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101.
102.
Chantal Guillard Hervé Delprat Can Hoang-van Pierre Pichat 《Journal of Atmospheric Chemistry》1993,16(1):47-59
The photodegradation of naphthalene (NPH), chosen as a model of polynuclear aromatic pollutants, has been studied in the presence of a layer of four water-insoluble inorganic solids which can be found in the troposphere (TiO2, Fe2O3, muscovite, and a fly ash sample). Direct photolysis of NPH is negligible at >340 nm. Dark adsorption of NPH on TiO2 (mainly anatase, nonporous, 50 m2 g–1) at 293 K corresponds to a surface coverage ofca. 50% at equilibrium. Under these conditions (saturated surface), the stationary-state photocatalytic degradation reaches 0.4 molecule nm–2 h–1 (>340 nm, radiant fluxca. 22 mW cm–2). Dioxygen is required and its partial pressure in air is such that the degradation is zero order in O2. Water vapor markedly increases the rate. The other particulates have also an effect, less important than that of TiO2, however quite noticeable with respect to surface area unit for the fly ash sample which contains 3.2% Fe2O3. Apart from 1,4-naphthoquinone, which is the main intermediate product in all cases, 2-naphthol, phthalide, phthaldialdehyde, phthalic acid, acetophenone, benzaldehyde, benzoic acid are also formed on dry TiO2. Depending on their volatility, these compounds are transferred to the gas phase or remain principally adsorbed on the solid particles where they are further transformed. For instance, phthalic acid (or anhydride) and benzoic acid are generated from 1,4-naphthoquinone. Degradation mechanisms are briefly discussed. 相似文献
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104.
我国地面气温参考站点遴选的依据、原则和方法 总被引:17,自引:0,他引:17
由于城市化和观测环境变化的影响,我国现有国家级气象台站网观测的地面气温资料许多已不能满足气候变化检测研究的要求。利用我国全部气象观测站网的台站信息,对地面气温资料序列质量进行了系统评价,遴选出可用于气温变化研究的参考站点。这项工作建立了地面气温参考站点遴选的原则、方法和步骤,并据此确定了138个地面气温参考站。这些台站可代表背景地面气温场,其长期气温观测资料可用作城市台站或国家级台站城市化增温评价的参考,也可直接用于我国地面气温变化的检测分析。 相似文献
105.
福建沿海赤潮灾害气象预报 总被引:3,自引:0,他引:3
根据福建沿海2001~2008年赤潮灾害资料以及相应时期的气象数据,寻找与赤潮灾害发生密切相关的气象因子,分析赤潮灾害发生期间的地面及不同高度的天气形势,并探讨南方涛动指数与赤潮灾害发生的关系,在此基础上根据前期气温、风、云及海况进行福建沿海赤潮灾害气象预报。研究结果表明,福建沿海的风、气温、湿度、日照和气压等气象因子与赤潮的发生存在着密切的关系,但不同海区影响赤潮发生的主要气象因子不尽相同,低层850 hPa和地面形势能较好地反映福建沿海赤潮发生的天气背景,南方涛动指数与第2年赤潮发生日数有着很好的对应关系,二者相关系数为-0.745。 相似文献
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107.
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109.
A copula-based multivariate analysis of Canadian RCM projected changes to flood characteristics for northeastern Canada 总被引:1,自引:0,他引:1
In the present work, climate change impacts on three spring (March–June) flood characteristics, i.e. peak, volume and duration, for 21 northeast Canadian basins are evaluated, based on Canadian regional climate model (CRCM) simulations. Conventional univariate frequency analysis for each flood characteristic and copula based bivariate frequency analysis for mutually correlated pairs of flood characteristics (i.e. peak–volume, peak–duration and volume–duration) are carried out. While univariate analysis is focused on return levels of selected return periods (5-, 20- and 50-year), the bivariate analysis is focused on the joint occurrence probabilities P1 and P2 of the three pairs of flood characteristics, where P1 is the probability of any one characteristic in a pair exceeding its threshold and P2 is the probability of both characteristics in a pair exceeding their respective thresholds at the same time. The performance of CRCM is assessed by comparing ERA40 (the European Centre for Medium-Range Weather Forecasts 40-year reanalysis) driven CRCM simulated flood statistics and univariate and bivariate frequency analysis results for the current 1970–1999 period with those observed at selected 16 gauging stations for the same time period. The Generalized Extreme Value distribution is selected as the marginal distribution for flood characteristics and the Clayton copula for developing bivariate distribution functions. The CRCM performs well in simulating mean, standard deviation, and 5-, 20- and 50-year return levels of flood characteristics. The joint occurrence probabilities are also simulated well by the CRCM. A five-member ensemble of the CRCM simulated streamflow for the current (1970–1999) and future (2041–2070) periods, driven by five different members of a Canadian Global Climate Model ensemble, are used in the assessment of projected changes, where future simulations correspond to A2 scenario. The results of projected changes, in general, indicate increases in the marginal values, i.e. return levels of flood characteristics, and the joint occurrence probabilities P1 and P2. It is found that the future marginal values of flood characteristics and P1 and P2 values corresponding to longer return periods will be affected more by anthropogenic climate change than those corresponding to shorter return periods but the former ones are subjected to higher uncertainties. 相似文献
110.
湖泊底泥疏浚环境效应:Ⅰ.内源磷释放控制作用 总被引:8,自引:1,他引:8
通过为期一年的疏浚模拟试验,在试验室培养疏浚与对照柱样研究了底泥疏浚对内源磷释放的控制效果.结果发现,疏浚表层30cm能够有效的消减沉积物中不f司形态磷含量与孔隙水中PO4^3-P含量.在一年的试验周期内,疏浚和对照柱沉积物-水界面的PO4^3-P通量分别为-143.8至14.4与-237.3至3047.6μg/(m^2·d),疏浚柱沉积物-水界面的磷通量总体上低于未疏浚对照的磷通量,尤其是在温度较高的月份,从2006年3-10月疏浚柱沉积物-水界面磷释放通量显著低于未疏浚对照柱,疏浚沉积物的磷的释放潜力低于未疏浚对照沉积物.研究结果表明,在外源磷得到有效控制的前提下,底泥疏浚是消减研究区内源磷负荷有效的技术手段. 相似文献