seasonal variations and from inter-survey variations linked to the varying degree of soil and subsoil drying off during the successive spring surveys. 相似文献
160.
Mariëtte Wolthers Laurent Charlet Peter R. van der Linde 《Geochimica et cosmochimica acta》2005,69(14):3483-3492
Arsenate, As(V), sorption onto synthetic iron(II) monosulfide, disordered mackinawite (FeS), is fast. As(V) sorption decreases above the point of zero surface charge of FeS and follows the pH-dependent concentration of positively charged surface species. No redox reaction is observed between the As(V) ions and the mineral surface over the time span of the experiments. This observation shows that As(V) dominantly forms an outer-sphere complex at the surface of mackinawite. Arsenite, As(III), sorption is not strongly pH-dependent and can be expressed by a Freundlich isotherm. Sorption is fast, although slower than that of As(V). As(III) also forms an outer-sphere complex at the surface of mackinawite. In agreement with previous spectroscopic studies, complexation at low As(V) and As(III) concentration occurs preferentially at the mono-coordinated sulfide edge sites. The Kd (L g−1) values obtained from linear fits to the isotherm data are ∼9 for As(V) and ∼2 for As(III). Stronger sorption of As(V) than As(III), and thus a higher As(III) mobility, may be reflected in natural anoxic sulfidic waters when disordered mackinawite controls arsenic mobility. 相似文献