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101.
Harald Geiger Ian Barnes Karl H. Becker Birger Bohn Theo Brauers Birgit Donner Hans-Peter Dorn Manfred Elend Carlos M. Freitas Dinis Dirk Grossmann Heinz Hass Holger Hein Axel Hoffmann Lars Hoppe Frank Hülsemann Dieter Kley Björn Klotz Hans G. Libuda Tobias Maurer Djuro Mihelcic Geert K. Moortgat Romeo Olariu Peter Neeb Dirk Poppe Lars Ruppert Claudia G. Sauer Oleg Shestakov Holger Somnitz William R. Stockwell Lars P. Thüner Andreas Wahner Peter Wiesen Friedhelm Zabel Reinhard Zellner Cornelius Zetzsch 《Journal of Atmospheric Chemistry》2002,42(1):323-357
Within the German Tropospheric Research Programme (TFS) numerous kinetic and mechanistic studies on the tropospheric reaction/degradation of the following reactants were carried out: oxygenated VOC, aromatic VOC, biogenic VOC, short-lived intermediates, such as alkoxy and alkylperoxy radicals.At the conception of the projects these selected groups were classes of VOC or intermediates for which the atmospheric oxidation mechanisms were either poorly characterised or totally unknown. The motivation for these studies was the attainment of significant improvements in our understanding of the atmospheric chemical oxidation processes of these compounds, particularly with respect to their involvement in photooxidant formation in the troposphere. In the present paper the types of experimental investigations performed and the results obtained within the various projects are briefly summarised. The major achievements are highlighted and discussed in terms of their contribution to improving our understanding of the chemical processes controlling photosmog formation in the troposphere. 相似文献
102.
Enforcing smoothness and assessing uncertainty in non-linear one-dimensional prestack seismic inversion 总被引:1,自引:0,他引:1
Estimation of elastic properties of rock formations from surface seismic amplitude measurements remains a subject of interest for the exploration and development of hydrocarbon reservoirs. This paper develops a global inversion technique to estimate and appraise 1D distributions of compressional‐wave velocity, shear‐wave velocity and bulk density, from normal‐moveout‐corrected PP prestack surface seismic amplitude measurements. Specific objectives are: (a) to evaluate the efficiency of the minimization algorithm (b) to appraise the impact of various data misfit functions, and (c) to assess the effect of the degree and type of smoothness criterion enforced by the inversion. Numerical experiments show that very fast simulated annealing is the most efficient minimization technique among alternative approaches considered for global inversion. It is also found that an adequate choice of data misfit function is necessary for a reliable and efficient match of noisy and sparse seismic amplitude measurements. Several procedures are considered to enforce smoothness of the estimated 1D distributions of elastic parameters, including predefined quadratic measures of length, flatness and roughness. Based on the general analysis of global inversion techniques, we introduce a new stochastic inversion algorithm that initializes the search for the minimum with constrained random distributions of elastic parameters and enforces predefined autocorrelation functions (semivariograms). This strategy readily lends itself to the assessment of model uncertainty. The new global inversion algorithm is successfully tested on noisy synthetic amplitude data. Moreover, we present a feasibility analysis of the resolution and uncertainty of prestack seismic amplitude data to infer 1D distributions of elastic parameters measured with wireline logs in the deepwater Gulf of Mexico. The new global inversion algorithm is computationally more efficient than the alternative global inversion procedures considered here. 相似文献
103.
Vyacheslav M. Zobin Carlos J. Navarro-Ochoa Gabriel A. Reyes-Dávila 《Bulletin of Volcanology》2006,69(2):141-147
In July–August 2003, the andesitic lava dome at Volcán de Colima, México, was destroyed by a sequence of explosions that replaced the 2×106 m3 dome with a crater 200 m across and 30 m deep. The two strongest explosions occurred on July 17 and August 28. The initial low-frequency impulses that they produced, which were recorded on broadband seismic records, allowed an estimation of the counter forces of the initiating process as being equal to 0.3×1011 N and 1×1011 N for the July and August events, respectively. The seismic characteristics follow the Nishimura-Hamaguchi scaling law for volcanic explosions, reflecting self-similarity in the processes initiating explosive events. The results also show that counter forces can discriminate between the sizes of explosive eruptions that are assigned the same magnitude by conventional methods of classification such as the Volcanic Explosivity Index. The increasing use of broadband seismometers may therefore provide the basis for using counter forces to determine the magnitude of explosive eruptions. 相似文献
104.
Breno L. Waichel Evandro F. de Lima Romulo Lubachesky Carlos A. Sommer 《Bulletin of Volcanology》2006,68(7-8):599-610
Inflated and compound pahoehoe flows have been identified within the central Paraná Continental Flood Basalts based upon their morphology, surface features, and internal zonation. Pahoehoe flow features have been studied at five localities in the western portion of Paraná State, Brazil: Ponte Queimada, Toledo, Rio Quitéria, Matelandia and Cascavel. We have interpreted the newly recognized flow features using concepts of Hawaiian pahoehoe formation and emplacement that have been previously applied to the Columbia River Basalt and Deccan Plateau. Surface features and/or internal structure typical from pahoehoe lavas are observed in all studied areas and features like inflation clefts, squeeze-ups, breakouts, and P-type lobes with two levels of pipe vesicles are indicative of inflation in these flows. The thinner, compound pahoehoe flows are predominantly composed of P-type lobes and probably emerged at the end of large inflated flows on shallow slopes. The presence of vesicular cores in the majority of compound lobes and the common occurrence of segregation structures suggests high water content in the pahoehoe lavas from the central PCFB. More volcanological studies are necessary to determinate the rheology of lavas and refine emplacement models.Editorial responsibility: C. Kilburn 相似文献
105.
Juan Carlos Bergmann 《Boundary-Layer Meteorology》2006,119(1):171-179
Precision measurements indicate that the stability capping of the neutral planetary boundary layer (PBL) that leads to a reduced
PBL height is caused by the very stable upper part of the PBL, rather than by an overlying inversion. Radiative processes
related to liquid water in boundary-layer clouds seem to play the key role for the formation of the stable upper PBL. The
famous Leipzig Profile – generally considered as an example of a neutral PBL – has been included in Hess’s analysis because
its PBL height is considerably lower than the ca. 3000 m to be expected by numerical models in truly neutral conditions. An
analysis of the original observations reveals that the Leipzig PBL was stable and that it can be consistently treated as a
‘normal’ stable PBL with a height of ca. 700 m. A further finding is that the super-geostrophic PBL wind speed maxima predicted
by almost all models are not observed in near-steady-state conditions. For the ‘ranking’ of analytical models versus numerical
models, the comparisons with measurements show that the analytical models perform comparably well and even partially better
than the numerical models. 相似文献
106.
The evolution of pore-water and the composition of solid phases in the vadose zone of pyritic tailings was studied by means of unsaturated column experiments. Several columns of water-saturated mine tailings were dried during 125 days under controlled laboratory conditions. The columns were dismantled at four successive drying stages and the evolution of pore-water, mineralogy, water content and temperature was characterized.Sulfide and aluminosilicate minerals present in the waste dissolved, releasing sulfate and other solutes (mainly Fe, Zn, Cu, Al, Mg and Ca) to the pore-water. Evaporation caused a crust of efflorescent, water-soluble sulfates to develop over the complete top surface of the columns and into the pores of the underlying waste material. This crust, which has also been identified in the field, changed the hydraulic properties of the tailings and produced a decrease in the evaporation rate of the columns. Moreover, these water-soluble precipitates (mainly rozenite, szomolnokite, halotrichite, hexahydrite, mirabilite and gypsum) acted as temporary sinks for Cd, Pb, Co and Ni, which could be released to the surface run-off or the groundwaters during rainfall events under field conditions.Pore-water evolution was determined not only by geochemical processes (dissolution of sulfides and aluminosilicates, precipitation of secondary phases) but also by thermal and hydraulic processes. Progressive dilution was observed in the lower part of the columns. Dilution was caused by the thermally driven vapor flux from the top of the column to its colder bottom and subsequent condensation therein. This process, which may also occur in tailings under sub-arid climate, played a key role on the evolution of pore-water with increasing drying. 相似文献
107.
For nearly a decade the La Paz-El Alto concession in Bolivia was heralded by donor organizations, the state and the commercial water industry alike as an emblematic ‘pro-poor’ water concession under the private sector model. Managed by one of the largest water multinationals in the world (the French company Suez), the network was extended beyond the new connections required by the original ‘pro-poor’ contract, acclaimed as a pioneer of new pro-poor technologies and frequently disseminated internationally as an example of best practice. This paper analyses the La Paz-El Alto concession’s pro-poor image focusing on issues of social exclusion and network extension, contract negotiation, participation and transparency. It documents the rise of social protest about the concession and critiques the failure of neoliberal regulatory systems to promote accountability to the poor. In the context of the continued transnationalisation of the water industry the paper highlights the need for new mechanisms and delivery models to ensure greater national control over private companies and the development of a framework for international water governance. 相似文献
108.
Aloísio J.B. Cotta Jacinta Enzweiler Stephen A. Wilson Carlos A. Pérez Antonio J.R. Nardy João H. Larizzatti 《Geostandards and Geoanalytical Research》2007,31(4):379-393
Reference materials (RM) are required for quantitative analyses and their successful use is associated with the degree of homogeneity, and the traceability and confidence limits of the values established by characterisation. During the production of a RM, the chemical characterisation can only commence after it has been demonstrated that the material has the required level of homogeneity. Here we describe the preparation of BRP-1, a proposed geochemical reference material, and the results of the tests to evaluate its degree of homogeneity between and within bottles. BRP-1 is the first of two geochemical RM being produced by Brazilian institutions in collaboration with the United States Geological Survey (USGS) and the International Association of Geoanalysts (IAG). Two test portions of twenty bottles of BRP-1 were analysed by wavelength dispersive-XRF spectrometry and major, minor and eighteen trace elements were determined. The results show that for most of the investigated elements, the units of BRP-1 were homogeneous at conditions approximately three times more rigorous than those strived for by the test of "sufficient homogeneity". Furthermore, the within bottle homogeneity of BRP-1 was evaluated using small beam (1 mm2 ) synchrotron radiation XRF spectrometry and, for comparison, the USGS reference materials BCR-2 and GSP-2 were also evaluated. From our data, it has been possible to assign representative minimum masses for some major constituents (1 mg) and for some trace elements (1-13 mg), except Zr in GSP-2, for which test portions of 74 mg are recommended. 相似文献
109.
110.
Mock 2dF and SDSS galaxy redshift surveys 总被引:1,自引:0,他引:1