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Dieke Postma Søren Jessen Mai Thanh Duc Pham Hung Viet Flemming Larsen 《Geochimica et cosmochimica acta》2010,74(12):3367-508
Sediments from the Red River and from an adjacent floodplain aquifer were investigated with respect to the speciation of Fe and As in the solid phase, to trace the diagenetic changes in the river sediment upon burial into young aquifers, and the related mechanisms of arsenic release to the groundwater. Goethite with subordinate amounts of hematite were, using Mössbauer spectroscopy, identified as the iron oxide minerals present in both types of sediment. The release kinetics of Fe, As, Mn and PO4 from the sediment were investigated in leaching experiments with HCl and 10 mM ascorbic acid, both at pH 3. From the river sediments, most of the Fe and As was mobilized by reductive dissolution with ascorbic acid while HCl released very little Fe and As. This suggests As to be associated with an Fe-oxide phase. For oxidized aquifer sediment most Fe was mobilized by ascorbic acid but here not much As was released. However, the reduced aquifer sediments contained a large pool of Fe(II) and As that is readily leached by HCl, probably derived from an unidentified authigenic Fe(II)-containing mineral which incorporates As as well. Extraction with ascorbic acid indicates that the river sediments contain both As(V) and As(III), while the reduced aquifer sediment almost exclusively releases As(III). The difference in the amount of Fe(II) leached from river and oxidized aquifer sediments by ascorbic acid and HCl, was attributed to reductive dissolution of Fe(III). The reactivity of this pool of Fe(III) was quantified by a rate law and compared to that of synthetic iron oxides. In the river mud, Fe(III) had a reactivity close to that of ferrihydrite, while the river sand and oxidized aquifer sediment exhibited a reactivity ranging from lepidocrocite or poorly crystalline goethite to hematite. Mineralogy by itself appears to be a poor predictor of the iron oxide reactivity in natural samples using the reactivity of synthetic Fe-oxides as a reference. Sediments were incubated, both unamended and with acetate added, and monitored for up to 2 months. The river mud showed the fastest release of both Fe and As, while the effect of acetate addition was minor. This suggests that the presence of reactive organic carbon is not rate limiting. In the case of the river and aquifer sediments, the release of Fe and As was always stimulated by acetate addition and here reactive organic carbon was clearly the rate limiting factor. The reduced aquifer sediment apparently can sustain slower but prolonged microbially-driven release of As. The highly reactive pools of Fe(III) and As in the river mud could be due to reoxidation of As and Fe contained in the reducing groundwater from the floodplain aquifers that are discharging into the river. Deposition of the suspended mud on the floodplain during high river stages is proposed to be a major flux of As onto the floodplain and into the underlying aquifers. 相似文献
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塔里木盆地塔中-巴楚地区上奥陶统良里塔格组米兰科维奇旋回性沉积记录研究 总被引:3,自引:0,他引:3
通过露头、钻井岩芯沉积相观察及高频旋回识别,结合全岩碳氧同位素旋回、自然伽玛能谱测井ln(Th/K)值频谱分析及地震反射特征,研究了塔里木盆地塔中—巴楚地区分布的上奥陶统良里塔格组开阔台地及外缓坡相碳酸盐岩中发育的四~六级高频层序(旋回)特征及其叠置关系。认为其六级米级旋回、五级准层序及四级准层序组可能分别与20~40ka、100ka及400ka周期的Milankovitch日-地轨道气候旋回有关,并识别出该区良里塔格组由11~12个400ka周期的准层序组构成。提出海相碳酸盐岩全岩或生物壳碳同位素值可作为反映全球海平面相对变化的指标及识别形成三级层序的主控因素(全球海平面变化、地区性构造沉降-抬升运动)的方法——碳同位素-沉积旋回对比分析法。晚奥陶世良里塔格组沉积时期,塔中台地北缘总体表现为向上变浅的加积型沉积叠置型式,主要与塔中I号断裂活动控制形成的高陡型镶边台地边缘有关;巴楚台地西北缘则表现为向上变浅的加积-进积复合型沉积叠置型式,主要与其断裂活动弱、受沉积作用控制为主的缓坡台地边缘有关。塔中-巴楚台地良里塔格组表现为一个完整三级层序的形成与演化,主要受控于该台地的构造(沉降-抬升)运动而不是全球海平面变化,属于典型的地区性构造层序及不具有全球对比意义。 相似文献
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河流相层序地层及岩性油气藏油气富集规律——以准噶尔盆地红29三维工区为例 总被引:1,自引:1,他引:0
以准噶尔盆地红山嘴油田红29三维工区中三叠统克拉玛依下亚组(克下组)为研究对象,根据钻井和测井资料对其进行高分辨率层序地层划分,识别出1个长期基准面旋回和3个中期基准面旋回(MSC1、MSC2、MSC3).在长期基准面旋回从上升到下降的过程中,河道弯曲指数明显出现低-高-低的分异特征,河道砂体连续性表现为好-差-好的演变.通过分析克下组油藏以及出油气特征,发现油气主要富集于MSC2中期基准面旋回中;该中期旋回内河道弯曲度较高,河道砂体连续性较差.结合岩性油气藏的成藏规律,总结出"富砂中找贫砂"的勘探思路.该思路指出,长期基准面上升到最高位置附近的"贫砂"层系也是岩性油气藏发育的有利层位,并提出断层-岩性型复合圈闭为有利的勘探目标. 相似文献