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821.
T. V. Klets 《Stratigraphy and Geological Correlation》2008,16(5):467-489
Geographic differentiation of conodontophorids between northern and southern latitudes commenced in the Triassic since the early Induan. Cosmopolitan long-lived genera of predominantly smooth morphotypes without sculpturing were characteristic of high-latitude basins of the Panboreal Superrealm. Since the early Olenekian until the Carnian inclusive, this superrealm consisted of the Siberian Realm that extended over Northeast Asia and the Canada-Svalbard Realm that included the Svalbard Archipelago and northern regions of Canada. Throughout the Triassic period, conodontophorids characteristic of the Tethys-Panthalassa Superrealm spanning the Tethys and low-latitude zones of the Pacific were highly endemic, very diverse in taxonomic aspect, having well-developed sculpturing and tempos of morphological transformations. Distinctions between the Early-Middle Triassic conodontophorids from northern and southern zones were not as great as afterward, and their impoverished assemblages from southern Tethyan basins were close in some respects to the Boreal ones. Their habitat basins of that time can be grouped into the Mediterranean-Pacific and India-Pakistan realms. Hence, the extent of geographic differentiation of conodontophorids was not constant and gradually grew, as their taxonomic diversity was reducing in northern basins but relatively increasing in southern ones. The Panboreal e Tethys-Panthalassa superrealms of conodontophorids, which are most clearly recognizable, are close to first-rank paleobiochores (superrealms) established earlier for ammonoids and bivalve mollusks. Main factor that controlled geographic differentiation of Triassic conodontophorids was climatic zoning. Initially lower diversity of southern Tethyan assemblages points probably to relatively cooler water regime in the peri-Gondwanan part of the Tethys. The established patterns in geographic distribution of conodontophorids characterize most likely the real trend of their differentiation and evolution, i.e., the distribution area contraction prior to complete extinction at the end of the Triassic 相似文献
822.
F. Parello A. Aiuppa H. Calderon F. Calvi D. Cellura V. Martinez M. Militello K. Vammen D. Vinti 《Applied Geochemistry》2008
This paper reports new geochemical data on dissolved major and minor constituents in surface waters and ground waters collected in the Managua region (Nicaragua), and provides a preliminary characterization of the hydrogeochemical processes governing the natural water evolution in this area. The peculiar geological features of the study site, an active tectonic region (Nicaragua Depression) characterized by active volcanism and thermalism, combined with significant anthropogenic pressure, contribute to a complex evolution of water chemistry, which results from the simultaneous action of several geochemical processes such as evaporation, rock leaching, mixing with saline brines of natural or anthropogenic origin. The effect of active thermalism on both surface waters (e.g., saline volcanic lakes) and groundwaters, as a result of mixing with variable proportions of hyper-saline geothermal Na–Cl brines (e.g., Momotombo geothermal plant), accounts for the high salinities and high concentrations of many environmentally-relevant trace elements (As, B, Fe and Mn) in the waters. At the same time the active extensional tectonics of the Managua area favour the interaction with acidic, reduced thermal fluids, followed by extensive leaching of the host rock and the groundwater release of toxic metals (e.g., Ni, Cu). The significant pollution in the area, deriving principally from urban and industrial waste-water, probably also contributes to the aquatic cycling of many trace elements, which attain concentrations above the WHO recommended limits for the elements Ni (∼40 μg/l) and Cu (∼10 μg/l) limiting the potential utilisation of Lake Xolotlan for nearby Managua. 相似文献
823.
824.
825.
826.
Rice is a major exposure route for arsenic in Chakdaha block,Nadia district,West Bengal,India: A probabilistic risk assessment 总被引:2,自引:0,他引:2
The importance or otherwise of rice as an exposure pathway for As ingestion by people living in Bengal and other areas impacted by hazardous As-bearing groundwaters is currently a matter of some debate. Here this issue is addressed by determining the overall increased cancer risk due to ingestion of rice in an As-impacted district of West Bengal. Human target cancer health risks have been estimated through the intake of As-bearing rice by using combined field, laboratory and computational methods. Monte Carlo simulations were run following fitting of model probability curves to measured distributions of (i) As concentration in rice and drinking water and (ii) inorganic As content of rice and fitting distributions to published data on (i) ingestion rates and (ii) body weight and point estimates on bioconcentration factors, exposure duration and other input variables. The distribution of As in drinking water was found to be substantially lower than that reported by previous authors for As in tube wells in the same area, indicating that the use of tube well water as a proxy for drinking water is likely to result in human health risks being somewhat overestimated. The calculated median increased lifetime cancer risk due to cooked rice intake was 7.62 × 10−4, higher than the 10−4–10−6 range typically used by the USEPA as a threshold to guide determination of regulatory values and similar to the equivalent risk from water intake. The median total risk from combined rice and water intake was 1.48 × 10−3. The contributions to this median risk from drinking water, rice and cooking of rice were found to be 48%, 44% and 8%, respectively. Thus, rice is a major potential source of As exposure in the As-affected study areas in West Bengal and the most important exposure pathway for groups exposed to low or no As in drinking water. 相似文献
827.
J.A. Saunders M.-K. Lee M. Shamsudduha P. Dhakal A. Uddin M.T. Chowdury K.M. Ahmed 《Applied Geochemistry》2008
Here new data from field bioremediation experiments and geochemical modeling are reported to illustrate the principal geochemical behavior of As in anaerobic groundwaters. In the field bioremediation experiments, groundwater in Holocene alluvial aquifers in Bangladesh was amended with labile water-soluble organic C (molasses) and MgSO4 to stimulate metabolism of indigenous SO4-reducing bacteria (SRB). In the USA, the groundwater was contaminated by Zn, Cd and SO4, and contained <10 μg/L As under oxidized conditions, and a mixture of sucrose and methanol were injected to stimulate SRB metabolism. In Bangladesh, groundwater was under moderately reducing conditions and contained ∼10 mg/L Fe and ∼100 μg/L As. In the USA experiment, groundwater rapidly became anaerobic, and dissolved Fe and As increased dramatically (As > 1000 μg/L) under geochemical conditions consistent with bacterial Fe-reducing conditions. With time, groundwater became more reducing and biogenic SO4 reduction began, and Cd and Zn were virtually completely removed due to precipitation of sphalerite (ZnS) and other metal sulfide mineral(s). Following precipitation of chalcophile elements Zn and Cd, the concentrations of Fe and As both began to decrease in groundwater, presumably due to formation of As-bearing FeS/FeS2. By the end of the six-month experiment, dissolved As had returned to below background levels. In the initial Bangladesh experiment, As decreased to virtually zero once biogenic SO4 reduction commenced but increased to pre-experiment level once SO4 reduction ended. In the ongoing experiment, both SO4 and Fe(II) were amended to groundwater to evaluate if FeS/FeS2 formation causes longer-lived As removal. Because As-bearing pyrite is the common product of SRB metabolism in Holocene alluvial aquifers in both the USA and Southeast Asia, it was endeavored to derive thermodynamic data for arsenian pyrite to better predict geochemical processes in naturally reducing groundwaters. Including the new data for arsenian pyrite into Geochemist’s Workbench, its stability field completely dominates in reducing Eh–pH space and “displaces” other As-sulfides (orpiment, realgar) that have been implied to be important in previous modeling exercises and reported in rare field conditions. 相似文献
828.
Kathleen A. Radloff Anya R. Manning Brian Mailloux Yan Zheng M. Moshiur Rahman M. Rezaul Huq Kazi M. Ahmed Alexander van Geen 《Applied Geochemistry》2008
Microbial Fe reduction is widely believed to be the primary mechanism of As release from aquifer sands in Bangladesh, but alternative explanations have been proposed. Long-term incubation studies using natural aquifer material are one way to address such divergent views. This study addresses two issues related to this approach: (1) the need for suitable abiotic controls and (2) the spatial variability of the composition of aquifer sands. Four sterilization techniques were examined using orange-colored Pleistocene sediment from Bangladesh and artificial groundwater over 8 months. Acetate (10 mM) was added to sacrificial vials before sterilization using either (1) 25 kGy of gamma irradiation, (2) three 1-h autoclave cycles, (3) a single addition of an antibiotic mixture at 1× or (4) 10× the typical dose, and (5) a 10 mM addition of azide. The effectiveness of sterilization was evaluated using two indicators of microbial Fe reduction, changes in diffuse spectral reflectance and leachable Fe(II)/Fe ratios, as well as changes in P-extractable As concentrations in the solid phase. A low dose of antibiotics was ineffective after 70 days, whereas autoclaving significantly altered groundwater composition. Gamma irradiation, a high dose of antibiotics, and azide were effective for the duration of the experiment. 相似文献
829.
830.
Flood hazard delineation combining geomorphological and hydrological methods: an example in the Northern Iberian Peninsula 总被引:2,自引:1,他引:1
Flood mapping requires the combination and integration of geomorphological and hydrological-hydraulic methods; however, despite
this, there is very little scientific literature that compares and validates both methods. Two types of analysis are addressed
in the present article. On the one hand, maps of flood plains have been elaborated using geomorphological evidence and historical
flood data in the mountainous area of northwestern Spain, covering an area of more then 232 km2 of floodplains. On the other hand, a hydrometeorological model has been developed (Clark semidistributed unit hydrograph)
in the Sarria River basin (155 km2, NW Spain). This basin is not gauged, hence the model was subjected to a goodness-of-fit test of its parameter (curve number)
by means of Monte Carlo simulation. The peak flows obtained by means of the hydrological model were used for hydraulic modeling
(one-phase, one-dimensional and steady flow) in a 4 km2 urban stretch of the river bed. The delineation of surface areas affected by floods since 1918, as well as those analyzed
subsequent to the geomorphological study, reveals a high degree of reliability in the delineation of the flooded areas with
frequent recurrence intervals (<50 years). If we compare these flooded surface areas with the estimate obtained by the hydrological-hydraulic
method we can see that the latter method overestimates the extent of the surface water by 144% for very frequent recurrence
intervals (>10 years) and underestimates it as the recurrence interval increases, by up to 80% less floodplain for exceptional
events (>500 years). Finally, a management map is put forth combining the most reliable results available by integrating both
methods.
Originally presented at the Sixth International Conference on Geomorphology. 相似文献