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271.
Andrew J. Mason Gideon M. Henderson Anton Vaks 《Geostandards and Geoanalytical Research》2013,37(3):261-275
A new method for the simultaneous recovery of U, Th and Pb from ca. 0.5 g calcium carbonate samples for the purpose of U‐(Th)‐Pb geochronometry is presented. The protocol employs ion‐exchange chromatography. Standard anion exchange resin (AG 1‐X8 100–200 mesh) was used as the static phase, and 90% acetic acid was used as the mobile phase to elute the unwanted matrix components; dilute nitric acid was used to elute the U, Th and Pb. Blanks of 1.8 pg Th, 6.4 pg Pb and 8.4 pg U were obtained. The protocol was evaluated by determining the isotopic composition of U‐Th‐Pb separates obtained from an in‐house reference material (prepared from a natural speleothem) by MC‐ICP‐MS. An independently dated speleothem was also reanalysed. Based on these tests, the extraction protocol had an acceptable blank and produced a Pb separate sufficiently free of matrix‐induced instrumental biases to be appropriate for U‐Th‐Pb chronology. 相似文献
272.
M. A. Muñoz A. Faz J. A. Acosta S. Martínez-Martínez J. M. Arocena 《Environmental Earth Sciences》2013,69(1):141-149
Gold mining activities in Apolobamba area, northwest of La Paz, Bolivia have created serious environmental concern and great risk to human health. The current methods used to extract gold are too primitive resulting in metal contamination of soil and water. The objectives of this study were to: (1) determine the degree of metal pollution, and (2) assess the risk to human health and environment in the Apolobamba area. Soil, water, sediment samples, and mine spills were collected and analyzed. Metals including Pb, Cu, Zn, Cd, and Hg concentrations were higher in surface soils than in subsurface soils indicating active atmospheric deposition of metals. Sediment samples had elevated levels of metals probably from mine spills discharged into the Sunchulli River. Surface soils in the Sunchulli community show the highest levels of Pb and Hg in all soil samples and may pose a risk to the health of the human population and environment. 相似文献
273.
Emmanuel Jacquet Marine Paulhiac‐Pison Olivier Alard Anton T. Kearsley Matthieu Gounelle 《Meteoritics & planetary science》2013,48(10):1981-1999
We report trace element analyses by laser ablation inductively coupled plasma mass spectrometry (LA‐ICP‐MS) of metal grains from nine different CR chondrites, distinguishing grains from chondrule interior (“interior grains”), chondrule surficial shells (“margin grains”), and the matrix (“isolated grains”). Save for a few anomalous grains, Ni‐normalized trace element patterns are similar for all three petrographic settings, with largely unfractionated refractory siderophile elements and depleted volatile Au, Cu, Ag, S. All three types of grains are interpreted to derive from a common precursor approximated by the least‐melted, fine‐grained objects in CR chondrites. This also excludes recondensation of metal vapor as the origin of the bulk of margin grains. The metal precursors were presumably formed by incomplete condensation, with evidence for high‐temperature isolation of refractory platinum‐group‐element (PGE)‐rich condensates before mixing with lower temperature PGE‐depleted condensates. The rounded shape of the Ni‐rich, interior grains shows that they were molten and that they equilibrated with silicates upon slow cooling (1–100 K h?1), largely by oxidation/evaporation of Fe, hence their high Pd content, for example. We propose that Ni‐poorer, amoeboid margin grains, often included in the pyroxene‐rich periphery common to type I chondrules, result from less intense processing of a rim accreted onto the chondrule subsequent to the melting event recorded by the interior grains. This means either that there were two separate heating events, which formed olivine/interior grains and pyroxene/margin grains, respectively, between which dust was accreted around the chondrule, or that there was a single high‐temperature event, of which the chondrule margin records a late “quenching phase,” in which case dust accreted onto chondrules while they were molten. In the latter case, high dust concentrations in the chondrule‐forming region (at least three orders of magnitude above minimum mass solar nebula models) are indicated. 相似文献
274.
Rodríguez-Ortega MJ Rodríguez-Ariza A Gómez-Ariza JL Muñoz-Serrano A López-Barea J 《Marine pollution bulletin》2009,58(1):64-327
Molecular biomarkers are among the most sensitive and earliest responses to pollutants. However, lack of detailed knowledge on variability of responses and their possible seasonal variation limit their use. In addition, the seasonality of biological processes modulates the response of organisms to pollutant stressors. Using multivariate statistics, we have studied the influence of environmental and biological factors on the response of a battery of molecular biomarkers in the clam Chamaelea gallina collected along the South-Spanish littoral. Multivariate discriminant analysis clearly distinguished biomarker response between clean and polluted areas, using heavy metals as indicator of pollution. Such differences disappeared when the dataset was normalised for metal content, thus indicating that pollution was the main significant cause of the changes observed between clean and polluted sites. In conclusion, this work shows that, when applying a complete biomarker panel, multivariate statistical tools can be used to discern pollutant- from non pollutant-related responses. 相似文献
275.
276.
The study of overland flow of water over an erodible sediment leads to a coupled model describing the evolution of the topographic
elevation and the depth of the overland water film. The spatially uniform solution of this model is unstable, and this instability
corresponds to the formation of rills, which in reality then grow and coalesce to form large-scale river channels. In this
paper we consider the deduction and mathematical analysis of a deterministic model describing river channel formation and
the evolution of its depth. The model involves a degenerate nonlinear parabolic equation (satisfied on the interior of the
support of the solution) with a super-linear source term and a prescribed constant mass. We propose here a global formulation
of the problem (formulated in the whole space, beyond the support of the solution) which allows us to show the existence of
a solution and leads to a suitable numerical scheme for its approximation. A particular novelty of the model is that the evolving
channel self-determines its own width, without the need to pose any extra conditions at the channel margin. 相似文献
277.
Maria V. Pastor Josep L. Pelegrí Alonso Hernández-Guerra Jordi Font Jordi Salat Mikhail Emelianov 《Continental Shelf Research》2008
A historical data set is used to describe the coastal transition zone off Northwest Africa during spring 1973 and fall 1975, from 17° to 26°N, with special emphasis on the interaction between subtropical (North Atlantic Central Waters) and tropical (South Atlantic Central Waters) gyres. The near-surface geostrophic circulation, relative to 300 m, is quite complex. Major features are a large cyclonic pattern north of Cape Blanc (21°N) and offshore flow at the Cape Verde front. The large cyclone occurs in the region of most intense winds, and resembles a large meander of the baroclinic southward upwelling jet. The Cape Verde frontal system displays substantial interleaving that may partly originate as mesoscale features at the coastal upwelling front. Property–property diagrams show that the front is an effective barrier to all properties except temperature. The analysis of the Turner angle suggests that the frontal system is characterized by large heat horizontal diffusion as a result of intense double diffusion, which results in the smoothing of the temperature horizontal gradients. Nine cross-shore sections are used to calculate along-shore geostrophic water-mass and nutrient transports and to infer exchanges between the coastal transition zone and the deep ocean (import: deep ocean to transition zone; export: transition zone to deep ocean). These exchanges compare well with mean wind-induced transports and actual geostrophic cross-shore transport estimates. The region is divided into three areas: southern (18–21°N), central (21–23.5°N), and northern (23.5–26°N). In the northern area geostrophic import is roughly compensated with wind-induced export during both seasons. In the central area geostrophic import is greater than wind-induced export during spring, resulting in net import of both water (0.8 Sv) and nitrate (14 kmol s−1), but during fall both factors again roughly cancel. In the southern area geostrophy and wind join to export water and nutrients during both seasons, they increase from 0.6 Sv and 3 kmol s−1 during fall to 2.9 Sv and 53 kmol s−1 during spring. 相似文献
278.
Chris Harris H. Stuart Smith Anton P. le Roex 《Contributions to Mineralogy and Petrology》2000,138(2):164-175
We have measured the δ18O values of the major phenocrysts (olivine, clinopyroxene and plagioclase) present in lavas from Tristan da Cunha and Gough
Island. These islands, which result from the same mantle plume, have enriched radiogenic isotope ratios and are, therefore,
prime candidates for an oxygen isotope signature that is distinct from that of MORB. Consistent differences between the δ18O values of olivine, pyroxene and feldspar in the Gough lavas show that the phenocrysts in the mafic Gough Island lavas are
in oxygen isotope equilibrium. The olivines in lavas with SiO2 <50 wt% have a mean δ18O value of 5.19‰, consistent with crystallization from a magma having the same oxygen isotope composition as MORB. Phenocrysts
in all the Gough lavas show a systematic increase in δ18O value as silica content increases, which is consistent with closed-system fractional crystallization. The lack of enrichment
in δ18O of the Gough magmas suggests that the mantle source contained <2% recycled sediment. In contrast, the Tristan lavas with
SiO2 >48 wt% contain phenocrysts which have δ18O values that are systematically ∼0.3‰ lower than their counterparts from Gough. We suggest that the parental mafic Tristan
magmas were contaminated by material from the volcanic edifice that acquired low δ18O values by interaction with water at high temperatures. The highly porphyritic SiO2-poor lavas show a negative correlation between olivine δ18O value and whole-rock silica content rather than the expected positive correlation. The minimum δ18O value occurs at an SiO2 content of about 45 wt%. Below 45 wt% SiO2, magmas evolved via a combination of assimilation, fractionational crystallization and crystal accumulation; above 45 wt%
SiO2, magmas appeared to have evolved via closed-system fractional crystallization.
Received: 23 November 1998 / Accepted: 27 September 1999 相似文献
279.
280.
J. J. Álvaro E. Vennin A. Muñoz B. Sánchez-Valverde J. L. Ojeda 《International Journal of Earth Sciences》2000,89(2):366-376
The stratigraphy of carbonate/shale couplets, cycles and cycle-stacking patterns in a Cambrian shallow water platform (Iberian
Chains, NE Spain) are related to sea-level changes driven by orbital forcing and by tectonic pulses. The interplay of both
effects can be discriminated in the Iberian fault-controlled platform, in which the tectonic activity can be analysed by accurate
and detailed biostratigraphic correlations based on trilobite zonation. The stratigraphic hierarchy of rhythmically interbedded
limestones and shales, in two coeval but structurally separated geodynamic settings, yields cycle ratios of 1.44 :1. This
ratio is supported by time thickness and spectral analysis, which is based on a graphic method of analysis: the Map of Grey
Lines. The cycle ratio seems to be evidence for orbital forcing by obliquity and precession cycles predicted for early Paleozoic
time. Carbonate/shale couplets, the smallest rhythmic units recognisable in the field, represent short-term, periodic fluctuations
in supply of terrigenous sediments and carbonate productivity of uncertain origin, which could be associated with one of several
harmonics of the former orbital cycles. The pulsating tectonic activity was approximated by using a quantitative analysis
of tectonically induced subsidence (Shaw method). Recurrence frequencies of tectonic pulses were estimated and dated by biostratigraphy.
As a result, tectonic disturbances in the Cambrian Iberian platform show an episodic periodicity comparable to that of orbital
eccentricity cycles, which could mask their recognition.
Received: 15 November 1999 / Accepted: 9 February 2000 相似文献