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101.
Jean-François Lambert Lorenzo Stievano Irène Lopes Marwen Gharsallah Lingyu Piao 《Planetary and Space Science》2009,57(4):460-21825
We present here selected results recently obtained on the molecular characterization of amino acids adsorption on oxide minerals and their further polymerization by thermal activation, in the general frame of assessing Bernal's hypothesis on the origin of biopolymers on mineral surfaces. Adsorption mechanisms may be identified by a combination of vibrational spectroscopy, 13C solid-state NMR, and molecular modeling. Depending on a particular amino acid, the oxide surface investigated, and the water activity during adsorption (i.e., whether it is carried out from the gas phase or from an aqueous solution), contributions from electrostatic adsorption, outer-sphere and inner-sphere (coordination) complexes may be observed. These mechanisms result in significant adsorption selectivities from equimolar mixtures of different amino acids. Upon thermal activation at moderate temperatures (150-160 °C), clean polymerization events occur and can easily be observed by thermogravimetric analysis. There are some hints of selectivity in this step too. The water activity during thermal treatment plays an important role for the thermodynamics of polymerization. 相似文献
102.
Resurfacing of Titan by ammonia-water cryomagma 总被引:1,自引:0,他引:1
The Cassini Titan Radar Mapper observed on Titan several large features interpreted as cryovolcanic during the October 26, 2004 pass at high northern latitudes [Lopes, R.M.C., and 43 colleagues, 2007. Icarus 186, 395-412]. To date, models of ammonia-water resurfacing have not been tied to specific events or evolutionary stages of Titan. We propose a model of cryovolcanism that involves cracking at the base of the ice shell and formation of ammonia-water pockets in the ice. As these ammonia-water pockets undergo partial freezing in the cold ice shell, the ammonia concentration in the pockets increases, decreasing the negative buoyancy of the ammonia-water mixture. If the ice shell is contaminated by silicates delivered in impacts, the liquid-solid density difference would be even less. While the liquid cannot easily become buoyant relative to the surrounding ice, these concentrated ammonia-water pockets are sufficiently close to the neutral buoyancy point that large-scale tectonic stress patterns (tides, non-synchronous rotation, satellite volume changes, solid state convection, or subsurface pressure gradients associated with topography) would enable the ammonia to erupt effusively onto the surface. Rather than suggesting steady-state volcanism over the history of the Solar System, we favor a scenario where the cryovolcanic features could have been associated with episodic (potentially late) geological activity. 相似文献
103.
José Miguel Reichert José Carlos de Deus Junior Norton Borges Junior Rosane Barbosa Lopes Cavalcante 《水文研究》2021,35(8):e14285
The introduction of exotic, fast-growing forest species in the Pampa biome (Southern Grasslands) is a controversial topic, considering the potential effect on water and soil resources. This repository contains hydrologic data (rainfall, discharge and turbidity) collected since 2011 in three small (≤1.1 km2), paired experimental catchments of the “Ponta da Canas” site, in the Pampa biome in subtropical Brazil. Two catchments are predominantly covered with eucalyptus plantations, and one with livestock-grazing degraded grassland. For each catchment, the collected data include 10-min resolution rainfall, streamflow, and turbidity (except for one of the eucalyptus catchments), automatically recorded in 10-min intervals. In each catchment, rainfall is measured with an automatic tipping-bucket rain gauge; stream depth is determined with a pressure transducer at the spillway, and a rating curve is used to estimate discharge; and turbidity is measured with a turbidimeter. The collected data are being used to understand water balance and sediment production under the distinct land uses, to improve forest management, and comply with State legislation. 相似文献
104.
Short-term variability of multiple biomarker response in fish from estuaries: Influence of environmental dynamics 总被引:1,自引:0,他引:1
Fonseca VF França S Vasconcelos RP Serafim A Company R Lopes B Bebianno MJ Cabral HN 《Marine environmental research》2011,72(4):172-178
Short-term variability in biomarker responses and the effects of temperature and salinity variation were explored in three fish species (Dicentrarchus labrax, Solea senegalensis and Pomatoschistus microps) occurring in the Tejo estuary. Short-term variability in biomarkers was observed in all species although no pattern was discerned over time (days to weeks). Antioxidant enzymes activity (superoxide dismutase (SOD) and catalase (CAT)) showed low temporal variability, indicating some constancy or baseline level in antioxidant responses. Only CAT activity in S.?senegalensis was correlated with temperature, suggesting that exposure to contaminants triggered antioxidant acclimation. Higher short-term variability was observed in xenobiotic biotransformation enzymes activity (phase I ethoxyresorufin O-deethylase (EROD) and phase II glutathione S-transferase (GST)). Yet a significant correlation between EROD and GST in D.?labrax and S.?senegalensis suggests a concomitant response to contaminants. Moreover the lack of correlation between xenobiotic biotransformation enzymes and abiotic variables on concordant time scales, suggest a high specificity of these biomarkers to chemical exposure, rather than high variability due to environmental dynamics. 相似文献
105.
Helena Coelho Teresa Lopes da Silva Alberto Reis Henrique Queiroga João Serôdio Ricardo Calado 《Estuarine, Coastal and Shelf Science》2011
Mud snails Hydrobia ulvae occupy different habitats in complex estuarine ecosystems. In order to determine if fatty acid profiles displayed by mud snails can be used to identify the habitat that they occupy within the same estuary, fatty acids of H. ulvae from one mudflat and one seagrass meadow in the Ria de Aveiro (Portugal) were analyzed and compared to those displayed by microphytobenthos (MPB), the green leaves (epiphyte-free) of Zostera noltii, as well as those exhibited by the epiphytic community colonizing this seagrass. MPB and epiphytic diatom-dominated samples displayed characteristic fatty acids, such as 16:1n-7 and 20:5n-3, while 18:2n-6 and 18:3n-3 were the dominant fatty acids in the green leaves of Z. noltii. Significant differences between the fatty acid profiles of H. ulvae specimens sampled in the mudflat and the seagrass meadow could be identified, with those from the mudflat displaying higher levels of fatty acids known to be characteristic of MPB. This result points towards the well known existence of grazing activity on MPB by mud snails. The fatty acid profiles displayed by H. ulvae inhabiting the seagrass meadows show no evidence of direct bioaccumulation of the two most abundant polyunsaturated fatty acids of Z. noltii (18:2n-6 and 18:3n-3) in the mud snails, which probably indicates that either these compounds can be metabolized to produce energy, used as precursors for the synthesis of essential fatty acids, or that the snails do not consume seagrass leaves at all. Moreover, the fatty acid profiles of mud snails inhabiting the seagrass meadows revealed the existence of substantial inputs from microalgae, suggesting that the epiphytic community colonizing the leaves of Z. noltii displays an important role on the diet of these organisms. This assumption is supported by the high levels of 20:5n-3 and 22:6n-3 recorded in mud snails sampled from seagrass meadows. In conclusion, fatty acid analyses of H. ulvae can be successfully used to identify the habitat occupied by these organisms within the same estuary (e.g. mudflats and seagrass meadows) and reveal the existence of contrasting dietary regimes. 相似文献
106.
107.
Kannan K. R. Iyer Jeevan Joseph Bruna C. F. L. Lopes D. N. Singh Alessandro Tarantino 《Geomechanics and Geoengineering》2018,13(2):88-103
The soil–water retention (SWR) characteristics of the clays play an important role in controlling their engineering behaviour, particularly, in the unsaturated state. Although, researchers have attempted to understand the water retention characteristics of the clays in their reconstituted or remoulded state, such studies are rare for the clays in their intact state. In this context, it becomes important to understand the influence of initial state of compaction, which would create different pore and fabric structure (viz., microstructure), on the water retention characteristics of the clays. With this in view, SWR behaviour was experimentally determined for the swelling clays (dried from different compaction states, viz., intact, reconstituted and remoulded) by employing Dewpoint PotentiaMeter (WP4C®). The changes in the pore size distribution of the clays at different stages of drying cycle were also studied by employing the Mercury Intrusion Porosimetry. The study reveals that the SWR curves for the intact and reconstituted specimens of the clays converge beyond a certain stage of drying. Also, a critical analysis of changes in the pore structure of the swelling clay specimens, during drying, indicates that the progressively deforming pore structure plays an important role in controlling its water retention characteristics to a great extent. 相似文献
108.
F. Paganelli M.A. Janssen R. West J.I. Lunine S.D. Wall R.M. Lopes R.L. Kirk L. Roth the Radar Team 《Icarus》2007,191(1):211-222
The first five Titan flybys with Cassini's Synthetic Aperture RADAR (SAR) and radiometer are examined with emphasis on the calibration and interpretation of the high-resolution radiometry data acquired during the SAR mode (SAR-radiometry). Maps of the 2-cm wavelength brightness temperature are obtained coincident with the SAR swath imaging, with spatial resolution approaching 6 km. A preliminary calibration shows that brightness temperature in these maps varies from 64 to 89 K. Surface features and physical properties derived from the SAR-radiometry maps and SAR imaging are strongly correlated; in general, we find that surface features with high radar reflectivity are associated with radiometrically cold regions, while surface features with low radar reflectivity correlate with radiometrically warm regions. We examined scatterplots of the normalized radar cross-section σ0 versus brightness temperature, finding differing signatures that characterize various terrains and surface features. Implications for the physical and compositional properties of these features are discussed. The results indicate that volume scattering is important in many areas of Titan's surface, particularly Xanadu, while other areas exhibit complex brightness temperature variations consistent with variable slopes or surface material and compositional properties. 相似文献
109.
Loki is the largest patera and the most energetic hotspot on Jupiter's moon Io, in turn the most volcanically active body in the Solar System, but the nature of the activity remains enigmatic. We present detailed analysis of Galileo Near-Infrared Mapping Spectrometer (NIMS) and PhotoPolarimeter/Radiometer (PPR) observations covering the 1.5-100 μm wavelength range during the I24, I27, and I32 flybys. The general pattern of activity during these flybys is consistent with previously proposed models of a resurfacing wave periodically crossing a silicate lava lake. In particular our analysis of the I32 NIMS observations shows, over much of the observed patera, surface temperatures and implied ages closely matching those expected for a wave advancing counterclockwise at 0.94-1.38 km/day. The age pattern is different than other published analyses which do not show as clearly this azimuthal pattern. Our analysis also shows two additional distinctly different patera surfaces. The first is located along the inner and outer margins where components with a 3.00-4.70-μm color temperature of 425 K exist. The second is located at the southwestern margin where components with a 550-K color temperature exist. Although the high temperatures could be caused by disruption of a lava lake crust, some additional mechanism is required to explain why the southwest margin is different from the inner or outer ones. Finally, analysis of the temperature profiles across the patera reveal a smoothness that is difficult to explain by simple lava cooling models. Paradoxically, at a subpixel level, wide temperature distributions exist which may be difficult to explain by just the presence of hot cracks in the lava crust. The resurfacing wave and lava cooling models explain well the overall characteristics of the observations. However, additional physical processes, perhaps involving heat transport by volatiles, are needed to explain the more subtle features. 相似文献
110.
Leandro Duarte Campos Sulsiene Machado de Souza Diogo Alves de Sordi Felipe Mattos Tavares Evandro Luiz Klein Elem Cristina dos Santos Lopes 《Natural Resources Research》2017,26(4):509-534
The Gurupi Belt hosts a Paleoproterozoic gold province located in north–northeastern Brazil, at the borders of Pará and Maranhão states. It is considered to be an extension of the prolific West African Craton’s Birimian gold province into South America. Additionally, the belt has been the object of recent mineral exploration programs with significant resource discoveries. This study presents the results of predictive mapping using up-to-date mineral system concepts and recently finished regional-scale geological mapping, stream sediment and airborne geophysical surveys conducted by the Geological Survey of Brazil. We relate gold mineralization to an initially enriched crust, metamorphism, deep fluid pathways, structurally controlled damage zones and hydrothermal alteration. Prospective targets were generated using only regional public datasets and knowledge-driven targeting technique. This work did not incorporate any known gold deposits, yet it predicted the largest known deposits and their satellite targets. Besides, high prospective targets mapped almost 40% of known primary gold occurrences within 7% of the project area. This work allowed considerable search area reduction and identification of new target areas, thus collaborating on reducing costs, time and risk of mineral exploration. Results indicate that we achieved an efficient understanding of the geological processes related to the Gurupi Belt mineral system. 相似文献