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191.
The goal of this study was to demonstrate how the extent of denitrification, which is indirectly related to dissolved organ carbon and directly related to oxygen concentrations, can also be linked to unsaturated-zone thickness, a mappable aquifer property. Groundwater from public supply and monitoring wells in Northport on Long Island, New York state (USA), were analyzed for denitrification reaction progress using dissolved N2/Ar concentrations by membrane inlet mass spectrometry. This technique allows for discernment of small amounts of excess N2, attributable to denitrification. Results show an average 15 % of total nitrogen in the system was denitrified, significantly lower than model predictions of 35 % denitrification. The minimal denitrification is due to low dissolved organic carbon (29.3–41.1 μmol L?1) and high dissolved oxygen concentrations (58–100 % oxygen saturation) in glacial sediments with minimal solid-phase electron donors to drive denitrification. A mechanism is proposed that combines two known processes for aquifer re-aeration in unconsolidated sands with thick (>10 m) unsaturated zones. First, advective flux provides 50 % freshening of pore space oxygen in the upper 2 m due to barometric pressure changes. Then, oxygen diffusion across the water-table boundary occurs due to high volumetric air content in the unsaturated-zone catchment area. 相似文献
192.
Stress-induced evolution of anisotropic thermal conductivity of dry granular materials 总被引:1,自引:1,他引:0
Jinhyun Choo Young Jin Kim Jung Hwoon Lee Tae Sup Yun Jangguen Lee Young Seok Kim 《Acta Geotechnica》2013,8(1):91-106
Various factors, such as the volumetric fraction of constituents, mineralogy, and pore fluids, affect heat flow in granular materials. Although the stress applied on granular materials controls the formation of major pathways for heat flow, few studies have focused on a detailed investigation of its significance with regard to the thermal conductivity and anisotropy of the materials. This paper presents a numerical investigation of the stress-induced evolution of anisotropic thermal conductivity of dry granular materials with supplementary experimental results. Granular materials under a variety of stress conditions in element testing are analyzed by the three-dimensional discrete element method, and quantitative variations in their anisotropic effective thermal conductivity are calculated via the network model and conductivity tensor measurements. Results show that the directional development of contact area and fabric under anisotropic stress conditions leads to the evolution of anisotropy in thermal conductivity. The anisotropy induced in thermal conductivity by shear stress is higher than that induced by compressive stress because shear stress causes more significant changes in microstructural configurations and boundary conditions. The shear-stress-induced evolution of anisotropy between principal thermal conductivities depends on dilatancy as well as shearing mode, and the shear-driven discontinuity localizes the conductivity. Factors involved in the stress-induced evolution and their implications on the thermal conductivity characterization are discussed. 相似文献
193.
Pyrite paragenesis and multiple sulfur isotope distribution in late Archean and early Paleoproterozoic Hamersley Basin sediments 总被引:1,自引:0,他引:1
Michaela A. Partridge Suzanne D. Golding Kim A. Baublys Elisa Young 《Earth and Planetary Science Letters》2008,272(1-2):41-49
The sulfur isotope record in late Archean and early Paleoproterozoic rocks is of considerable importance because it provides evidence for changes in early Earth atmospheric oxygen levels and potentially constrains the origin and relative impact of various microbial metabolisms during the transition from an anoxic to oxic atmosphere. Mass independently fractionated (MIF) sulfur isotopes reveal late Archean and early Paleoproterozoic sulfur sources in different pyrite morphologies in Western Australia's Hamersley Basin. Multiple sulfur isotope values in late Archean pyrite vary according to morphology. Fine grained pyrite has positive sulfur MIF, indicating a reduced elemental sulfur source, whereas pyrite nodules have negative sulfur MIF, potentially derived from soluble sulfate via microbial sulfate reduction. The Hamersley Basin δ34S–Δ33S record suggests that the extent of oxygenation of the surface ocean fluctuated through the Late Archean from at least 2.6 Ga, more than 150 million yr before the Great Oxidation Event. In the early Paleoproterozoic, there is less distinction between pyrite morphologies with respect to sulfur isotope fractionation, and pyrite from the Brockman Iron Formation trends toward modern sulfur isotope values. An important exception to this is the strong negative MIF recorded in layer parallel pyrite in Paleoproterozoic carbonate facies iron formation. This may suggest that deeper water hydrothermal environments remained anoxic while shallower water environments became more oxidised by the early Paleoproterozoic. The results of the current study indicate that sulfide paragenesis is highly significant when investigating Archean and early Paleoproterozoic multiple sulfur isotope compositions and sulfur sources. 相似文献
194.
The purpose of this study was to examine the historical change in sedimentation rates in lakes that have been impacted by river regulation and agricultural activities in the Ishikari River floodplain. We dated sediment cores using caesium‐137 (137Cs) dating and tephrochronology, and we estimated sediment sources from 137Cs concentrations in the topsoil of representative land covers. We found that, between 1739 and 1963, the distance between the lake and the main river channel and whether or not the lake was connected to the river affected the sedimentation rates. After 1963, agricultural drainage systems were established in the Ishikari River floodplain. The average sedimentation rate before and after the construction of drainage ditches varied between 1–66 and 87–301 mg cm–2 a–1, respectively. The increase in the sedimentation rate after 1963 was caused by the construction of a number of drainage networks, as well as extensive cultivation activity and/or fragmentation of the swamp buffers surrounding the lakes. The 137Cs activities at the surfaces of the lake as well as the catchment‐derived 137Cs contributions and 137Cs inventory in the lake profiles were used to examine the sediment influx from the various drainage areas after the establishment of the drainage system. Our results indicate that the majority of the lake sediments were derived from cultivated areas, and therefore the catchment‐derived 137Cs contribution in the lakes was strongly correlated with the sedimentation rate. The 137Cs inventory across all of the lake profiles was also significantly greater than the atmospheric fallout. We identified a negative correlation between the 137Cs lake profile inventory and the sedimentation rate. This is because the sediment originating from the drainage areas contained low 137Cs concentrations, which diluted the overall concentration of 137Cs in the lake sediment. Copyright © 2009 John Wiley & Sons, Ltd. 相似文献
195.
Movement of Heavy Metals in Soil through Preferential Flow Paths under Different Rainfall Intensities 总被引:1,自引:0,他引:1
Preferential flow in soils deserves attention due to its potential role in accelerating the movement of contaminants to groundwater. This study investigates the movement of Cd, Cu, and Pb through preferential flow paths under different applied rainfall intensities. Artificial acid rain (pH of 4.1) containing CdCl2, CuCl2, and Pb(NO3)2 was applied to undisturbed soil and repacked sand columns at low and high intensities, and leachate metals and chloride concentrations were measured. Cd was found in the leachate at both low and high rates in all columns, while the increase in Cu concentrations in the leachate was detected only at the high rate of the undisturbed columns. Pb was retained in both columns. For undisturbed columns, the breakthrough curves of Cd and Cu were similar to those of Cl, showing early initial breakthrough by preferential flow and dependency on rainfall intensities. The Cd concentrations were detected in the leachate from repacked columns for high rate rainfall, implying that even homogeneous soil may not be perfectly able to retain metals and the initially wet condition is more harmful for subsurface contaminant transport. In conclusion, the study demonstrated that, despite its highly sorptive nature, the transport of some metals may be as fast as that of a tracer under preferential flow conditions, and the rainfall intensity is a significant factor for the degree of transport. 相似文献
196.
Large-scale dune activity in the Nebraska Sand Hills and elsewhere on the western Great Plains has been linked to prehistoric “megadroughts” that triggered the activation of regional dune fields. The effect of megadroughts on the smaller dune fields east of the Nebraska Sand Hills has never been assessed, however. This study focuses on the Duncan dune field near the confluence of the Loup and Platte rivers in eastern Nebraska. Seventeen optically stimulated luminescence age estimates were obtained and reveal two periods of dune activation that occurred between 4.4 to 3.4 ka and 0.8 to 0.5 ka. Significantly, both periods chronologically overlap large-scale dune activity identified in the Nebraska Sand Hills. Geochemical evidence indicates that the Duncan dunes received sand not only from the terrace underlying them, but also from the Loup River. These data link dune activity in the Duncan area, at least indirectly, to increased sediment supply from streams that drain the Sand Hills during megadroughts, implying the activation of the dunes occurred as an indirect response to regional megadroughts. Calculations of dune migration rates, however, argue in favor of local, drought-driven hydrologic changes as a causative factor in dune activation, in other words, a direct effect of megadroughts. Whether the impact was direct or indirect, it is highly likely that the repeated reactivation of the Duncan dunes resulted in some way from regional, large-magnitude droughts. Other paleoclimate proxies from the Great Plains tend to support this conclusion. We conclude that the megadroughts that have been identified in the Sand Hills and other Great Plains dune fields were indeed regional events with far-reaching effects. 相似文献
197.
Projections of ocean climate for northwestern Pacific Ocean 总被引:1,自引:1,他引:0
The long-term adjustment processes of atmosphere and ocean in response to gradually increased atmospheric CO2 concentration have been analyzed in 70 and 140a integrations with NCAR fully-coupled climate system model (CSM). In these experiments the CO2 concentration has been increased to double and quadruples the initial concentration, respectively. After 70a, at the time of CO2 doubling, the model predicts surface air temperature rises by 1.2 and 1.5K for the globe and the northwestern Pacific Ocean, respectively. The behavior of the quadrupling run is similar: each global and regional mean surface air temperatures increase by 2.8 and 3.0K at the time of CO2 quadrupling. From the experiments, surface air temperature changes in the northwestern Pacific Ocean will be more distinctive compared with the global average, mainly due to exceptionally large warming and sea level change near the entrance of the Kuroshio extension. 相似文献
198.
Tetsuichi TAKAGI Sang–Mo KOH Moon–Young KIM Kazuki NAITO Sadahisa SUDO 《Resource Geology》2000,50(4):243-256
Abstract: The Milyang pyrophyllite deposit, which is embedded in the Late Cretaceous Yuchon Group of the Kyongsang Supergroup, is one of the largest hydrothermal clay deposits in the Kyongsang basin, southeast Korea. Host rocks of the deposit are porphyritic andesite lava and minor andesitic lapilli tuff. In the Milyang district, a hydrothermally altered zone is about 2 × 3 km in extent; we can recognize the concentric arrangement of advanced argillic, propylitic, and sericitic alteration zones from the central to peripheral parts of the zone. The Milyang pyrophyllite deposit forms a part of the advanced argillic alteration zone. The Milyang pyrophyllite deposit is subdivided into the following four zones based on mineral assemblages: the pyrophyllite zones 1, 2, 3, and the silicified zone. The pyrophyllite zone 1, which occupies the central part of the deposit, comprises mainly pyrophyllite, kaolinite, and diaspore without quartz. Diaspore nodules often concentrate in beds 40–50 cm thick. Andalusite, dumortierite, and tourmaline locally occur as network veins, crack‐filler, or small spherulitic spots. The Al2O3 content of the ore ranges from 27 to 36 wt%. The pyrophyllite zone 2, which constitutes a major part of the deposit, comprises mainly pyrophyllite, kaolinite, and quartz. The Al2O3 content of the ore ranges from 15 to 24 wt%. The pyro‐phyllite zone 3 is the hematite‐rich marginal facies of the deposit. The silicified zone, which occurs as beds and septa, is mostly composed of quartz with minor pyrophyllite and kaolinite; the SiO2 contents range from 79 to 90 wt%. Comparing chemical compositions of the high‐Al ores with those of unaltered host andesite, the Fe, Ca, alkalis, HFSE, and HREE contents are significantly depleted, whereas S, B, As, Sr, and LREE are enriched. The hydrothermal alteration of the Milyang pyrophyllite deposit can be classified into the following four stages: 1) extensive sericitic and propylitic alteration, 2) medium‐temperature (200–250°C) advanced argillic alteration, 3) high‐temperature (250–350°C or more) advanced argillic alteration, and 4) retrograde low‐temperature alteration. The heat and some volatile components such as B and S would be derived from the Pulguksa Granite intruded underneath the deposit. 相似文献
199.
The establishment of local self-government was a key part of the post-1989 transformation in East and Central Europe. Local
government in both Western and East and Central Europe has increasingly been expected to play a role in local economic development
(LED). Local government is one important agent in the complex processes of building 'institutional thickness' to ensure the
development of local economies and the quality of life of inhabitants. This paper presents the results of a national postal
questionnaire survey of the LED role of the lowest level of local self-government in Poland, the gmina or commune. The paper
establishes a baseline of knowledge regarding: the local economic problems faced by communes; their attitudinal, strategic
and organisational responses; and the main factors which are hindering the communes' LED role.
This revised version was published online in July 2006 with corrections to the Cover Date. 相似文献
200.