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101.
The redox state of subduction zones: insights from arc-peridotites 总被引:23,自引:0,他引:23
Spinel peridotites from a variety of island arcs have been utilised to calculate the redox state of the mantle wedge above subduction zones. Oxygen fugacities (fO2 values) calculated from the ferric iron content of spinels, measured by Electron Microprobe (EMP) using secondary standards [Wood, B.J., Virgo, D., 1989. Upper mantle oxidation state: ferric iron contents of lherzolite spinels by 57Fe Mössbauer spectroscopy and resultant oxygen fugacities. Geochim. Cosmochim. Acta, 53, 1277–1291.], yield values which range from 0.3 to 2.0 above the fayalite–magnetite–quartz (FMQ) buffer. These data provide further evidence that the mantle wedge is ubiquitously oxidised relative to oceanic and ancient cratonic mantle. There is no correlation between fO2 values and the presence of hydrous phases and, in fact, the most oxidised samples contain no hydrous phases. Within individual suites there is no correlation between fO2 and degree of depletion as indicated by spinel Cr#, except for a suite of reacted forearc-peridotites. However, when the data is viewed as a whole there is broad a positive correlation between fO2 and spinel Cr# suggesting that partial melting processes may influence the redox state of the mantle wedge. We suggest that the ultimate source of the oxygen which oxidises the mantle wedge is from the subducted slab. It is not clear whether this oxidising agent is a solute-rich hydrous fluid or a water-bearing silicate melt. However, our data does indicate that silicate melts are effective oxidisers of the depleted shallow upper mantle. Simple mass balance calculations based on the ferric iron content of primitive subduction zone magmas indicates that the source region must contain 0.6–1.0 wt.% Fe2O3. This amount of Fe2O3 in a fertile spinel peridotite yields an oxygen fugacity of 0.5–1.7 log units above FMQ in the IAB source. If water is the sole oxidising agent in the mantle wedge then 0.030–0.075 wt.% H2O is required which is considerably less than the 0.25% H2O envisaged by Stolper and Newman [Stolper, E.M., Newman, S., 1994. The role of water in the petrogenesis of Mariana trough magmas. Earth Planet. Sci. Lett., 121, 293–325.], suggesting water is not necessarily an efficient oxidising agent. Alternatively, ferric iron may be added to the mantle wedge by addition of a ferric iron-rich sediment melt or more likely as a solute-rich hydrous fluid. This model would produce spinel, orthopyroxene or amphibole in the wedge with only a slight increase in fO2 of the source region. Although it is unclear which model is correct the maximum fO2 of the fertile mantle wedge is unlikely to be above FMQ+2 and therefore some decompression melting in the mantle wedge is required to explain the higher fO2 values of primitive arc lavas than arc-peridotites. 相似文献
102.
103.
Influence of forest and shrub canopies on precipitation partitioning and isotopic signatures 下载免费PDF全文
Chris Soulsby Hannah Braun Matthias Sprenger Markus Weiler Doerthe Tetzlaff 《水文研究》2017,31(24):4282-4296
Over a 4‐month summer period, we monitored how forest (Pinus sylvestris ) and heather moorland (Calluna spp. and Erica spp.) vegetation canopies altered the volume and isotopic composition of net precipitation (NP) in a southern boreal landscape in northern Scotland. During that summer period, interception losses were relatively high and higher under forests compared to moorland (46% of gross rainfall [GR] compared with 35%, respectively). Throughfall (TF) volumes exhibited marked spatial variability in forests, depending upon local canopy density, but were more evenly distributed under heather moorland. In the forest stands, stemflow was a relatively small canopy flow path accounting for only 0.9–1.6% of NP and only substantial in larger events. Overall, the isotopic composition of NP was not markedly affected by canopy interactions; temporal variation of stable water isotopes in TF closely corresponded to that of GR with differences of TF‐GR being ?0.52‰ for δ2H and ?0.14‰ for δ18O for forests and 0.29‰ for δ2H and ?0.04‰ for δ18O for heather moorland. These differences were close to, or within, analytical precision of isotope determination, though the greater differences under forest were statistically significant. Evidence for evaporative fractionation was generally restricted to low rainfall volumes in low intensity events, though at times, subtle effects of liquid–vapour moisture exchange and/or selective transmission though canopies were evident. Fractionation and other effects were more evident in stemflow but only marked in smaller events. The study confirmed earlier work that increased forest cover in the Scottish Highlands will likely cause an increase in interception and green water fluxes at the expenses of blue water fluxes to streams. However, the low‐energy, humid environment means that isotopic changes during such interactions will only have a minor overall effect on the isotopic composition of NP. 相似文献
104.
Ground-based observations of the CO2 distribution on Mars were made this past opposition from Cerro Tololo Interamerican Observatory. Almost complete coverage of the Martian surface from 40°N to 60°S was obtained. Agreement with previous Kitt Peak observations is good, and confirmation of a pressure anomaly in the Tharsis region has been obtained. The ridge whose eastern slope is Syrtis Major stops at about 15°S, in agreement with the 1971 radar data. The Noachis-Hellas region south of Syrtis Major appears at about average altitude, indicating that the dust storm of 1971 was already active in that region as early as the end of August. 相似文献
105.
John H. Parkinson 《Solar physics》1975,42(1):183-207
Absolute intensities and wavelengths for 98 X-ray emission lines between 9 and 22.5 Å are reported. The active region spectra were obtained with three rocket-borne crystal spectrometers. Identifications are proposed for 62 of the lines and a model of the emitting plasma is constructed from the intensities of the strongest lines. The emission measure (N e 2 V) of the model peaks at 3 × 106 K with a value of 1.5 × 1047 cm?3 and decreases to 1046 cm?3 at 5 × 106 K. Effective oscill and collision strengths are calculated for the other transitions that are observed. The relative intensities of O viii and Ne ix give an oxygen : neon abundance ratio of 8 ∶ 1. The intensities of the satellite lines to helium-like lines are investigated and it is shown that these lines can be used with confidence in constructing active region models. 相似文献
106.
J. H. Parkinson 《Solar physics》1973,28(2):487-493
The temperature and density structure of a typical coronal active region is deduced from X-ray observations of several active regions. Observations of the limb transits of three regions from OSO-5 indicate that the X-ray emission originates between 2 × 104 km and 1.5 × 105 km. An emission measure-temperature distribution is deduced from high resolution X-ray spectra obtained with a rocket observation of two similar regions. These observations are combined to give a model of a typical active region, the temperature varying from 2 to 6 × 106 K with corresponding densities between 2 × 109 and 1010 cms–3. 相似文献
107.
108.
Hannah T.M. Heinrich Phil J. Bremer Christopher J. Daughney 《Geochimica et cosmochimica acta》2008,72(17):4185-4200
Acid-base titrations and electrophoretic mobility measurements were conducted on the thermophilic bacteria Anoxybacillus flavithermus and Geobacillus stearothermophilus at two different growth times corresponding to exponential and stationary/death phase. The data showed significant differences between the two investigated growth times for both bacterial species. In stationary/death phase samples, cells were disrupted and their buffering capacity was lower than that of exponential phase cells. For G. stearothermophilus the electrophoretic mobility profiles changed dramatically. Chemical equilibrium models were developed to simultaneously describe the data from the titrations and the electrophoretic mobility measurements. A simple approach was developed to determine confidence intervals for the overall variance between the model and the experimental data, in order to identify statistically significant changes in model fit and thereby select the simplest model that was able to adequately describe each data set. Exponential phase cells of the investigated thermophiles had a higher total site concentration than the average found for mesophilic bacteria (based on a previously published generalised model for the acid-base behaviour of mesophiles), whereas the opposite was true for cells in stationary/death phase. The results of this study indicate that growth phase is an important parameter that can affect ion binding by bacteria, that growth phase should be considered when developing or employing chemical models for bacteria-bearing systems. 相似文献
109.
Aaron Zimmerman Holly J. Stein Judith L. Hannah Dejan Koželj Kamen Bogdanov Tudor Berza 《Mineralium Deposita》2008,43(1):1-21
The Apuseni–Banat–Timok–Srednogorie magmatic–metallogenic belt (ABTS belt), forms a substantial metallogenic province in the
Balkan-South Carpathian system in southeastern Europe. The belt hosts porphyry, skarn, and epithermal deposits mined since
pre-Roman times. Generally, the deposits, prospects, and occurrences within the belt are linked to magmatic centers of calc-alkaline
affinity. Fifty-one rhenium-osmium (Re–Os) ages and Re concentration data for molybdenites define systematic geochronologic
trends and constrain the geochemical-metallogenic evolution of the belt in space and time. From these data and additional
existing geologic-geochemical data, a general tectonic history for the belt is proposed. Mineralization ages in Apuseni-Banat,
Timok, and Panagyurishte (the central district of the larger E–W Srednogorie Zone) range from 72–83, 81–88, and 87–92 Ma,
respectively, and clearly document increasing age from the northwestern districts to the southeastern districts. Further,
Re–Os ages suggest rapidly migrating pulses of Late Cretaceous magmatic–hydrothermal activity with construction of deposits
in ~1 m.y., districts in ~10 m.y., and the entire 1,500 km belt in ~20 m.y. Ages in both Timok and Panagyurishte show systematic
younging, while deposit ages in Banat and Apuseni are less systematic reflecting a restricted evolution of the tectonic system.
Systematic differences are also observed for molybdenite Re concentrations on the belt scale. Re concentrations generally
range from hundreds to thousands of parts per million, typical of subduction-related Cu–Au–Mo–(PGE) porphyry systems associated
with the generation of juvenile crust. The geochronologic and geochemical trends are compatible with proposed steepening of
subducting oceanic slab and relaxation of upper continental plate compression. Resulting influx of sub-continental mantle
lithosphere (SCML) and asthenosphere provide a fertile metal source and heat, while the subducting slab contributes connate
and mineral dehydration fluids, which facilitate partial melting and metal leaching of SCML and asthenosphere. Cu–Au–Mo–(PGE)
porphyry deposits may develop where melts are trapped at shallow crustal levels, often with associated volcanism and epithermal-style
deposits (South Banat, Timok, and Panagyurishte). Mo–Fe–Pb–Zn skarn deposits may develop where felsic melts are trapped adjacent
to Mesozoic limestones at moderate crustal levels (North Banat and Apuseni). Systematic spatial variations in deposit style,
commodity enrichment, Re–Os ages, and Re concentrations support specific tectonic processes that led to ore formation. In
a post-collisional setting, subduction of Vardar oceanic crust may have stalled, causing slab steepening and rollback. The
slab rollback relaxes compression, facilitating and enhancing orogenic collapse of previously thickened Balkan-South Carpathian
crust. The progression of coupled rollback-orogenic collapse is evidenced by the width of Late Cretaceous extensional basins
and northward younging of Re–Os ages, from Panagyurishte (~60 km; 92–87 Ma) to Timok (~20 km; 88–81 Ma) to Apuseni-Banat (~5 km;
83–72 Ma). Generation of a well-endowed mineral belt, such as the ABTS, requires a temporally and spatially restricted window
of magmatic–hydrothermal activity. This window is quickly opened as upper plate compression relaxes, thereby inducing melt
generation and ingress of melt to higher crustal levels. The window is just as quickly closed as upper plate compression is
reinstated. The transient tectonic state responsible for economic mineralization in the ABTS belt may be a paleo-analogue
to transient intervals in the present subduction tectonics of SE Asia where much mineral wealth has been created in the last
few million years. 相似文献
110.
Brian Mills Dan Unrau Carla Parkinson Brenda Jones Jennifer Yessis Kelsey Spring Laurel Pentelow 《Natural Hazards》2008,47(2):157-183
This article summarizes research completed to assess the risk of lightning-related injuries and fatalities in Canada. Although
lightning mortality has declined significantly over the past century, it remains a common meteorological hazard that regularly
kills and injures. Based on an analysis of media reports, vital statistics, hospital admission and emergency room visit records,
and fire loss data, the authors estimate that on average about 9–10 lightning-related deaths and 92–164 injuries occur each
year in Canada. The distribution of casualties reflects current provincial population and cloud-to-ground lightning densities.
Consistent with similar studies in other developed nations, most lightning-related fatalities and injuries in Canada occur
during the June-August summer season, coincident with peak lightning, and during the Thursday-Saturday period, most likely
related to higher rates of participation in outdoor activities. The majority of victims are male, less than 46 years old,
and engaged in outdoor recreational activities when injured or killed in a lightning incident. Media reports used in the study
were found to underestimate both lightning mortality (36%) and morbidity (20–600%).
相似文献
Brian MillsEmail: |