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101.
Christoph Kern Holger Sihler Leif Vogel Claudia Rivera Martha Herrera Ulrich Platt 《Bulletin of Volcanology》2009,71(6):659-670
Active Long Path Differential Optical Absorption Spectroscopy (LP-DOAS) measurements of halogen oxides were conducted at Masaya
Volcano, in Nicaragua from April 14 to 26, 2007. The active LP-DOAS system allowed night-time halogen measurements and reduced
the ClO detection limit by an order of magnitude when compared to previous passive DOAS measurements, as wavelengths below
300 nm could be used for the DOAS retrievals. BrO was detected with an average BrO/SO2 molecular ratio of approximately 3 × 10−5 during the day. However, BrO values were below the detection limit of the instrument for all night-time measurements, a strong
indication that BrO is not directly emitted, but rather the result of photochemical formation in the plume itself according
to the autocatalytic “bromine explosion” mechanism. Despite the increased sensitivity, both ClO and OClO could not be detected.
The achieved upper limits for the X/SO2 ratios were 5 × 10−3 and 7 × 10−6, respectively. A rough calculation suggests that ClO and OClO should be present at similar abundances in volcanic plumes.
Since the DOAS technique is orders of magnitude more sensitive for OClO than for ClO, this indicates that OClO should always
be detectable in plumes in which ClO is found. However, further LP-DOAS studies are needed to conclusively clarify the role
of chlorine oxides in volcanic plumes. 相似文献
102.
On the modifications of near-inertial waves at fronts: implications for energy transfer across scales 总被引:1,自引:1,他引:0
Leif N. Thomas 《Ocean Dynamics》2017,67(10):1335-1350
In the ocean, wind-generated kinetic energy (KE) manifests itself primarily in balanced currents and near-inertial waves. The dynamics of these flows is strongly constrained by the Earth’s rotation, causing the KE in balanced currents to follow an inverse cascade but also preventing wave-wave interactions from fluxing energy in the near-inertial band to lower frequencies and higher vertical wavenumbers. How wind-generated KE is transferred to small-scale turbulence and dissipated is thus a non-trivial problem. This article presents a review of recent theoretical calculations and numerical simulations that demonstrate how some surprising modifications to internal wave physics by the lateral density gradients present at ocean fronts allow for strong interactions between balanced currents and near-inertial waves that ultimately result in energy loss for both types of motion. 相似文献
103.
104.
Patterns in community structure and functioning of motile epibenthic fauna were investigated in shallow (0–1 m) sediment habitats along the Skagerrak–Baltic estuarine gradient (salinity range from 4 to 34). The study area was divided into five regions, reflecting different sea-basins along the 1260 km coastline, and fauna was collected at six sites within each region. Ten replicate samples of motile epibenthic fauna were taken randomly at each site with a portable drop trap (bottom area 1 m2) in June and September in 2004. 相似文献
105.
Based on seismic profiles, multibeam bathymetry and sediment cores, an improved understanding of the deglaciation/postglacial history of the southern part of the Norwegian Channel has been obtained. The Norwegian Channel Ice Stream started to recede from the shelf edge ca. 15.5 ka BP (14C ages are used throughout). Approximately 500–1000 years later the ice margin was located east of the deep Skagerrak trough. At that time, the Norwegian Channel off southern Norway had become a large fjord-like embayment, surrounded by the grounded ice sheet along the northern slope and possibly stagnant ice remnants at the southern flank. The Norwegian Channel off southern Norway has been the main sediment trap of the North Sea, and south of Egersund more than 200 m of sediments have been deposited since the start of the deglaciation. Five seismic units are mapped. The oldest unit E occurs in some of the deepest troughs, and was deposited immediately after the ice became buoyant. Unit D is acoustically massive and comprises mass-movement deposits in eastern Skagerrak and south of Egersund. Unit C (in the channel southwest of Lista/Egersund) is interpreted to comprise mainly bottom current deposits derived from palaeo-rivers, e.g. Elben. During deposition of unit C (ca. 14.5–13 ka BP), there was limited inflow of Atlantic water. A change in depositional environment at ca. 13 ka BP is related to an increased inflow of saline water and more open hydrographic circulation. Widely distributed, acoustically stratified clays of unit B were deposited ca. 13–10 ka BP. The Holocene Unit A shows a depositional pattern broadly similar to that of unit B. 相似文献
106.
Photochemical production of ammonium and transformation of dissolved organic matter in the Baltic Sea 总被引:13,自引:1,他引:13
Colin A. Stedmon Stiig Markager Lars Tranvik Leif Kronberg Tove Sltis Winnie Martinsen 《Marine Chemistry》2007,104(3-4):227-240
The release of ammonium from the photochemical degradation of dissolved organic matter (DOM) has been proposed by earlier studies as a potentially important remineralisation pathway for refractory organic nitrogen. In this study the photochemical production of ammonium from Baltic Sea DOM was assessed in the laboratory. Filtered samples from the Bothnian Bay, the Gulf of Finland and the Arkona Sea were exposed to UVA light at environmentally relevant levels, and the developments in ammonium concentrations, light absorption, fluorescence and molecular size distribution were followed. The exposures resulted in a decrease in DOM absorption and loss of the larger sized fraction of DOM. Analysis of the fluorescence properties of DOM using parallel factor analysis (PARAFAC) identified 6 independent components. Five components decreased in intensity as a result of the UVA exposures. One component was produced as a result of the exposures and represents labile photoproducts derived from terrestrial DOM. The characteristics of DOM in samples from the Bothnian Bay and Gulf of Finland were similar and dominated by terrestrially derived material. The DOM from the Arkona Sea was more autochthonous in character. Photoammonification differed depending on the composition of DOM. Calculated photoammonification rates in surface waters varied between 121 and 382 μmol NH4+ L− 1 d− 1. Estimated areal daily production rates ranged between 37 and 237 μmol NH4+ m− 2 d− 1, which are comparable to atmospheric deposition rates and suggest that photochemical remineralisation of organic nitrogen may be a significant source of bioavailable nitrogen to surface waters during summer months with high irradiance and low inorganic nitrogen concentrations. 相似文献
107.
Ingemar Bergelin Karsten Obst Ulf Söderlund Kent Larsson Leif Johansson 《International Journal of Earth Sciences》2011,100(4):787-804
More than 100 volcanic necks composed of basanites and melanephelinites occur in Scania, southern Sweden, at the junction
of two major tectonic lineaments, the Phanerozoic Sorgenfrei-Tornquist Zone (STZ) and the Proterozoic Protogine Zone. New
40Ar/39Ar isotope analyses of whole rock fragments of nine selected basalt necks suggest that the Mesozoic alkaline volcanism in
the Scanian province commenced earlier than previously reported and comprised three separate volcanic episodes that span a
total period of ca. 80 Myr: a first Jurassic (191–178 Ma), a second at the Jurassic/Cretaceous boundary (ca. 145 Ma), and
a final middle Cretaceous episode (ca. 110 Ma). The new results allow for precise time correlations between eruption events
in the Scanian and those in the North Sea volcanic provinces. The older, early Jurassic event in Scania is largely synchronous
with that in the Egersund Basin and the Forties field whereas the event at ca. 145 Ma is correlated with activity in the Central
Graben. These volcanic episodes also correlate in age with Kimmerian tectonic activity. Volcanic activity in the middle Cretaceous
period has also been dated in the triple junction in the North Sea and offshore in the Netherland Sector. The correlation
of basalt volcanism in Scania with the Egersund nephelinites strongly suggest that volcanism was triggered by repeated tectonic
activity along the STZ. Geochemical data of alkaline mafic rocks in the Scanian and the North Sea volcanic provinces imply
that different provinces have largely unique geochemical signatures in favour of a heterogeneous mantle in the North Sea volcanic
region. However, basalts of different generations in one and the same province cannot be readily separated on the basis of
geochemistry, suggesting that the same lithospheric mantle was the source of repeated volcanism over time in each province.
The data suggest a low degree of melting of a volatile-bearing mantle lherzolite enriched in incompatible elements with the
exception of the Forties basalts in the rift centre, produced by larger degree of melting and evolved by fractional crystallization. 相似文献
108.
Cores taken from an ombrotrophic peat bog in the coastal zone of Halland, southwest Sweden, were examined for wind transported mineral grains, pollen and humidity indicators. The core covers the period from 6500 cal. yr BP to present. Ombrotrophic conditions existed from ca. 4200 cal. yr BP onwards. Bog surface wetness fluctuated strongly until ca. 3700 cal. yr BP, with an apparent dominance of dry summer conditions from 4800–4500 cal. yr BP. Local wet shifts occurred around 4300, 2800, 2400 and 1500 cal. yr BP, whereas the most recent 600 years of the record show increasingly dry conditions. Mineral grain content, interpreted as aeolian sand influx (ASI), was used as a proxy for (winter) storm frequency and intensity until ca. 1500 cal. yr BP, after which increasing human impact, as reconstructed by pollen analysis, became a second important potential cause for increased sand drift. Strongly increased storminess occurred at 4800, 4200, 2800–2200, 1500, 1100 and 400–50 cal. yr BP, indicating a dominance of cold and stormy winters during these periods. Many of these storm periods apparently coincide with storm events in other sites in southwestern Scandinavia, suggesting that our ASI record reflects a regional scale climatic signal. Furthermore these stormy periods correlate to well‐known cold phases in the North Atlantic region, suggesting a link to large‐scale fluctuations in atmospheric circulation patterns. Copyright © 2006 John Wiley & Sons, Ltd. 相似文献
109.
Leif Holmlid 《Icarus》2006,180(2):555-564
The long-lived excited state of matter called Rydberg Matter (RM) may explain several spectroscopic features in space, like the diffuse interstellar bands (DIBs) and the unidentified infrared bands (UIR, UIB). RM is here used to interpret some previously unexplained or inconsistent features in comets: (1) line absorption in the emission from the nucleus, (2) IR band emission from the coma, (3) selective and variable molecular line emission from the coma, (4) extended sources of molecules in the coma, (5) degree of linear polarization of light scattered from the coma. (1) The unexplained IR absorptions observed in the flyby of the nucleus of the Comet Borrelly agree well with RM emission bands observed by stimulated emission in the laboratory. It is proposed that RM is the so-called ultrared matter or at least formed from it. (2) The IR bands previously attributed to silicate particles are shown to be better described by RM theory. Transitions in atoms in RM are shown to dominate. (3) The inverted RM medium will optically amplify light from molecular transitions in the comet comae, in agreement with observations that many of the molecular IR emission lines lie within the emission bands from RM, or much too close to Rydberg transitions to be accidental. (4) The unexplained extended sources observed, e.g., for CO are proposed to be due to release of molecules previously incorporated in the RM clusters at low temperature. Such clusters may be the very small particles observed by space probes. (5) Finally, the largely unexplained measurements of the degree of linear polarization of scattered sunlight from comets are explained as due to scattering by the planar RM clusters. Quantitative agreement is demonstrated. 相似文献
110.
Leif Holmlid 《Astrophysics and Space Science》2006,305(1):91-98
The detailed processes giving maser line radiation from various molecules in space are not well understood, as can be seen from many recent detailed studies of maser line emission with high spatial and velocity resolution, and with polarization measurements. We now propose an improved maser mechanism based on amplification of the original molecular line emission by stimulated emission in Rydberg Matter (RM) clouds in HII regions, containing clusters H
N
and (H2)
N
. This mechanism will amplify the molecular lines, depending on the position, velocity, cluster size and state of excitation of the clusters in the RM cloud. RM will only support certain frequencies, corresponding to rotational transitions of the clusters. The bond lengths in the RM clusters are known within 1% from radio frequency emission measurements in the laboratory, and it is now shown that all the commonly studied maser lines agree well with stimulated emission transitions in several types of RM clusters simultaneously. This may explain the strongly varying intensities of neighboring or related maser lines, an important effect that is not well understood previously. It is also pointed out that the magnetic field due to RM is of the same order of magnitude as observed from the Zeeman splitting in maser lines; thus, the molecules that are the original sources of the lines may be embedded in the RM clouds, for example in dense HII regions that are likely to be RM regions. 相似文献