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941.
Daniel D. Riemer Eric C. Apel John J. Orlando Geoffrey S. Tyndall William H. Brune Eric J. Williams William A. Lonneman James D. Neece 《Journal of Atmospheric Chemistry》2008,61(3):227-242
As part of the 2000 Texas Air Quality Study (TexAQS), we studied the isoprene oxidation process under ambient conditions to
discern the presence of chlorine atom (Cl) chemistry in the Houston, Texas urban area. By measuring chloromethylbutenone (CMBO)
and an isomer of chloromethylbutenal (CMBA), we clearly observed sixteen episodes of active Cl chemistry during the 24-day
experiment. Estimated median Cl concentration during each of these episodes was between the detection limit of ~102 atoms cm−3 and 50 - 30 + 70 ×104 50_{ - 30}^{ + 70} \times {10^4} atoms cm−3. Cl concentration during all the episodes averaged 7.6 - 2.0 + 4.7 ×104 7.6_{ - 2.0}^{ + 4.7} \times {10^4} atoms cm−3 and thus amounted to less than 3% of the OH concentration during the same periods. During the episodes, the fraction of oxidation
chemistry initiated by Cl ranged from 3–43% and was strongly dependent on the quantity and type of hydrocarbons present in
the atmosphere. Because of its intermittent presence and low concentration, Cl is not a broadly influential oxidant in the
Houston, Texas urban area. 相似文献
942.
Observations were made of a shallow stratus of upslope origin using an aircraft equipped with insitu probes and with a vertically-pointing radar of 3-mm wavelength. A cloud layer of 300 m thickness was found below the inversion; an additional layer of 100 m thickness was located within the inversion. The coldest temperature within the cloud was -2°C and the cloud contained no ice particles. Drizzle drops up to 180 Am were present in both cloud layers.The observations reveal precipitation and air motion structures of approximately 1 km horizontal dimensions. The origin of this organization appears to be weak convection. In addition, mixing played an important role in forming the cloud droplet and drizzle drop size distributions. 相似文献
943.
944.
We review the theoretical basis for, and the advantages of, random flight models for the trajectories of tracer particles in turbulence. We then survey their application to calculate dispersion in the principal types of atmospheric turbulence (stratified, vertically-inhomogeneous, Gaussian or non-Gaussian turbulence in the surface layer and above), and show that they are especially suitable for some problems (e.g., quantifying ground emissions). 相似文献
945.
946.
Cliff recession on the high rocky coast between Gabicce and Pesaro Adriatic sea causes a wide range of mass movement processes on the whole slope, affecting both the bedrock and the overburden. The outcropping late Miocene rock formations are represented by marls, marly limestones, dark laminated mudstones and bedded sandstones and marls. Mass movements are common because of stratification and discontinuities in the rocks that, together with the presence of groundwater and weathering processes, reduce the overall strength of the slopes. A model for the evolution of this coastal area is proposed, which involves cyclic basal erosion, followed by mass movement that favours debris accumulation at the base of the cliff. The longshore currents have to then remove the material before a new cycle can begin. 相似文献
947.
A Spatial Variant of the Basic Reproduction Number for the New Orleans Yellow Fever Epidemic of 1878
Andrew Curtis Jacqueline W. Mills Jason K. Blackburn 《The Professional geographer》2007,59(4):492-502
A spatial variant of the basic reproduction number (R0), here defined as the number of subsequent deaths attributed to an initial mortality, can be used to identify geographic variation within an epidemic. A spatial R0 was calculated at the neighborhood level, here defined by a 50‐m buffer surrounding an index case, for mortality data from the 1878 yellow fever epidemic of New Orleans. The highest number of secondary mortalities linked to a neighborhood index case was twelve, with a further eighty‐seven extrapolated morbidity cases. Results also highlight the importance of multideath residences and cultural contacts in neighborhood‐level disease spread. 相似文献
948.
The main features of the spatial and temporal oscillations of the annual runoff of the rivers in the Upper Ob basin, which is characterized by various landscape and hydrologic conditions, are discussed. It is found that the coefficients of pair correlation of the annual runoff have been decreasing since the late 1990s-early 2000s. Correlation functions for mountain areas should be constructed separately for river basins ranked according to the prevailing type of river feed. The coefficients of pair correlation can be described by multiple regression equations, which, apart from the distance between the centers of gravity of the basins, may include landscape characteristics such as the difference in their average elevation and forest cover. 相似文献
949.
950.