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91.
Vladimir A. Krasnopolsky Jean Pierre Maillard Tobias C. Owen Robert A. Toth Michael D. Smith 《Icarus》2007,192(2):396-403
Oxygen and carbon isotope ratios in the martian CO2 are key values to study evolution of volatiles on Mars. The major problems in spectroscopic determinations of these ratios on Mars are uncertainties associated with: (1) equivalent widths of the observed absorption lines, (2) line strengths in spectroscopic databases, and (3) thermal structure of the martian atmosphere during the observation. We have made special efforts to reduce all these uncertainties. We observed Mars using the Fourier Transform Spectrometer at the Canada–France–Hawaii Telescope. While the oxygen and carbon isotope ratios on Mars were byproducts in the previous observations, our observation was specifically aimed at these isotope ratios. We covered a range of 6022 to 6308 cm−1 with the highest resolving power of ν/δν=3.5×105 and a signal-to-noise ratio of 180 in the middle of the spectrum. The chosen spectral range involves 475 lines of the main isotope, 184 lines of 13CO2, 181 lines of CO18O, and 119 lines of CO17O. (Lines with strengths exceeding 10−27 cm at 218 K are considered here.) Due to the high spectral resolution, most of the lines are not blended. Uncertainties of retrieved isotope abundances are in inverse proportion to resolving power, signal-to-noise ratio, and square root of the number of lines. Laboratory studies of the CO2 isotope spectra in the range of our observation achieved an accuracy of 1% in the line strengths. Detailed observations of temperature profiles using MGS/TES and data on temperature variations with local time from two GCMs are used to simulate each absorption line at various heights in each part of the instrument field of view and then sum up the results. Thermal radiation of Mars' surface and atmosphere is negligible in the chosen spectral range, and this reduces errors associated with uncertainties in the thermal structure on Mars. Using a combination of all these factors, the highest accuracy has been achieved in measuring the CO2 isotope ratios: 13C/12C = 0.978 ± 0.020 and 18O/16O = 1.018 ± 0.018 times the terrestrial standards. Heavy isotopes in the atmosphere are enriched by nonthermal escape and sputtering, and depleted by fractionation with solid-phase reservoirs. The retrieved ratios show that isotope fractionation between CO2 and oxygen and carbon reservoirs in the solid phase is almost balanced by nonthermal escape and sputtering of O and C from Mars. 相似文献
92.
Cassini VIMS detected carbon dioxide on the surface of Iapetus during its insertion orbit. We evaluated the CO2 distribution on Iapetus and determined that it is concentrated almost exclusively on Iapetus’ dark material. VIMS spectra show a 4.27-μm feature with an absorption depth of 24%, which, if it were in the form of free ice, requires a layer 31 nm thick. Extrapolating for all dark material on Iapetus, the total observable CO2 would be 2.3 × 108 kg.Previous studies note that free CO2 is unstable at 10 AU over geologic timescales. Carbon dioxide could, however, be stable if trapped or complexed, such as in inclusions or clathrates. While complexed CO2 has a lower thermal volatility, loss due to photodissociation by UV radiation and gravitational escape would occur at a rate of 2.6 × 107 kg year−1. Thus, Iapetus’ entire inventory of surface CO2 could be lost within a few decades.The high loss/destruction rate of CO2 requires an active source. We conducted experiments that generated CO2 by UV radiation of simulated icy regolith under Iapetus-like conditions. The simulated regolith was created by flash-freezing degassed water, crushing it into sub-millimeter sized particles, and then mixing it with isotopically labeled amorphous carbon (13C) dust. These samples were placed in a vacuum chamber and cooled to temperatures between 50 K and 160 K. The samples were irradiated with UV light, and the products were measured using a mass spectrometer, from which we measured 13CO2 production at a rate of 2.0 × 1012 mol s−1. Extrapolating to Iapetus and adjusting for the solar UV intensity and Iapetus’ surface area, we calculated that CO2 production for the entire surface would be 1.1 × 107 kg year−1, which is only a factor of two less than the loss rate. As such, UV photochemical generation of CO2 is a plausible source of the detected CO2. 相似文献
93.
Impacts of comets and asteroids play an important role in volatile delivery on the Moon. We use a novel method for tracking vapor masses that reach escape velocity in hydrocode simulations of cometary impacts to explore the effects of volatile retention. We model impacts on the Moon to find the mass of vapor plume gravitationally trapped on the Moon as a function of impact velocity. We apply this result to the impactor velocity distribution and find that the total impactor mass retained on the Moon is approximately 6.5% of the impactor mass flux. Making reasonable assumptions about water content of comets and the comet size-frequency distribution, we derive a water flux for the Moon. After accounting for migration and stability of water ice at the poles, we estimate a total 1.3×108-4.3×109 metric tons of water is delivered to the Moon and remains stable at the poles over 1 Ga. A factor of 30 uncertainty in the estimated cometary impact flux is primarily responsible for this large range of values. The calculated mass of water is sufficient to account for the neutron fluxes poleward of 75° observed by Lunar Prospector. A similar analysis for water delivery to the Moon via asteroid impacts shows that asteroids provide six times more water mass via impacts than comets. 相似文献
94.
Accretional temperature profiles for Saturn’s large moon Titan are used to determine the conditions needed for accretion to avoid global melting as a function of the timing, duration, and nebular conditions of Titan’s accretion. We find that Titan can accrete undifferentiated in a “gas-starved” disk even with modest quantities of ammonia mixed in with its ices. Simulations of impact-induced core formation are used to show that Titan can remain only partially differentiated after an outer Solar System late heavy bombardment capable of melting its outer layers, permitting some of its rock to consolidate into a core. 相似文献
95.
The Tycho Epoch Photometry Annex A, a data base of photometry of more than 34 000 bright stars, has been searched for periodic variable stars with approximately sinusoidal light curves. Advantage was taken of special properties of the observing programme (photometry in two wavebands, availability of repeated measurements) to use simple but efficient variable selection criteria. Details of 70 strong candidate variables are presented. 相似文献
96.
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98.
Ultrasonic data for the velocities of SiO2-stishovite have been determined as a function of pressure to 10 kbar at room temperature for polycrystalline specimens hot-pressed at pressures P = 120kbar and temperatures T = 900°C. These cylindrical specimens are 2 mm in diameter and 0.9–1.4 mm long and have a grain size less than 10 μm. Compressional and shear wave velocities were measured both parallel and perpendicular to the axis of pressing and were found to be isotropic at 10 kbar with νp = 11.0 ± 0.2km/sec andνs = 6.9 ± 0.3km/sec; this shear velocit is substantially higher than that of Mizutani et al. (1972) perhaps due to the presence of crack orientations in their specimen which affected νs but not νp. The Murnaghan P-V trajectories calculated from the ultrasonic data [bulk modulus Ks = 2.5 ± 0.3Mbar and assuming (?Ks/?P)T = 6 ± 2] are consistent with recent hydrostatic compression data and with the shock wave compression data above 600 kbar. The combined evidence from the data of the ultrasonic and hydrostatic compression techniques suggests that the most probable value of the bulk modulus of stishovite at zero pressure is close to the upper limit of the uncertainty of our ultrasonically determined value, K0 = 2.7?2.8Mbar. Elasticity data for rutile-type oxides are not compatible with normal Ks-V0 systematics perhaps due to the neglect of non-central forces in the lattice model. These new stishovite data would make it impossible to satisfy the elasticity-density data of the lower mantle using an oxide mixture with either olivine or pyroxene stoichiometry. 相似文献
99.
The US Minerals Management Service (MMS) is responsible for safe and environmentally sound management of offshore oil and gas resources. In recent years, there has been a tremendous increase in both activities and plans for deepwater development of these resources in the Gulf of Mexico (GOM). As the industry meets the enormous technical challenges involved, there is a concomitant effort to assure environmental protection of deep-ocean and coastal resources. This paper will outline the research planning and program currently underway to assess impacts, identify potential problems, and discover more about unknown resources of the deep ocean. 相似文献
100.
Bowser Lake, a fiord lake in the northern Coast Mountains of British Columbia, contains a thick Holocene fill consisting mainly of silt and clay varves. These sediments were carried into the lake by proglacial Bowser River which drains a high-energy, heavily glacierized basin. Sedimentation in the lake is controlled by seasonal snow and ice melt, by autumn rainstorms, and by rare, but very large jökulhlaups from glacier-dammed lakes in the upper Bowser River basin which complicate environmental inferences from the sedimentary record. Sediment is dispersed through the deep western part of the lake by energetic turbidity currents. The turbidity currents apparently do not overtop a sill that separates the western basin from much shallower areas to the east. Large amounts of silt and clay are deposited from suspension in the eastern part of the lake, but sediment accumulation rates there are much lower than to the west. Several strong acoustic reflectors punctuate the varved fill in the western basin; these may be thick or relatively coarse beds deposited during jökulhlaups or exceptionally large storms. The contemporary sediment yield to Bowser Lake, estimated from sediments in the lake, is about 360 t km-2a-1. This is a relatively high value, but it is less than yields insome other, similar montane basins with extensive snow and ice cover.The most likely explanation for the difference is that large amounts of sediment have been, and continue to be, stored on the Bowser delta andin small proglacial lakes. 相似文献