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W. Shotyk M.E. Goodsite F. Roos-Barraclough N. Givelet G. Le Roux A.K. Cheburkin J. Heinemeier S.A. Norton 《Geochimica et cosmochimica acta》2005,69(1):1-17
A monolith representing 5420 14C yr of peat accumulation was collected from a blanket bog at Myrarnar, Faroe Islands. The maximum Hg concentration (498 ng/g at a depth of 4.5 cm) coincides with the maximum concentration of anthropogenic Pb (111 μg/g). Age dating of recent peat accumulation using 210Pb (CRS model) shows that the maxima in Hg and Pb concentrations occur at AD 1954 ± 2. These results, combined with the isotopic composition of Pb in that sample (206Pb/207Pb = 1.1720 ± 0.0017), suggest that coal burning was the dominant source of both elements. From the onset of peat accumulation (ca. 4286 BC) until AD 1385, the ratios Hg/Br and Hg/Se were constant (2.2 ± 0.5 × 10-4 and 8.5 ± 1.8 × 10-3, respectively). Since then, Hg/Br and Hg/Se values have increased, also reaching their maxima in AD 1954. The age date of the maximum concentrations of anthropogenic Hg and Pb in the Faroe Islands is consistent with a previous study of peat cores from Greenland and Denmark (dated using the atmospheric bomb pulse curve of 14C), which showed maximum concentrations in AD 1953.The average rate of atmospheric Hg accumulation from 1520 BC to AD 1385 was 1.27 ± 0.38 μg/m2/yr. The Br and Se concentrations and the background Hg/Br and Hg/Se ratios were used to calculate the average rate of natural Hg accumulation for the same period, 1.32 ± 0.36 μg/m2/yr and 1.34 ± 0.29 μg/m2/yr, respectively. These fluxes are similar to the preanthropogenic rates obtained using peat cores from Switzerland, southern Greenland, southern Ontario, Canada, and the northeastern United States. Episodic volcanic emissions and the continual supply of marine aerosols to the Faroe Islands, therefore, have not contributed significantly to the Hg inventory or the Hg accumulation rates, relative to these other areas. The maximum rate of Hg accumulation was 34 μg/m2/yr. The greatest fluxes of anthropogenic Hg accumulation calculated using Br and Se, respectively, were 26 and 31 μg/m2/yr. The rate of atmospheric Hg accumulation in 1998 (16 μg/m2/yr) is comparable to the values recently obtained by atmospheric transport modeling for Denmark, the Faroe Islands, and Greenland. 相似文献
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David L. Poulsen Craig T. Simmons Corinne Le Galle La Salle Jim W. Cox 《Hydrogeology Journal》2006,14(7):1339-1359
Understanding catchment-scale patterns of groundwater and stream salinity are important in land- and water-salinity management. A large-scale assessment of groundwater and stream data was undertaken in the eastern Mt Lofty Ranges of South Australia using geographical information systems (GIS), regional scale hydrologic data, hydrograph separation and hydrochemical techniques. Results of the study show: (1) salts were mostly of marine origin (75%), while sulfate and bicarbonate from mineral weathering comprised most of the remainder, (2) elevated groundwater salinities and stable water isotopic compositions similar to mean rainfall indicated that plant transpiration was the primary salt accumulation mechanism, (3) key factors explaining groundwater salinity were geology and rainfall, with overall catchment salinity inversely proportional to average annual rainfall, and groundwater salinity ‘hotspots’ (EC >8 mS/cm) associated with geological formations comprising sulfidic marine siltstones and shales, (4) shallow groundwater correlated with elevated stream salinity, implying that baseflow contributed to stream salt loads, with most of the annual salt load (estimated to be 24,500 tonnes) occurring in winter when baseflow volume was highest. Salt-load analysis using stream data could be a practical, low-cost technique to rapidly target the investigation of problem areas within a catchment. 相似文献
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O. Malam Issa Y. Le Bissonnais O. Planchon David Favis‐Mortlock Norbert Silvera John Wainwright 《地球表面变化过程与地形》2006,31(8):929-939
Field‐ and laboratory‐scale rainfall simulation experiments were carried out in an investigation of the temporal variability of erosion processes on interrill areas, and the effects of such variation upon sediment size characteristics. Poorly aggregated sandy soils from the semi‐arid environment of Senegal, West Africa, were used on both a 40 m2 field plot and a 0·25 m2 laboratory plot; rainfall intensity for all experiments was 70 mm h?1 with a duration of 1 to 2 hours. Time‐series measurements were made of the quantity and the size distribution of eroded material: these permitted an estimate of the changing temporal balance between the main erosion processes (splash and wash). Results from both spatial scales showed a similar temporal pattern of runoff generation and sediment concentration. For both spatial scales, the dominant erosional process was detachment by raindrops; this resulted in a dynamic evolution of the soil surface under raindrop impact, with the rapid formation of a sieving crust followed by an erosion crust. However, a clear difference was observed between the two scales regarding the size of particles detached by both splash and wash. While all measured values were lower than the mean weight diameter (MWD) value of the original soil (mean 0·32 mm), demonstrating the size‐selective nature of wash and splash processes, the MWD values of washed and splashed particles at the field scale ranged from 0·08 to 0·16 mm and from 0·12 to 0·30 mm respectively, whereas the MWD values of washed and splashed particles at the laboratory scale ranged from 0·13 to 0·29 mm and from 0·21 to 0·32 mm respectively. Thus only at the field scale were the soil particles detached by splash notably coarser than those transported by wash. This suggests a transport‐limited erosion process at the field scale. Differences were also observed between the dynamics of the soil loss by wash at the two scales, since results showed wider scatter in the field compared to the laboratory experiments. This scatter is probably related to the change in soil surface characteristics due to the size‐selectivity of the erosion processes at this spatial scale. Copyright © 2006 John Wiley & Sons, Ltd. 相似文献
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C. J. Farrugia H. K. Biernat N. V. Erkaev L. M. Kistler G. Le C. T. Russell 《Annales Geophysicae》1998,16(5):518-527
We compare numerical results obtained from a steady-state MHD model of solar wind flow past the terrestrial magnetosphere with documented observations made by the AMPTE/IRM spacecraft on 24 October, 1985, during an inbound crossing of the magnetosheath. Observations indicate that steady conditions prevailed during this about 4 hour-long crossing. The magnetic shear at spacecraft entry into the magnetosphere was 15°. A steady density decrease and a concomitant magnetic field pile-up were observed during the 40 min interval just preceding the magnetopause crossing. In this plasma depletion layer (1) the plasma beta dropped to values below unity; (2) the flow speed tangential to the magnetopause was enhanced; and (3) the local magnetic field and velocity vectors became increasingly more orthogonal to each other as the magnetopause was approached (Phan et al., 1994). We model parameter variations along a spacecraft orbit approximating that of AMPTE/IRM, which was at slightly southern GSE latitudes and about 1.5 h postnoon Local Time. We model the magnetopause as a tangential discontinuity, as suggested by the observations, and take as input solar wind parameters those measured by AMPTE/IRM just prior to its bow shock crossing. We find that computed field and plasma profiles across the magnetosheath and plasma depletion layer match all observations closely. Theoretical predictions on stagnation line flow near this low-shear magnetopause are confirmed by the experimental findings. Our theory does not give, and the data on this pass do not show, any localized density enhancements in the inner magnetosheath region just outside the plasma depletion layer. 相似文献
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SCIPION is a new state of the art digital sounder that has been developed by France Telecom-CNET for ionospheric monitoring and research. Extensive data processing using DSP technology has resulted in a low power, low cost and full featured system for both vertical and oblique soundings. A SCIPION system is in the process of being installed in Dakar, Senegal, to study HF propagation in the sub-equatorial ionosphere. However, preliminary results have still been obtained during experiments wit a prototype system. In this paper, the system is described and some illustrative examples of its capabilities are shown. 相似文献
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