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141.
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The launch of the P78-2 (SCATHA) satellite in January 1979 has provided a new opportunity to study the energetic ion composition in the high altitude equatorial regions of the earth's magnetosphere. In particular detailed pitch angle distributions were obtained as a function of ion species and energy. The energies measured range from ~ 90 to 250 keV/nucleon for Z ? 2. Data are presented which were acquired in late March and early April 1979. The relative abundance of He and CNO nuclei are found to be ~ 10?2 and 5 × 10?4 respectively at L ? 5.5. Only an upper limit on the relative abundance of Fe group nuclei of < 3 × 10?7 was obtained. The angular distributions of the heavy ions was found to be very steep for and then to flatten markedly. 相似文献
143.
Buckling-restrained braces(BRBs)have recently become popular in the United States for use as primary members of seismic lateral-force-resisting systems.A BRB is a steel brace that does not buckle in compression but instead yields in both tension and compression.Although design guidelines for BRB applications have been developed,systematic procedures for assessing performance and quantifying reliability are still needed.This paper presents an analytical framework for assessing buckling-restrained braced f... 相似文献
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Iron (III) oxides are ubiquitous in near-surface soils and sediments and interact strongly with dissolved phosphates via sorption, co-precipitation, mineral transformation and redox-cycling reactions. Iron oxide phases are thus, an important reservoir for dissolved phosphate, and phosphate bound to iron oxides may reflect dissolved phosphate sources as well as carry a history of the biogeochemical cycling of phosphorus (P). It has recently been demonstrated that dissolved inorganic phosphate (DIP) in rivers, lakes, estuaries and the open ocean can be used to distinguish different P sources and biological reaction pathways in the ratio of 18O/16O (δ18OP) in PO43−. Here we present results of experimental studies aimed at determining whether non-biological interactions between dissolved inorganic phosphate and solid iron oxides involve fractionation of oxygen isotopes in PO4. Determination of such fractionations is critical to any interpretation of δ18OP values of modern (e.g., hydrothermal iron oxide deposits, marine sediments, soils, groundwater systems) to ancient and extraterrestrial samples (e.g., BIF’s, Martian soils). Batch sorption experiments were performed using varied concentrations of synthetic ferrihydrite and isotopically-labeled dissolved ortho-phosphate at temperatures ranging from 4 to 95 °C. Mineral transformations and morphological changes were determined by X-Ray, Mössbauer spectroscopy and SEM image analyses.Our results show that isotopic fractionation between sorbed and aqueous phosphate occurs during the early phase of sorption with isotopically-light phosphate (P16O4) preferentially incorporated into sorbed/solid phases. This fractionation showed negligible temperature-dependence and gradually decreased as a result of O-isotope exchange between sorbed and aqueous-phase phosphate, to become insignificant at greater than ∼100 h of reaction. In high-temperature experiments, this exchange was very rapid resulting in negligible fractionation between sorbed and aqueous-phase phosphate at much shorter reaction times. Mineral transformation resulted in initial preferential desorption/loss of light phosphate (P16O4) to solution. However, the continual exchange between sorbed and aqueous PO4, concomitant with this mineralogical transformation resulted again in negligible fractionation between aqueous and sorbed PO4 at long reaction times (>2000 h). This finding is consistent with results obtained from natural marine samples. Therefore, 18O values of dissolved phosphate (DIP) in sea water may be preserved during its sorption to iron-oxide minerals such as hydrothermal plume particles, making marine iron oxides a potential new proxy for dissolved phosphate in the oceans. 相似文献
148.
Craig Stroud Sasha Madronich Elliot Atlas Christopher Cantrell Alan Fried Brian Wert Brian Ridley Fred Eisele Lee Mauldin Richard Shetter Barry Lefer Frank Flocke Andy Weinheimer Mike Coffey Brian Heikes Robert Talbot Donald Blake 《Journal of Atmospheric Chemistry》2004,47(2):107-138
Local ozone production and loss rates for the arctic free troposphere (58–85° N, 1–6 km, February–May) during the TroposphericOzone Production about the Spring Equinox (TOPSE) campaign were calculated using a constrained photochemical box model. Estimates were made to assess the importance of local photochemical ozone production relative to transport in accounting for the springtime maximum in arctic free tropospheric ozone. Ozone production and loss rates from our diel steady-state box model constrained by median observations were first compared to two point box models, one run to instantaneous steady-state and the other run to diel steady-state. A consistent picture of local ozone photochemistry was derived by all three box models suggesting that differences between the approaches were not critical. Our model-derived ozone production rates increased by a factor of 28 in the 1–3 km layer and a factor of 7 in the 3–6 kmlayer between February and May. The arctic ozone budget required net import of ozone into the arctic free troposphere throughout the campaign; however, the transport term exceeded the photochemical production only in the lower free troposphere (1–3 km) between February and March. Gross ozone production rates were calculated to increase linearly with NOx mixing ratiosup to 300 pptv in February and for NOx mixing ratios up to 500 pptv in May. These NOx limits are an order of magnitude higher thanmedian NOx levels observed, illustrating the strong dependence ofgross ozone production rates on NOx mixing ratios for the majority of theobservations. The threshold NOx mixing ratio needed for netpositive ozone production was also calculated to increase from NOx 10pptv in February to 25 pptv in May, suggesting that the NOx levels needed to sustain net ozone production are lower in winter than spring. This lower NOx threshold explains how wintertime photochemical ozone production can impact the build-up of ozone over winter and early spring. There is also an altitude dependence as the threshold NOx neededto produce net ozone shifts to higher values at lower altitudes. This partly explains the calculation of net ozone destruction for the 1–3 km layerand net ozone production for the 3–6 km layer throughout the campaign. 相似文献
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150.
B.F. Blake T.J. Dixon P.H. Jones M.L. Tasker 《Estuarine, Coastal and Shelf Science》1985,20(5):559-568
Stomach contents were examined from 750 guillemots collected at several sites in the northern North Sea. The dietary composition was compared between months and between localities in order to assess seasonal and geographical trends in feeding strategy.From March to August sandeels dominated the diet, but in September a changeover period occurred when clupeid and gadoid remains became increasingly frequent in the stomach contents. This situation persisted over the winter period, but the importance of the two fish families varied with area, clupeids being more important in more southerly samples and gadoids in the north. Dietary data were considered in relation to available fisheries information and to known guillemot distribution patterns. 相似文献