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761.
Rolf?S.?ArvidsonEmail author Cornelius?Fischer Andreas?Luttge 《Aquatic Geochemistry》2015,21(5):415-422
We compare the canonical treatment of calcite’s dissolution rate from the literature in a closed system, particle batch reactor, with the alternative approach suggested by Truesdale (Aquat Geochem, 2015). We show that the decay of rate over time can be understood in terms of the evolution and distribution of reactive sites on the surface of these particles. We also emphasize that interpretation of observed rates must not exclude the fundamental role of crystal defects, whose importance is already implicitly reflected in the common form of rate laws in geochemistry. The empirical behavior of overall rate in closed systems, such as those described by Truesdale, may thus reflect relationships between defect centers and the generation of steps over the calcite surface (previously documented for silicates), such that below a critical free energy limit, there is insufficient driving force to open hollow cores and thus a loss of reaction mechanism. Dissolution in this very-near-equilibrium regime will be dependent on the distribution of extant steps and the energetics of new kink site nucleation. However, these sensitivities are complicated in the case of particle systems by grain boundaries, edges, corners, and other terminations. Such discontinuities constitute a defect class whose overall kinetic importance will be strongly tied to particle diameter and which can act independently of the internal strain field imposed by screw and edge dislocations. 相似文献
762.
763.
Black hole astrophysics is expected to have a major breakthrough any day. Theoretical understanding is well advanced, so the breakthrough has to come from observers. Conclusive and direct evidence of event horizons, signatures of tidal deformation of gas clouds (and eventual disappearance of matter behind horizons) could be obtained in matter of months. At this juncture, we wish to summarize how the subject came to this stage and what is the state-of-the-art flow solution around a black hole. We touch upon the most crucial issue of (un)predictability of this subject. We believe that if viscosity is roughly what MRI simulations are pointing to us, we still require very detailed knowledge of properties of the companion, especially time dependent mass transfer from the companion to the black hole. 相似文献
764.
Progressive failure leading to the 3 December 2013 rockfall at Puigcercós scarp (Catalonia,Spain) 总被引:1,自引:1,他引:0
A detailed analysis of the pre-failure behavior of the 3 December 2013 rockfall (1,012 m3) occurred on Puigcercós pilot study area (Catalonia, Spain) is presented. The exact date of failure was obtained based on a photographic monitoring performed every 4 h. The long-term monitoring (2,217 days) of the rock slope carried out by a Terrestrial LiDAR allowed the early detection of both pre-failure deformation and precursory rockfalls preceding the final failure. By means of the analysis of the pre-failure deformation, four different deformed areas were detected and the tertiary creep phase was observed in three of them. An attempt to predict the time to failure was performed using the Fukuzono’s (1985) method. Furthermore, the temporal evolution of the precursory rockfalls occurred in those four areas during the progressive failure showed a close resemblance with the exponential pattern of the cumulated displacements at tertiary creep stage. Finally, the study of the meteorological conditions did not show any single triggering factor associated with the final failure. Reversely, the increase in the occurrence of precursory rockfalls on several areas of the slope together with the observed acceleration on the deformation pattern reinforce the role of a progressive degradation of the stability conditions, which ultimately leaded to the 3 December rockfall event. 相似文献
765.
通过沉积物岩石学特征、粒度分布特征、沉积构造与生物化石特征、单井分析等综合方法,对志靖—安塞地区长9油层组沉积相发育及分布特征进行了研究。结果表明,鄂尔多斯盆地志靖—安塞地区在首次湖侵期长9期发育三角洲-湖泊沉积体系,主要发育三角洲前缘亚相和浅湖亚相。长92期研究区北部大面积发育三角洲前缘沉积,西南部发育小面积三角洲前缘沉积,浅湖面积较小,呈喇叭状向东南方向开口。长91期沉积格局基本上继承了长92期的特点,但浅湖的范围有所加大。三角洲前缘水下分流河道砂体整体上呈北东—南西向条带状展布。长9期湖侵过程形成了具生烃潜力的泥岩,主要分布在吴起—志丹—安塞一带,在志丹东南部区域最厚,可达20m,并呈现向东南方向继续变厚延伸的趋势。储集空间的存在和烃源岩的发育使得研究区长9储层具有较好的勘探前景。 相似文献
766.
This work presents the refractory black carbon(rBC)results of a snow and firn core drilled in West Antarctica(79°55'34.6"S,94°21'13.3"W)during the 2014?15 austral summer,collected by Brazilian researchers as part of the First Brazilian West Antarctic Ice Sheet Traverse.The core was drilled to a depth of 20 m,and we present the results of the first 8 m by comparing two subsampling methods—solid-state cutting and continuous melting—both with discrete sampling.The core was analyzed at the Department of Geological Sciences,Central Washington University(CWU),WA,USA,using a single particle soot photometer(SP2)coupled to a CETAC Marin-5 nebulizer.The continuous melting system was recently assembled at CWU and these are its first results.We also present experimental results regarding SP2 reproducibility,indicating that sample concentration has a greater influence than the analysis time on the reproducibility for low rBC concentrations,like those found in the Antarctic core.Dating was carried out using mainly the rBC variation and sulfur,sodium and strontium as secondary parameters,giving the core 17 years(1998?2014).The data show a well-defined seasonality of rBC concentrations for these first meters,with geometric mean summer/fall concentrations of 0.016μg L^?1 and geometric mean winter/spring concentrations of 0.063μg L^?1.The annual rBC concentration geometric mean was 0.029μg L^?1(the lowest of all rBC cores in Antarctica referenced in this work),while the annual rBC flux was 6.1μg m^?2 yr^?1(the lowest flux in West Antarctica records so far). 相似文献
767.
768.
利用多种常规观测资料和NCEP/NCAR再分析资料,分析了2017年3月1日江苏北部出现的一次罕见冷空气雷雨大风天气过程的发生背景、地面要素和云团演变特征,同时从大气动力、热力和水汽条件出发分析了午后对流的成因。结果表明:此次过程发生前,江苏地区位于高空槽前,对流层中低层有冷式切变线伴随两股冷空气南下,受江苏省北部地面气旋阻挡,冷空气在上游堆积,当气旋东移入海冷空气爆发式南下时,造成严重的大风灾害。此次过程中,对流层中高层大气降温而低层回温使大气温度直减率增大,为对流发生提供不稳定条件,但水汽输送主要集中在低层,且高层大气无明显抽吸作用,导致此次过程未发生强对流性降水,主要以大风灾害性天气为主。 相似文献
769.
Kochendorfer et al. (Boundary-Layer Meterol, 145:383–398, 2012) conducted an experiment to evaluate azimuth and angle-of-attack dependent errors of sonic anemometer measurements. Several questions are raised regarding the experimental design and the presented results. The finding that instruments with non-orthogonal sonic paths underestimate fluctuations of vertical wind speed and consequently also scalar fluxes by about 10 % is compared with the results of a hitherto unpublished side-by-side field comparison and other past intercomparison experiments. Scale considerations are presented that raise considerable doubts on the validity of the implicit assumption of Kochendorfer et al. (2012) that the turbulent wind vector is highly correlated across a distance of 1.2 m at a height of 2.5 m over flat grassland, which corresponds to the separation between the sonic anemometers tested in their experiment. Nevertheless, new developments in sonic anemometer design to minimize transducer-shadow effects are desirable. 相似文献
770.